Coherence of nitrogen-vacancy electronic spin ensembles in diamond

We present an experimental and theoretical study of electronic spin decoherence in ensembles of nitrogen-vacancy (NV) color centers in bulk high-purity diamond at room temperature. Under appropriate conditions, we find ensemble NV spin coherence times (T[superscript 2]) comparable to that of single...

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Bibliographic Details
Main Authors: Stanwix, P. L., Pham, L. M., Maze, Jeronimo R., Le Sage, David, Yeung, T. K., Cappellaro, Paola, Hemmer, P. R., Yacoby, A., Lukin, M. D., Walsworth, R. L.
Other Authors: Massachusetts Institute of Technology. Department of Nuclear Science and Engineering
Format: Article
Language:en_US
Published: American Physical Society 2011
Online Access:http://hdl.handle.net/1721.1/64424
https://orcid.org/0000-0003-3207-594X
Description
Summary:We present an experimental and theoretical study of electronic spin decoherence in ensembles of nitrogen-vacancy (NV) color centers in bulk high-purity diamond at room temperature. Under appropriate conditions, we find ensemble NV spin coherence times (T[superscript 2]) comparable to that of single NV with T[superscript 2]>600 μs for a sample with natural abundance of [superscript 13]C and paramagnetic impurity density ~10[superscript 15] cm[superscript −3]. We also observe a sharp decrease in the coherence time with misalignment of the static magnetic field relative to the NV electronic spin axis, consistent with theoretical modeling of NV coupling to a [superscript 13]C nuclear-spin bath. The long coherence times and increased signal-to-noise provided by room-temperature NV ensembles will aid many applications of NV centers in precision magnetometry and quantum information.