Experimental characterization of coherent magnetization transport in a one-dimensional spin system

We experimentally characterize the non-equilibrium, room-temperature magnetization dynamics of a spin chain evolving under an effective double-quantum (DQ) Hamiltonian. We show that the Liouville space operators corresponding to the magnetization and the two-spin correlations evolve 90 degrees out o...

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Main Authors: Ramanathan, Chandrasekhar, Cappellaro, Paola, Viola, Lorenza, Cory, David G.
Other Authors: Massachusetts Institute of Technology. Department of Nuclear Science and Engineering
Format: Article
Language:en_US
Published: Institute of Physics Publishing 2012
Online Access:http://hdl.handle.net/1721.1/70848
https://orcid.org/0000-0003-3207-594X
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author Ramanathan, Chandrasekhar
Cappellaro, Paola
Viola, Lorenza
Cory, David G.
author2 Massachusetts Institute of Technology. Department of Nuclear Science and Engineering
author_facet Massachusetts Institute of Technology. Department of Nuclear Science and Engineering
Ramanathan, Chandrasekhar
Cappellaro, Paola
Viola, Lorenza
Cory, David G.
author_sort Ramanathan, Chandrasekhar
collection MIT
description We experimentally characterize the non-equilibrium, room-temperature magnetization dynamics of a spin chain evolving under an effective double-quantum (DQ) Hamiltonian. We show that the Liouville space operators corresponding to the magnetization and the two-spin correlations evolve 90 degrees out of phase with each other, and drive the transport dynamics. For a nearest-neighbor-coupled N-spin chain, the dynamics are found to be restricted to a Liouville operator space whose dimension scales only as N2, leading to a slow growth of multi-spin correlations. Even though long-range couplings are present in the real system, we find excellent agreement between the analytical predictions and our experimental results, confirming that leakage out of the restricted Liouville space is slow on the timescales investigated. Our results indicate that the group velocity of the magnetization is 6.04 ± 0.38 μm s−1, corresponding to a coherent transport over N ≈ 26 spins on the experimental timescale. As the DQ Hamiltonian is related to the standard one-dimensional XX Hamiltonian by a similarity transform, our results can be directly extended to XX quantum spin chains, which have been extensively studied in the context of both quantum magnetism and quantum information processing.
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spelling mit-1721.1/708482022-10-03T09:02:12Z Experimental characterization of coherent magnetization transport in a one-dimensional spin system Ramanathan, Chandrasekhar Cappellaro, Paola Viola, Lorenza Cory, David G. Massachusetts Institute of Technology. Department of Nuclear Science and Engineering Cappellaro, Paola Cappellaro, Paola We experimentally characterize the non-equilibrium, room-temperature magnetization dynamics of a spin chain evolving under an effective double-quantum (DQ) Hamiltonian. We show that the Liouville space operators corresponding to the magnetization and the two-spin correlations evolve 90 degrees out of phase with each other, and drive the transport dynamics. For a nearest-neighbor-coupled N-spin chain, the dynamics are found to be restricted to a Liouville operator space whose dimension scales only as N2, leading to a slow growth of multi-spin correlations. Even though long-range couplings are present in the real system, we find excellent agreement between the analytical predictions and our experimental results, confirming that leakage out of the restricted Liouville space is slow on the timescales investigated. Our results indicate that the group velocity of the magnetization is 6.04 ± 0.38 μm s−1, corresponding to a coherent transport over N ≈ 26 spins on the experimental timescale. As the DQ Hamiltonian is related to the standard one-dimensional XX Hamiltonian by a similarity transform, our results can be directly extended to XX quantum spin chains, which have been extensively studied in the context of both quantum magnetism and quantum information processing. United States. National Security Agency (NSA under ARO contract number W911NF0510469) National Science Foundation (U.S.) (award 0702295) National Science Foundation (U.S.) (DMR-1005926) National Science Foundation (U.S.) (PHY-0903727) Canada Excellence Research Chairs Program 2012-05-16T18:42:44Z 2012-05-16T18:42:44Z 2011-10 2011-06 Article http://purl.org/eprint/type/JournalArticle 1367-2630 http://hdl.handle.net/1721.1/70848 Ramanathan, Chandrasekhar et al. “Experimental Characterization of Coherent Magnetization Transport in a One-dimensional Spin System.” New Journal of Physics 13.10 (2011): 103015. Web. https://orcid.org/0000-0003-3207-594X en_US http://dx.doi.org/10.1088/1367-2630/13/10/103015 New Journal of Physics Creative Commons Attribution 3.0 http://creativecommons.org/licenses/by/3.0/ application/pdf Institute of Physics Publishing New Journal of Physics
spellingShingle Ramanathan, Chandrasekhar
Cappellaro, Paola
Viola, Lorenza
Cory, David G.
Experimental characterization of coherent magnetization transport in a one-dimensional spin system
title Experimental characterization of coherent magnetization transport in a one-dimensional spin system
title_full Experimental characterization of coherent magnetization transport in a one-dimensional spin system
title_fullStr Experimental characterization of coherent magnetization transport in a one-dimensional spin system
title_full_unstemmed Experimental characterization of coherent magnetization transport in a one-dimensional spin system
title_short Experimental characterization of coherent magnetization transport in a one-dimensional spin system
title_sort experimental characterization of coherent magnetization transport in a one dimensional spin system
url http://hdl.handle.net/1721.1/70848
https://orcid.org/0000-0003-3207-594X
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