Revisiting the “In-clustering” question in InGaN through the use of aberration-corrected electron microscopy below the knock-on threshold

The high intensity of light emitted in In[subscript x]Ga[subscript 1−x]N/GaN heterostructures has been generally attributed to the formation of indium-rich clusters in In[subscript x]Ga[subscript 1−x]N quantum wells (QWs). However, there is significant disagreement about the existence of such cluste...

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Main Authors: Baloch, Kamal H., Johnston-Peck, Aaron C., Kisslinger, Kim, Stach, Eric A., Gradecak, Silvija
Other Authors: Massachusetts Institute of Technology. Department of Materials Science and Engineering
Format: Article
Language:en_US
Published: American Institute of Physics (AIP) 2013
Online Access:http://hdl.handle.net/1721.1/79641
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author Baloch, Kamal H.
Johnston-Peck, Aaron C.
Kisslinger, Kim
Stach, Eric A.
Gradecak, Silvija
author2 Massachusetts Institute of Technology. Department of Materials Science and Engineering
author_facet Massachusetts Institute of Technology. Department of Materials Science and Engineering
Baloch, Kamal H.
Johnston-Peck, Aaron C.
Kisslinger, Kim
Stach, Eric A.
Gradecak, Silvija
author_sort Baloch, Kamal H.
collection MIT
description The high intensity of light emitted in In[subscript x]Ga[subscript 1−x]N/GaN heterostructures has been generally attributed to the formation of indium-rich clusters in In[subscript x]Ga[subscript 1−x]N quantum wells (QWs). However, there is significant disagreement about the existence of such clusters in as-grown In[subscript x]Ga[subscript 1−x]N QWs. We employ atomically resolved CS-corrected scanning transmission electron microscopy and electron energy loss spectroscopy at 120 kV—which we demonstrate to be below the knock-on displacement threshold—and show that indium clustering is not present in as-grown In[subscript 0.22]Ga[subscript 0.78]N QWs. This artifact-free, atomically resolved method can be employed for investigating compositional variations in other In[subscript x]Ga[subscript 1−x]N/GaN heterostructures.
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spelling mit-1721.1/796412022-09-29T12:32:35Z Revisiting the “In-clustering” question in InGaN through the use of aberration-corrected electron microscopy below the knock-on threshold Baloch, Kamal H. Johnston-Peck, Aaron C. Kisslinger, Kim Stach, Eric A. Gradecak, Silvija Massachusetts Institute of Technology. Department of Materials Science and Engineering Massachusetts Institute of Technology. Research Laboratory of Electronics Baloch, Kamal H. Gradecak, Silvija The high intensity of light emitted in In[subscript x]Ga[subscript 1−x]N/GaN heterostructures has been generally attributed to the formation of indium-rich clusters in In[subscript x]Ga[subscript 1−x]N quantum wells (QWs). However, there is significant disagreement about the existence of such clusters in as-grown In[subscript x]Ga[subscript 1−x]N QWs. We employ atomically resolved CS-corrected scanning transmission electron microscopy and electron energy loss spectroscopy at 120 kV—which we demonstrate to be below the knock-on displacement threshold—and show that indium clustering is not present in as-grown In[subscript 0.22]Ga[subscript 0.78]N QWs. This artifact-free, atomically resolved method can be employed for investigating compositional variations in other In[subscript x]Ga[subscript 1−x]N/GaN heterostructures. United States. Dept. of Energy. Office of Basic Energy Sciences (Contract DE-AC02- 98CH10886) United States. Dept. of Energy. Office of Basic Energy Sciences (United States. Dept. of Energy. Center for Excitonics Award DE-SC0001088) 2013-07-22T15:18:45Z 2013-07-22T15:18:45Z 2013-05 2013-04 Article http://purl.org/eprint/type/JournalArticle 00036951 1077-3118 http://hdl.handle.net/1721.1/79641 Baloch, Kamal H., Aaron C. Johnston-Peck, Kim Kisslinger, Eric A. Stach, and Silvija Gradečak. “Revisiting the ‘In-clustering’ question in InGaN through the use of aberration-corrected electron microscopy below the knock-on threshold.” Applied Physics Letters 102, no. 19 (2013): 191910. © 2013 AIP Publishing LLC en_US http://dx.doi.org/10.1063/1.4807122 Applied Physics Letters Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. application/pdf American Institute of Physics (AIP) MIT web domain
spellingShingle Baloch, Kamal H.
Johnston-Peck, Aaron C.
Kisslinger, Kim
Stach, Eric A.
Gradecak, Silvija
Revisiting the “In-clustering” question in InGaN through the use of aberration-corrected electron microscopy below the knock-on threshold
title Revisiting the “In-clustering” question in InGaN through the use of aberration-corrected electron microscopy below the knock-on threshold
title_full Revisiting the “In-clustering” question in InGaN through the use of aberration-corrected electron microscopy below the knock-on threshold
title_fullStr Revisiting the “In-clustering” question in InGaN through the use of aberration-corrected electron microscopy below the knock-on threshold
title_full_unstemmed Revisiting the “In-clustering” question in InGaN through the use of aberration-corrected electron microscopy below the knock-on threshold
title_short Revisiting the “In-clustering” question in InGaN through the use of aberration-corrected electron microscopy below the knock-on threshold
title_sort revisiting the in clustering question in ingan through the use of aberration corrected electron microscopy below the knock on threshold
url http://hdl.handle.net/1721.1/79641
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