Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media

Geological carbon dioxide (CO[subscript 2]) sequestration entails capturing and injecting CO[subscript 2][subscript 2]into deep saline aquifers for long-term storage. The injected CO[subscript 2] partially dissolves in groundwater to form a mixture that is denser than the initial groundwater. The lo...

Full description

Bibliographic Details
Main Authors: Fu, Xiaojing, Cueto-Felgueroso, Luis, Juanes, Ruben
Other Authors: Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
Format: Article
Language:en_US
Published: Royal Society, The 2015
Online Access:http://hdl.handle.net/1721.1/92724
https://orcid.org/0000-0001-7120-704X
https://orcid.org/0000-0002-7370-2332
https://orcid.org/0000-0003-3958-7382
_version_ 1826203791686369280
author Fu, Xiaojing
Cueto-Felgueroso, Luis
Juanes, Ruben
author2 Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
author_facet Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
Fu, Xiaojing
Cueto-Felgueroso, Luis
Juanes, Ruben
author_sort Fu, Xiaojing
collection MIT
description Geological carbon dioxide (CO[subscript 2]) sequestration entails capturing and injecting CO[subscript 2][subscript 2]into deep saline aquifers for long-term storage. The injected CO[subscript 2] partially dissolves in groundwater to form a mixture that is denser than the initial groundwater. The local increase in density triggers a gravitational instability at the boundary layer that further develops into columnar plumes of CO[subscript 2]-rich brine, a process that greatly accelerates solubility trapping of the CO[subscript 2]. Here, we investigate the pattern-formation aspects of convective mixing during geological CO[subscript 2] sequestration by means of high-resolution three-dimensional simulation. We find that the CO[subscript 2] concentration field self-organizes as a cellular network structure in the diffusive boundary layer at the top boundary. By studying the statistics of the cellular network, we identify various regimes of finger coarsening over time, the existence of a non-equilibrium stationary state, and a universal scaling of three-dimensional convective mixing.
first_indexed 2024-09-23T12:43:06Z
format Article
id mit-1721.1/92724
institution Massachusetts Institute of Technology
language en_US
last_indexed 2024-09-23T12:43:06Z
publishDate 2015
publisher Royal Society, The
record_format dspace
spelling mit-1721.1/927242022-10-01T10:40:51Z Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media Fu, Xiaojing Cueto-Felgueroso, Luis Juanes, Ruben Massachusetts Institute of Technology. Department of Civil and Environmental Engineering Juanes, Ruben Fu, Xiaojing Cueto-Felgueroso, Luis Juanes, Ruben Geological carbon dioxide (CO[subscript 2]) sequestration entails capturing and injecting CO[subscript 2][subscript 2]into deep saline aquifers for long-term storage. The injected CO[subscript 2] partially dissolves in groundwater to form a mixture that is denser than the initial groundwater. The local increase in density triggers a gravitational instability at the boundary layer that further develops into columnar plumes of CO[subscript 2]-rich brine, a process that greatly accelerates solubility trapping of the CO[subscript 2]. Here, we investigate the pattern-formation aspects of convective mixing during geological CO[subscript 2] sequestration by means of high-resolution three-dimensional simulation. We find that the CO[subscript 2] concentration field self-organizes as a cellular network structure in the diffusive boundary layer at the top boundary. By studying the statistics of the cellular network, we identify various regimes of finger coarsening over time, the existence of a non-equilibrium stationary state, and a universal scaling of three-dimensional convective mixing. 2015-01-07T16:00:51Z 2015-01-07T16:00:51Z 2013-11 Article http://purl.org/eprint/type/JournalArticle 1364-503X 1471-2962 http://hdl.handle.net/1721.1/92724 Fu, X., L. Cueto-Felgueroso, and R. Juanes. “Pattern Formation and Coarsening Dynamics in Three-Dimensional Convective Mixing in Porous Media.” Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences 371, no. 2004 (November 4, 2013): 20120355–20120355. https://orcid.org/0000-0001-7120-704X https://orcid.org/0000-0002-7370-2332 https://orcid.org/0000-0003-3958-7382 en_US http://dx.doi.org/10.1098/rsta.2012.0355 Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences Creative Commons Attribution-Noncommercial-Share Alike http://creativecommons.org/licenses/by-nc-sa/4.0/ application/pdf Royal Society, The Anne Graham
spellingShingle Fu, Xiaojing
Cueto-Felgueroso, Luis
Juanes, Ruben
Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media
title Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media
title_full Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media
title_fullStr Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media
title_full_unstemmed Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media
title_short Pattern formation and coarsening dynamics in three-dimensional convective mixing in porous media
title_sort pattern formation and coarsening dynamics in three dimensional convective mixing in porous media
url http://hdl.handle.net/1721.1/92724
https://orcid.org/0000-0001-7120-704X
https://orcid.org/0000-0002-7370-2332
https://orcid.org/0000-0003-3958-7382
work_keys_str_mv AT fuxiaojing patternformationandcoarseningdynamicsinthreedimensionalconvectivemixinginporousmedia
AT cuetofelguerosoluis patternformationandcoarseningdynamicsinthreedimensionalconvectivemixinginporousmedia
AT juanesruben patternformationandcoarseningdynamicsinthreedimensionalconvectivemixinginporousmedia