A nanoscale probe of the quasiparticle band structure for two dimensional electron systems

Thesis (Ph. D.)--Massachusetts Institute of Technology, Dept. of Physics, 2013.

Bibliographic Details
Main Author: Soumyanarayanan, Anjan
Other Authors: Young S. Lee.
Format: Thesis
Language:eng
Published: Massachusetts Institute of Technology 2014
Subjects:
Online Access:http://hdl.handle.net/1721.1/83821
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author Soumyanarayanan, Anjan
author2 Young S. Lee.
author_facet Young S. Lee.
Soumyanarayanan, Anjan
author_sort Soumyanarayanan, Anjan
collection MIT
description Thesis (Ph. D.)--Massachusetts Institute of Technology, Dept. of Physics, 2013.
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spelling mit-1721.1/838212019-04-10T07:13:15Z A nanoscale probe of the quasiparticle band structure for two dimensional electron systems Soumyanarayanan, Anjan Young S. Lee. Massachusetts Institute of Technology. Department of Physics. Massachusetts Institute of Technology. Department of Physics. Physics. Thesis (Ph. D.)--Massachusetts Institute of Technology, Dept. of Physics, 2013. Page 138 blank. Cataloged from PDF version of thesis. Includes bibliographical references (pages 121-137). The advent of a broad class of two-dimensional (2D) electronic materials has provided avenues to create and study designer electronic quantum phases. The coexistence of superconductivity, magnetism, density waves, and other ordered phases on the surfaces and interfaces of these 2D materials are governed by interactions which can be experimentally tuned with increasing precision. This motivates the need to develop spectroscopic probes that are sensitive to these tuning parameters, with the objective of studying the electronic properties and emergence of order in these materials. In the first part of this thesis, we report on spectroscopic studies of the topological semimetal antimony (Sb). Our simultaneous observation of Landau quantization and quasiparticle interference phenomena on this material enables their quantitative reconciliation - after two decades of their study on various materials. We use these observations to establish momentum-resolved scanning tunneling microscopy (MR-STM) as a robust nanoscale band structure probe, and reconstruct the multi-component dispersion of Sb(111) surface states. We quantify surface state parameters relevant to spintronics applications, and clarify the relationship between bulk conductivity and surface state robustness. At low momentum, we find a crossover in the single particle behavior from massless Dirac to massive Rashba character - a unique signature of topological surface states. In the second part of this thesis, we report on the spectroscopic study of charge density wave (CDW) order in the dichalcogenide 2H-NbSe2 - a model system for understanding the interplay of coexisting CDW and superconducting phases. We detail the observation of a previously unknown unidirectional (stripe) CDW smoothly interfacing with the familiar triangular CDW on this material. Our low temperature measurements rule out thermal fluctuations and point to local strain as the tuning parameter for this quantum phase transition. The distinct wavelengths and tunneling spectra of the two CDWs, in conjunction with band structure calculations, enable us to resolve two longstanding debates about the anomalous spectroscopic gap and the role of Fermi surface nesting in the CDW phase of NbSe2. Our observations motivate further spectroscopic studies of the phase evolution of the CDW, and of NbSe 2 as a prototypical strong coupling density wave system in the vicinity of a quantum critical point. by Anjan Soumyanarayanan. Ph.D. 2014-01-09T19:58:45Z 2014-01-09T19:58:45Z 2013 Thesis http://hdl.handle.net/1721.1/83821 865574606 eng M.I.T. theses are protected by copyright. They may be viewed from this source for any purpose, but reproduction or distribution in any format is prohibited without written permission. See provided URL for inquiries about permission. http://dspace.mit.edu/handle/1721.1/7582 138 pages application/pdf Massachusetts Institute of Technology
spellingShingle Physics.
Soumyanarayanan, Anjan
A nanoscale probe of the quasiparticle band structure for two dimensional electron systems
title A nanoscale probe of the quasiparticle band structure for two dimensional electron systems
title_full A nanoscale probe of the quasiparticle band structure for two dimensional electron systems
title_fullStr A nanoscale probe of the quasiparticle band structure for two dimensional electron systems
title_full_unstemmed A nanoscale probe of the quasiparticle band structure for two dimensional electron systems
title_short A nanoscale probe of the quasiparticle band structure for two dimensional electron systems
title_sort nanoscale probe of the quasiparticle band structure for two dimensional electron systems
topic Physics.
url http://hdl.handle.net/1721.1/83821
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