Particle laden flows through an inverted chimney with applications to ocean carbon sequestration

Plumes of negatively buoyant hydrate particles, formed by reacting liquid CO[subscript 2] with seawater at ocean depths of 1000–1500 m, have been suggested as a way to help sequester CO[subscript 2]. The vertical flux of CO[subscript 2] can be increased by constructing a shroud around the hydrate pa...

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Main Authors: Chow, Aaron C., Adams, E. Eric
Other Authors: Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
Format: Article
Language:en_US
Published: Springer-Verlag 2014
Online Access:http://hdl.handle.net/1721.1/85662
https://orcid.org/0000-0002-5577-683X
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author Chow, Aaron C.
Adams, E. Eric
author2 Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
author_facet Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
Chow, Aaron C.
Adams, E. Eric
author_sort Chow, Aaron C.
collection MIT
description Plumes of negatively buoyant hydrate particles, formed by reacting liquid CO[subscript 2] with seawater at ocean depths of 1000–1500 m, have been suggested as a way to help sequester CO[subscript 2]. The vertical flux of CO[subscript 2] can be increased by constructing a shroud around the hydrate particle source to shelter the plume from effects of ambient stratification and current. The shroud also serves as an inverted chimney, inducing a down draft that will transport the dissolving particles to a depth of lower ambient disturbance. Laboratory PIV measurements are compared to an analysis of an idealized shroud that is long, frictionless and driven by a single phase source of buoyancy distributed uniformly over the shroud base. Results indicate that induced draft, and hence dilution of dissolved CO[subscript 2], increases with plume buoyancy, and shroud length and diameter, but efficiency decreases with increasing ratio of particle slip velocity divided by the characteristic induced draft velocity. While larger particles show reduced plume-like behavior and hence are less efficient in inducing draft, they still generated about half of the theoretically predicted flow.
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spelling mit-1721.1/856622022-09-23T13:12:30Z Particle laden flows through an inverted chimney with applications to ocean carbon sequestration Chow, Aaron C. Adams, E. Eric Massachusetts Institute of Technology. Department of Civil and Environmental Engineering Adams, Eric E. Adams, E. Eric Plumes of negatively buoyant hydrate particles, formed by reacting liquid CO[subscript 2] with seawater at ocean depths of 1000–1500 m, have been suggested as a way to help sequester CO[subscript 2]. The vertical flux of CO[subscript 2] can be increased by constructing a shroud around the hydrate particle source to shelter the plume from effects of ambient stratification and current. The shroud also serves as an inverted chimney, inducing a down draft that will transport the dissolving particles to a depth of lower ambient disturbance. Laboratory PIV measurements are compared to an analysis of an idealized shroud that is long, frictionless and driven by a single phase source of buoyancy distributed uniformly over the shroud base. Results indicate that induced draft, and hence dilution of dissolved CO[subscript 2], increases with plume buoyancy, and shroud length and diameter, but efficiency decreases with increasing ratio of particle slip velocity divided by the characteristic induced draft velocity. While larger particles show reduced plume-like behavior and hence are less efficient in inducing draft, they still generated about half of the theoretically predicted flow. United States. Dept. of Energy (Ocean Carbon Sequestration Program, Biological and Environmental Research Grant DE-FG02-01ER63078) United States. Dept. of Energy (National Energy Technology Laboratory Grant DE-FG26-98FT40334) Martin Family Society of Fellows for Sustainability 2014-03-14T20:24:45Z 2014-03-14T20:24:45Z 2010-12 2010-08 Article http://purl.org/eprint/type/JournalArticle 1567-7419 1573-1510 http://hdl.handle.net/1721.1/85662 Chow, Aaron C., and E. Eric Adams. “Particle Laden Flows through an Inverted Chimney with Applications to Ocean Carbon Sequestration.” Environ Fluid Mech 12, no. 1 (February 2012): 3–21. https://orcid.org/0000-0002-5577-683X en_US http://dx.doi.org/10.1007/s10652-010-9200-1 Environmental Fluid Mechanics Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. application/pdf Springer-Verlag Adams
spellingShingle Chow, Aaron C.
Adams, E. Eric
Particle laden flows through an inverted chimney with applications to ocean carbon sequestration
title Particle laden flows through an inverted chimney with applications to ocean carbon sequestration
title_full Particle laden flows through an inverted chimney with applications to ocean carbon sequestration
title_fullStr Particle laden flows through an inverted chimney with applications to ocean carbon sequestration
title_full_unstemmed Particle laden flows through an inverted chimney with applications to ocean carbon sequestration
title_short Particle laden flows through an inverted chimney with applications to ocean carbon sequestration
title_sort particle laden flows through an inverted chimney with applications to ocean carbon sequestration
url http://hdl.handle.net/1721.1/85662
https://orcid.org/0000-0002-5577-683X
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