Thermal Conductivity Spectroscopy Technique to Measure Phonon Mean Free Paths

Size effects in heat conduction, which occur when phonon mean free paths (MFPs) are comparable to characteristic lengths, are being extensively explored in many nanoscale systems for energy applications. Knowledge of MFPs is essential to understanding size effects, yet MFPs are largely unknown for m...

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Main Authors: Schmidt, A. J., Minnich, Austin Jerome, Johnson, Jeremiah A., Esfarjani, Keivan, Dresselhaus, Mildred, Nelson, Keith Adam, Chen, Gang
Other Authors: Massachusetts Institute of Technology. Department of Chemistry
Format: Article
Language:en_US
Published: American Physical Society (APS) 2012
Online Access:http://hdl.handle.net/1721.1/68676
https://orcid.org/0000-0001-8492-2261
https://orcid.org/0000-0002-3968-8530
https://orcid.org/0000-0001-7804-5418
https://orcid.org/0000-0001-9157-6491
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author Schmidt, A. J.
Minnich, Austin Jerome
Johnson, Jeremiah A.
Esfarjani, Keivan
Dresselhaus, Mildred
Nelson, Keith Adam
Chen, Gang
author2 Massachusetts Institute of Technology. Department of Chemistry
author_facet Massachusetts Institute of Technology. Department of Chemistry
Schmidt, A. J.
Minnich, Austin Jerome
Johnson, Jeremiah A.
Esfarjani, Keivan
Dresselhaus, Mildred
Nelson, Keith Adam
Chen, Gang
author_sort Schmidt, A. J.
collection MIT
description Size effects in heat conduction, which occur when phonon mean free paths (MFPs) are comparable to characteristic lengths, are being extensively explored in many nanoscale systems for energy applications. Knowledge of MFPs is essential to understanding size effects, yet MFPs are largely unknown for most materials. Here, we introduce the first experimental technique which can measure MFP distributions over a wide range of length scales and materials. Using this technique, we measure the MFP distribution of silicon for the first time and obtain good agreement with first-principles calculations.
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spelling mit-1721.1/686762022-10-02T05:36:22Z Thermal Conductivity Spectroscopy Technique to Measure Phonon Mean Free Paths Schmidt, A. J. Minnich, Austin Jerome Johnson, Jeremiah A. Esfarjani, Keivan Dresselhaus, Mildred Nelson, Keith Adam Chen, Gang Massachusetts Institute of Technology. Department of Chemistry Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science Massachusetts Institute of Technology. Department of Mechanical Engineering Chen, Gang Minnich, Austin Jerome Johnson, Jeremiah A. Esfarjani, Keivan Dresselhaus, Mildred Nelson, Keith Adam Chen, Gang Size effects in heat conduction, which occur when phonon mean free paths (MFPs) are comparable to characteristic lengths, are being extensively explored in many nanoscale systems for energy applications. Knowledge of MFPs is essential to understanding size effects, yet MFPs are largely unknown for most materials. Here, we introduce the first experimental technique which can measure MFP distributions over a wide range of length scales and materials. Using this technique, we measure the MFP distribution of silicon for the first time and obtain good agreement with first-principles calculations. United States. Dept. of Energy. Office of Basic Energy Sciences (Grant No. DE-SC0001299/DE-FG02-09ER46577) Center for Clean Water and Clean Energy at MIT and KFUPM National Science Foundation (U.S.) 2012-01-27T18:08:05Z 2012-01-27T18:08:05Z 2011-08 2011-05 Article http://purl.org/eprint/type/JournalArticle 0031-9007 1079-7114 http://hdl.handle.net/1721.1/68676 Minnich, A. et al. “Thermal Conductivity Spectroscopy Technique to Measure Phonon Mean Free Paths.” Physical Review Letters 107.9 (2011): n. pag. Web. 27 Jan. 2012. © 2011 American Physical Society https://orcid.org/0000-0001-8492-2261 https://orcid.org/0000-0002-3968-8530 https://orcid.org/0000-0001-7804-5418 https://orcid.org/0000-0001-9157-6491 en_US http://dx.doi.org/10.1103/PhysRevLett.107.095901 Physical Review Letters Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. application/pdf American Physical Society (APS) APS
spellingShingle Schmidt, A. J.
Minnich, Austin Jerome
Johnson, Jeremiah A.
Esfarjani, Keivan
Dresselhaus, Mildred
Nelson, Keith Adam
Chen, Gang
Thermal Conductivity Spectroscopy Technique to Measure Phonon Mean Free Paths
title Thermal Conductivity Spectroscopy Technique to Measure Phonon Mean Free Paths
title_full Thermal Conductivity Spectroscopy Technique to Measure Phonon Mean Free Paths
title_fullStr Thermal Conductivity Spectroscopy Technique to Measure Phonon Mean Free Paths
title_full_unstemmed Thermal Conductivity Spectroscopy Technique to Measure Phonon Mean Free Paths
title_short Thermal Conductivity Spectroscopy Technique to Measure Phonon Mean Free Paths
title_sort thermal conductivity spectroscopy technique to measure phonon mean free paths
url http://hdl.handle.net/1721.1/68676
https://orcid.org/0000-0001-8492-2261
https://orcid.org/0000-0002-3968-8530
https://orcid.org/0000-0001-7804-5418
https://orcid.org/0000-0001-9157-6491
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