Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals

Height time hyperspectral near IR probing providing broad-band coverage is employed on PbSe nanocrystals, uncovering spectral evolution following high energy photo-excitation due to hot exciton relaxation and recombination. Separation of single, double and triple exciton state contributions to these...

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Main Authors: Gdor, I., Sachs, H., Roitblat, A., Ruhman, S., Strasfeld, David, Bawendi, Moungi G.
Other Authors: Massachusetts Institute of Technology. Department of Chemistry
Format: Article
Language:en_US
Published: EDP Sciences 2015
Online Access:http://hdl.handle.net/1721.1/93243
https://orcid.org/0000-0003-2220-4365
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author Gdor, I.
Sachs, H.
Roitblat, A.
Ruhman, S.
Strasfeld, David
Bawendi, Moungi G.
author2 Massachusetts Institute of Technology. Department of Chemistry
author_facet Massachusetts Institute of Technology. Department of Chemistry
Gdor, I.
Sachs, H.
Roitblat, A.
Ruhman, S.
Strasfeld, David
Bawendi, Moungi G.
author_sort Gdor, I.
collection MIT
description Height time hyperspectral near IR probing providing broad-band coverage is employed on PbSe nanocrystals, uncovering spectral evolution following high energy photo-excitation due to hot exciton relaxation and recombination. Separation of single, double and triple exciton state contributions to these spectra is demonstrated, and the mechanisms underlying the course of spectral evolution are investigated. In addition no sign of MEG was detected in this sample up to a photon energy 3.7 times that of the band gap.
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spelling mit-1721.1/932432022-10-01T01:59:55Z Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals Gdor, I. Sachs, H. Roitblat, A. Ruhman, S. Strasfeld, David Bawendi, Moungi G. Massachusetts Institute of Technology. Department of Chemistry Strasfeld, David Bawendi, Moungi G. Height time hyperspectral near IR probing providing broad-band coverage is employed on PbSe nanocrystals, uncovering spectral evolution following high energy photo-excitation due to hot exciton relaxation and recombination. Separation of single, double and triple exciton state contributions to these spectra is demonstrated, and the mechanisms underlying the course of spectral evolution are investigated. In addition no sign of MEG was detected in this sample up to a photon energy 3.7 times that of the band gap. 2015-01-30T19:50:33Z 2015-01-30T19:50:33Z 2013-03 Article http://purl.org/eprint/type/ConferencePaper 2100-014X http://hdl.handle.net/1721.1/93243 Gdor, I., H. Sachs, A. Roitblat, D. Strasfeld, M.G. Bawendi, and S. Ruhman. “Hyperspectral Probing of Exciton Dynamics and Multiplication in PbSe Nanocrystals.” Edited by M. Chergui, A. Taylor, S. Cundiff, R. de Vivie-Riedle, and K. Yamagouchi. EPJ Web of Conferences 41 (2013): 04037. https://orcid.org/0000-0003-2220-4365 en_US http://dx.doi.org/10.1051/epjconf/20134104037 EPJ Web of Conferences Creative Commons Attribution http://creativecommons.org/licenses/by/2.0 application/pdf EDP Sciences EPJ Web of Conferences
spellingShingle Gdor, I.
Sachs, H.
Roitblat, A.
Ruhman, S.
Strasfeld, David
Bawendi, Moungi G.
Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals
title Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals
title_full Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals
title_fullStr Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals
title_full_unstemmed Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals
title_short Hyperspectral Probing of Exciton dynamics and Multiplication in PbSe Nanocrystals
title_sort hyperspectral probing of exciton dynamics and multiplication in pbse nanocrystals
url http://hdl.handle.net/1721.1/93243
https://orcid.org/0000-0003-2220-4365
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