Theory of terahertz generation by optical rectification

Thesis: S.M., Massachusetts Institute of Technology, Department of Electrical Engineering and Computer Science, 2014.

Bibliographic Details
Main Author: Ravi, Koustuban
Other Authors: Franz X. Kärtner and Erich P. lppen.
Format: Thesis
Language:eng
Published: Massachusetts Institute of Technology 2015
Subjects:
Online Access:http://hdl.handle.net/1721.1/93837
_version_ 1811094459269513216
author Ravi, Koustuban
author2 Franz X. Kärtner and Erich P. lppen.
author_facet Franz X. Kärtner and Erich P. lppen.
Ravi, Koustuban
author_sort Ravi, Koustuban
collection MIT
description Thesis: S.M., Massachusetts Institute of Technology, Department of Electrical Engineering and Computer Science, 2014.
first_indexed 2024-09-23T16:00:24Z
format Thesis
id mit-1721.1/93837
institution Massachusetts Institute of Technology
language eng
last_indexed 2024-09-23T16:00:24Z
publishDate 2015
publisher Massachusetts Institute of Technology
record_format dspace
spelling mit-1721.1/938372019-04-12T21:49:58Z Theory of terahertz generation by optical rectification Ravi, Koustuban Franz X. Kärtner and Erich P. lppen. Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science. Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science. Electrical Engineering and Computer Science. Thesis: S.M., Massachusetts Institute of Technology, Department of Electrical Engineering and Computer Science, 2014. Cataloged from PDF version of thesis. Includes bibliographical references (pages 61-63). Intense pulses of light with wavelengths approximately ten times smaller than microwave sources and a hundred times larger than optical/near infra-red sources may be categorized as high-field Terahertz (THz) sources. By virtue of their large electromagnetic field amplitudes and relatively long wavelengths, they are uniquely amenable for electron acceleration, coherent X-ray generation and non-linear spectroscopy. Intra-pulse difference frequency generation or optical rectification of ultrafast optical pump pulses in nonlinear crystals has emerged as the most efficient approach for high-field THz generation. Earlier theoretical treatment of these systems had predicted conversion efficiencies as high as 10%, which opened up the possibility of generating THz pulses with energies on the order of 10 milli joules on a table-top. However, experimental demonstrations have achieved conversion efficiencies of only a few percent which motivates a re-examination of the existing theory. In this thesis, we re-formulate the problem by accounting for effects, previously not considered. These include: (i) the spatio-temporal distortions of ultrafast pulses, (ii) the nonlinear coupled interaction of optical and THz radiation in two spatial dimensions (2-D), (iii) self-phase modulation, (iv) stimulated Raman scattering and (v) crystal geometry. The key finding is that THz generation necessarily leads to broadening of the optical pump spectrum, resulting in a rapid spatio-temporal break-up of the pulse which limits further generation of THz radiation. Due to this self-limiting mechanism, the predicted conversion efficiencies reduce significantly in relation to earlier predictions, which is in line with experimental trends. Guidelines to optimize conversion efficiency and their ramifications on spatial and spectral properties of THz radiation are discussed. The predictions and analyses are supported by experiments. These findings direct future work towards careful engineering of such systems to achieve optimal THz pulse properties and the conception of approaches to circumvent the aforementioned self-limiting effects. by Koustuban Ravi. S.M. 2015-02-05T18:27:28Z 2015-02-05T18:27:28Z 2014 2014 Thesis http://hdl.handle.net/1721.1/93837 900736523 eng M.I.T. theses are protected by copyright. They may be viewed from this source for any purpose, but reproduction or distribution in any format is prohibited without written permission. See provided URL for inquiries about permission. http://dspace.mit.edu/handle/1721.1/7582 63 pages application/pdf Massachusetts Institute of Technology
spellingShingle Electrical Engineering and Computer Science.
Ravi, Koustuban
Theory of terahertz generation by optical rectification
title Theory of terahertz generation by optical rectification
title_full Theory of terahertz generation by optical rectification
title_fullStr Theory of terahertz generation by optical rectification
title_full_unstemmed Theory of terahertz generation by optical rectification
title_short Theory of terahertz generation by optical rectification
title_sort theory of terahertz generation by optical rectification
topic Electrical Engineering and Computer Science.
url http://hdl.handle.net/1721.1/93837
work_keys_str_mv AT ravikoustuban theoryofterahertzgenerationbyopticalrectification