Basal-plane nonlinear susceptibility: A direct probe of the single-ion physics in URu2Si2

he microscopic nature of the hidden order state in URu[subscript 2]Si[subscript 2] is dependent on the low-energy configurations of the uranium ions, and there is currently no consensus on whether it is predominantly 5f[supercript 2] or 5f[supercript 3]. Here we show that measurement of the basal-pl...

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Main Authors: Flint, Rebecca, Chandra, Premala, Coleman, Piers
Other Authors: Massachusetts Institute of Technology. Department of Physics
Format: Article
Language:en_US
Published: American Physical Society 2012
Online Access:http://hdl.handle.net/1721.1/75445
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author Flint, Rebecca
Chandra, Premala
Coleman, Piers
author2 Massachusetts Institute of Technology. Department of Physics
author_facet Massachusetts Institute of Technology. Department of Physics
Flint, Rebecca
Chandra, Premala
Coleman, Piers
author_sort Flint, Rebecca
collection MIT
description he microscopic nature of the hidden order state in URu[subscript 2]Si[subscript 2] is dependent on the low-energy configurations of the uranium ions, and there is currently no consensus on whether it is predominantly 5f[supercript 2] or 5f[supercript 3]. Here we show that measurement of the basal-plane nonlinear susceptibility can resolve this issue; its sign at low temperatures is a distinguishing factor. We calculate the linear and nonlinear susceptibilities for specific 5f[supercript 2] and 5f[supercript 3] crystal-field schemes that are consistent with current experiment. Because of its dual magnetic and orbital character, aΓ[subscript 5] magnetic non-Kramers doublet ground state of the U ion can be identified by χ[subscript 1][superscript c](T)∝χ[subscript 3]⊥(T), where we have determined the constant of proportionality for URu[subscript 2]Si[subscript 2].
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spelling mit-1721.1/754452022-10-02T07:06:11Z Basal-plane nonlinear susceptibility: A direct probe of the single-ion physics in URu2Si2 Flint, Rebecca Chandra, Premala Coleman, Piers Massachusetts Institute of Technology. Department of Physics Flint, Rebecca he microscopic nature of the hidden order state in URu[subscript 2]Si[subscript 2] is dependent on the low-energy configurations of the uranium ions, and there is currently no consensus on whether it is predominantly 5f[supercript 2] or 5f[supercript 3]. Here we show that measurement of the basal-plane nonlinear susceptibility can resolve this issue; its sign at low temperatures is a distinguishing factor. We calculate the linear and nonlinear susceptibilities for specific 5f[supercript 2] and 5f[supercript 3] crystal-field schemes that are consistent with current experiment. Because of its dual magnetic and orbital character, aΓ[subscript 5] magnetic non-Kramers doublet ground state of the U ion can be identified by χ[subscript 1][superscript c](T)∝χ[subscript 3]⊥(T), where we have determined the constant of proportionality for URu[subscript 2]Si[subscript 2]. National Science Foundation (U.S.) (Grant NSF DMR 0907179) National Science Foundation (U.S.) (Grant NSF 1066293) 2012-12-12T21:59:03Z 2012-12-12T21:59:03Z 2012-10 2012-07 Article http://purl.org/eprint/type/JournalArticle 1098-0121 1550-235X http://hdl.handle.net/1721.1/75445 Flint, Rebecca, Premala Chandra, and Piers Coleman. “Basal-plane Nonlinear Susceptibility: A Direct Probe of the Single-ion Physics in URu_{2}Si_{2}.” Physical Review B 86.15 (2012). ©2012 American Physical Society en_US http://dx.doi.org/10.1103/PhysRevB.86.155155 Physical Review B Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. application/pdf American Physical Society APS
spellingShingle Flint, Rebecca
Chandra, Premala
Coleman, Piers
Basal-plane nonlinear susceptibility: A direct probe of the single-ion physics in URu2Si2
title Basal-plane nonlinear susceptibility: A direct probe of the single-ion physics in URu2Si2
title_full Basal-plane nonlinear susceptibility: A direct probe of the single-ion physics in URu2Si2
title_fullStr Basal-plane nonlinear susceptibility: A direct probe of the single-ion physics in URu2Si2
title_full_unstemmed Basal-plane nonlinear susceptibility: A direct probe of the single-ion physics in URu2Si2
title_short Basal-plane nonlinear susceptibility: A direct probe of the single-ion physics in URu2Si2
title_sort basal plane nonlinear susceptibility a direct probe of the single ion physics in uru2si2
url http://hdl.handle.net/1721.1/75445
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AT chandrapremala basalplanenonlinearsusceptibilityadirectprobeofthesingleionphysicsinuru2si2
AT colemanpiers basalplanenonlinearsusceptibilityadirectprobeofthesingleionphysicsinuru2si2