Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media
Geological carbon dioxide (CO[subscript 2]) sequestration entails capturing and injecting CO[subscript 2][subscript 2]into deep saline aquifers for long-term storage. The injected CO[subscript 2] partially dissolves in groundwater to form a mixture that is denser than the initial groundwater. The lo...
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Royal Society, The
2015
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Online Access: | http://hdl.handle.net/1721.1/92724 https://orcid.org/0000-0001-7120-704X https://orcid.org/0000-0002-7370-2332 https://orcid.org/0000-0003-3958-7382 |
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author | Fu, Xiaojing Cueto-Felgueroso, Luis Juanes, Ruben |
author2 | Massachusetts Institute of Technology. Department of Civil and Environmental Engineering |
author_facet | Massachusetts Institute of Technology. Department of Civil and Environmental Engineering Fu, Xiaojing Cueto-Felgueroso, Luis Juanes, Ruben |
author_sort | Fu, Xiaojing |
collection | MIT |
description | Geological carbon dioxide (CO[subscript 2]) sequestration entails capturing and injecting CO[subscript 2][subscript 2]into deep saline aquifers for long-term storage. The injected CO[subscript 2] partially dissolves in groundwater to form a mixture that is denser than the initial groundwater. The local increase in density triggers a gravitational instability at the boundary layer that further develops into columnar plumes of CO[subscript 2]-rich brine, a process that greatly accelerates solubility trapping of the CO[subscript 2]. Here, we investigate the pattern-formation aspects of convective mixing during geological CO[subscript 2] sequestration by means of high-resolution three-dimensional simulation. We find that the CO[subscript 2] concentration field self-organizes as a cellular network structure in the diffusive boundary layer at the top boundary. By studying the statistics of the cellular network, we identify various regimes of finger coarsening over time, the existence of a non-equilibrium stationary state, and a universal scaling of three-dimensional convective mixing. |
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format | Article |
id | mit-1721.1/92724 |
institution | Massachusetts Institute of Technology |
language | en_US |
last_indexed | 2024-09-23T12:43:06Z |
publishDate | 2015 |
publisher | Royal Society, The |
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spelling | mit-1721.1/927242022-10-01T10:40:51Z Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media Fu, Xiaojing Cueto-Felgueroso, Luis Juanes, Ruben Massachusetts Institute of Technology. Department of Civil and Environmental Engineering Juanes, Ruben Fu, Xiaojing Cueto-Felgueroso, Luis Juanes, Ruben Geological carbon dioxide (CO[subscript 2]) sequestration entails capturing and injecting CO[subscript 2][subscript 2]into deep saline aquifers for long-term storage. The injected CO[subscript 2] partially dissolves in groundwater to form a mixture that is denser than the initial groundwater. The local increase in density triggers a gravitational instability at the boundary layer that further develops into columnar plumes of CO[subscript 2]-rich brine, a process that greatly accelerates solubility trapping of the CO[subscript 2]. Here, we investigate the pattern-formation aspects of convective mixing during geological CO[subscript 2] sequestration by means of high-resolution three-dimensional simulation. We find that the CO[subscript 2] concentration field self-organizes as a cellular network structure in the diffusive boundary layer at the top boundary. By studying the statistics of the cellular network, we identify various regimes of finger coarsening over time, the existence of a non-equilibrium stationary state, and a universal scaling of three-dimensional convective mixing. 2015-01-07T16:00:51Z 2015-01-07T16:00:51Z 2013-11 Article http://purl.org/eprint/type/JournalArticle 1364-503X 1471-2962 http://hdl.handle.net/1721.1/92724 Fu, X., L. Cueto-Felgueroso, and R. Juanes. “Pattern Formation and Coarsening Dynamics in Three-Dimensional Convective Mixing in Porous Media.” Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences 371, no. 2004 (November 4, 2013): 20120355–20120355. https://orcid.org/0000-0001-7120-704X https://orcid.org/0000-0002-7370-2332 https://orcid.org/0000-0003-3958-7382 en_US http://dx.doi.org/10.1098/rsta.2012.0355 Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences Creative Commons Attribution-Noncommercial-Share Alike http://creativecommons.org/licenses/by-nc-sa/4.0/ application/pdf Royal Society, The Anne Graham |
spellingShingle | Fu, Xiaojing Cueto-Felgueroso, Luis Juanes, Ruben Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media |
title | Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media |
title_full | Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media |
title_fullStr | Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media |
title_full_unstemmed | Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media |
title_short | Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media |
title_sort | pattern formation and coarsening dynamics in three dimensional convective mixing in porous media |
url | http://hdl.handle.net/1721.1/92724 https://orcid.org/0000-0001-7120-704X https://orcid.org/0000-0002-7370-2332 https://orcid.org/0000-0003-3958-7382 |
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