Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals
Height time hyperspectral near IR probing providing broad-band coverage is employed on PbSe nanocrystals, uncovering spectral evolution following high energy photo-excitation due to hot exciton relaxation and recombination. Separation of single, double and triple exciton state contributions to these...
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EDP Sciences
2015
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Online Access: | http://hdl.handle.net/1721.1/93243 https://orcid.org/0000-0003-2220-4365 |
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author | Gdor, I. Sachs, H. Roitblat, A. Ruhman, S. Strasfeld, David Bawendi, Moungi G. |
author2 | Massachusetts Institute of Technology. Department of Chemistry |
author_facet | Massachusetts Institute of Technology. Department of Chemistry Gdor, I. Sachs, H. Roitblat, A. Ruhman, S. Strasfeld, David Bawendi, Moungi G. |
author_sort | Gdor, I. |
collection | MIT |
description | Height time hyperspectral near IR probing providing broad-band coverage is employed on PbSe nanocrystals, uncovering spectral evolution following high energy photo-excitation due to hot exciton relaxation and recombination. Separation of single, double and triple exciton state contributions to these spectra is demonstrated, and the mechanisms underlying the course of spectral evolution are investigated. In addition no sign of MEG was detected in this sample up to a photon energy 3.7 times that of the band gap. |
first_indexed | 2024-09-23T11:12:09Z |
format | Article |
id | mit-1721.1/93243 |
institution | Massachusetts Institute of Technology |
language | en_US |
last_indexed | 2024-09-23T11:12:09Z |
publishDate | 2015 |
publisher | EDP Sciences |
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spelling | mit-1721.1/932432022-10-01T01:59:55Z Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals Gdor, I. Sachs, H. Roitblat, A. Ruhman, S. Strasfeld, David Bawendi, Moungi G. Massachusetts Institute of Technology. Department of Chemistry Strasfeld, David Bawendi, Moungi G. Height time hyperspectral near IR probing providing broad-band coverage is employed on PbSe nanocrystals, uncovering spectral evolution following high energy photo-excitation due to hot exciton relaxation and recombination. Separation of single, double and triple exciton state contributions to these spectra is demonstrated, and the mechanisms underlying the course of spectral evolution are investigated. In addition no sign of MEG was detected in this sample up to a photon energy 3.7 times that of the band gap. 2015-01-30T19:50:33Z 2015-01-30T19:50:33Z 2013-03 Article http://purl.org/eprint/type/ConferencePaper 2100-014X http://hdl.handle.net/1721.1/93243 Gdor, I., H. Sachs, A. Roitblat, D. Strasfeld, M.G. Bawendi, and S. Ruhman. “Hyperspectral Probing of Exciton Dynamics and Multiplication in PbSe Nanocrystals.” Edited by M. Chergui, A. Taylor, S. Cundiff, R. de Vivie-Riedle, and K. Yamagouchi. EPJ Web of Conferences 41 (2013): 04037. https://orcid.org/0000-0003-2220-4365 en_US http://dx.doi.org/10.1051/epjconf/20134104037 EPJ Web of Conferences Creative Commons Attribution http://creativecommons.org/licenses/by/2.0 application/pdf EDP Sciences EPJ Web of Conferences |
spellingShingle | Gdor, I. Sachs, H. Roitblat, A. Ruhman, S. Strasfeld, David Bawendi, Moungi G. Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals |
title | Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals |
title_full | Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals |
title_fullStr | Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals |
title_full_unstemmed | Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals |
title_short | Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals |
title_sort | hyperspectral probing of exciton dynamics and multiplication in pbse nanocrystals |
url | http://hdl.handle.net/1721.1/93243 https://orcid.org/0000-0003-2220-4365 |
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