Zone folding effect in Raman G-band intensity of twisted bilayer graphene

The G-band Raman intensity is calculated for twisted bilayer graphene as a function of laser excitation energy based on the extended tight binding method. Here we explicitly consider the electron-photon and electron-phonon matrix elements of twisted bilayer graphene to calculate the resonance Raman...

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Main Authors: Sato, Kentaro, Saito, Riichiro, Cong, Chunxiao, Yu, Ting, Dresselhaus, Mildred
Other Authors: Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science
Format: Article
Language:en_US
Published: American Physical Society 2013
Online Access:http://hdl.handle.net/1721.1/75831
https://orcid.org/0000-0001-8492-2261
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author Sato, Kentaro
Saito, Riichiro
Cong, Chunxiao
Yu, Ting
Dresselhaus, Mildred
author2 Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science
author_facet Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science
Sato, Kentaro
Saito, Riichiro
Cong, Chunxiao
Yu, Ting
Dresselhaus, Mildred
author_sort Sato, Kentaro
collection MIT
description The G-band Raman intensity is calculated for twisted bilayer graphene as a function of laser excitation energy based on the extended tight binding method. Here we explicitly consider the electron-photon and electron-phonon matrix elements of twisted bilayer graphene to calculate the resonance Raman intensity. The G-band Raman intensity is sensitive to the laser excitation energy and the twisting angle between the layers as a result of folding the electronic energy band structure. The Van Hove energy singularity, which is an electron transition energy between the conduction and valence bands, depends on n−m of the twisting vector (n,m). The relative intensity of the G band as a function of twisting vectors is presented, which should be useful for the experimental identification of the twisting angle.
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spelling mit-1721.1/758312022-10-01T15:01:36Z Zone folding effect in Raman G-band intensity of twisted bilayer graphene Sato, Kentaro Saito, Riichiro Cong, Chunxiao Yu, Ting Dresselhaus, Mildred Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science Massachusetts Institute of Technology. Department of Physics Dresselhaus, Mildred The G-band Raman intensity is calculated for twisted bilayer graphene as a function of laser excitation energy based on the extended tight binding method. Here we explicitly consider the electron-photon and electron-phonon matrix elements of twisted bilayer graphene to calculate the resonance Raman intensity. The G-band Raman intensity is sensitive to the laser excitation energy and the twisting angle between the layers as a result of folding the electronic energy band structure. The Van Hove energy singularity, which is an electron transition energy between the conduction and valence bands, depends on n−m of the twisting vector (n,m). The relative intensity of the G band as a function of twisting vectors is presented, which should be useful for the experimental identification of the twisting angle. National Science Foundation (U.S.) (Grant DMR-10- 1004147) 2013-01-07T18:23:29Z 2013-01-07T18:23:29Z 2012-09 2012-07 Article http://purl.org/eprint/type/JournalArticle 1098-0121 1550-235X http://hdl.handle.net/1721.1/75831 Sato, Kentaro et al. “Zone Folding Effect in Raman G-band Intensity of Twisted Bilayer Graphene.” Physical Review B 86.12 (2012). © 2012 American Physical Society https://orcid.org/0000-0001-8492-2261 en_US http://dx.doi.org/10.1103/PhysRevB.86.125414 Physical Review B Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. application/pdf American Physical Society APS
spellingShingle Sato, Kentaro
Saito, Riichiro
Cong, Chunxiao
Yu, Ting
Dresselhaus, Mildred
Zone folding effect in Raman G-band intensity of twisted bilayer graphene
title Zone folding effect in Raman G-band intensity of twisted bilayer graphene
title_full Zone folding effect in Raman G-band intensity of twisted bilayer graphene
title_fullStr Zone folding effect in Raman G-band intensity of twisted bilayer graphene
title_full_unstemmed Zone folding effect in Raman G-band intensity of twisted bilayer graphene
title_short Zone folding effect in Raman G-band intensity of twisted bilayer graphene
title_sort zone folding effect in raman g band intensity of twisted bilayer graphene
url http://hdl.handle.net/1721.1/75831
https://orcid.org/0000-0001-8492-2261
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