How emissions, climate, and land use change will impact mid-century air quality over the United States: a focus on effects at national parks

We use a global coupled chemistry–climate–land model (CESM) to assess the integrated effect of climate, emissions and land use changes on annual surface O[subscript 3] and PM[subscript 2.5] in the United States with a focus on national parks (NPs) and wilderness areas, using the RCP4.5 and RCP8.5 pr...

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Main Authors: Val Martin, M., Lamarque, Jean-Francois, Tilmes, S., Emmons, L. K., Schichtel, B. A., Heald, Colette L.
Other Authors: Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
Format: Article
Language:en_US
Published: Copernicus GmbH 2015
Online Access:http://hdl.handle.net/1721.1/96343
https://orcid.org/0000-0003-2894-5738
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author Val Martin, M.
Lamarque, Jean-Francois
Tilmes, S.
Emmons, L. K.
Schichtel, B. A.
Heald, Colette L.
author2 Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
author_facet Massachusetts Institute of Technology. Department of Civil and Environmental Engineering
Val Martin, M.
Lamarque, Jean-Francois
Tilmes, S.
Emmons, L. K.
Schichtel, B. A.
Heald, Colette L.
author_sort Val Martin, M.
collection MIT
description We use a global coupled chemistry–climate–land model (CESM) to assess the integrated effect of climate, emissions and land use changes on annual surface O[subscript 3] and PM[subscript 2.5] in the United States with a focus on national parks (NPs) and wilderness areas, using the RCP4.5 and RCP8.5 projections. We show that, when stringent domestic emission controls are applied, air quality is predicted to improve across the US, except surface O[subscript 3] over the western and central US under RCP8.5 conditions, where rising background ozone counteracts domestic emission reductions. Under the RCP4.5 scenario, surface O[subscript 3] is substantially reduced (about 5 ppb), with daily maximum 8 h averages below the primary US Environmental Protection Agency (EPA) National Ambient Air Quality Standards (NAAQS) of 75 ppb (and even 65 ppb) in all the NPs. PM[subscript 2.5] is significantly reduced in both scenarios (4 μg m[superscript −3]; ~50%), with levels below the annual US EPA NAAQS of 12 μg m[superscript −3] across all the NPs; visibility is also improved (10–15 dv; >75 km in visibility range), although some western US parks with Class I status (40–74 % of total sites in the US) are still above the 2050 planned target level to reach the goal of natural visibility conditions by 2064. We estimate that climate-driven increases in fire activity may dominate summertime PM2.5 over the western US, potentially offsetting the large PM2.5 reductions from domestic emission controls, and keeping visibility at present-day levels in many parks. Our study indicates that anthropogenic emission patterns will be important for air quality in 2050. However, climate and land use changes alone may lead to a substantial increase in surface O[subscript 3] (2–3 ppb) with important consequences for O[subscript 3] air quality and ecosystem degradation at the US NPs. Our study illustrates the need to consider the effects of changes in climate, vegetation, and fires in future air quality management and planning and emission policy making.
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spelling mit-1721.1/963432022-10-01T10:40:43Z How emissions, climate, and land use change will impact mid-century air quality over the United States: a focus on effects at national parks Val Martin, M. Lamarque, Jean-Francois Tilmes, S. Emmons, L. K. Schichtel, B. A. Heald, Colette L. Massachusetts Institute of Technology. Department of Civil and Environmental Engineering Heald, Colette L. We use a global coupled chemistry–climate–land model (CESM) to assess the integrated effect of climate, emissions and land use changes on annual surface O[subscript 3] and PM[subscript 2.5] in the United States with a focus on national parks (NPs) and wilderness areas, using the RCP4.5 and RCP8.5 projections. We show that, when stringent domestic emission controls are applied, air quality is predicted to improve across the US, except surface O[subscript 3] over the western and central US under RCP8.5 conditions, where rising background ozone counteracts domestic emission reductions. Under the RCP4.5 scenario, surface O[subscript 3] is substantially reduced (about 5 ppb), with daily maximum 8 h averages below the primary US Environmental Protection Agency (EPA) National Ambient Air Quality Standards (NAAQS) of 75 ppb (and even 65 ppb) in all the NPs. PM[subscript 2.5] is significantly reduced in both scenarios (4 μg m[superscript −3]; ~50%), with levels below the annual US EPA NAAQS of 12 μg m[superscript −3] across all the NPs; visibility is also improved (10–15 dv; >75 km in visibility range), although some western US parks with Class I status (40–74 % of total sites in the US) are still above the 2050 planned target level to reach the goal of natural visibility conditions by 2064. We estimate that climate-driven increases in fire activity may dominate summertime PM2.5 over the western US, potentially offsetting the large PM2.5 reductions from domestic emission controls, and keeping visibility at present-day levels in many parks. Our study indicates that anthropogenic emission patterns will be important for air quality in 2050. However, climate and land use changes alone may lead to a substantial increase in surface O[subscript 3] (2–3 ppb) with important consequences for O[subscript 3] air quality and ecosystem degradation at the US NPs. Our study illustrates the need to consider the effects of changes in climate, vegetation, and fires in future air quality management and planning and emission policy making. United States. National Park Service (Grant H2370 094000/J2350103006) National Science Foundation (U.S.) (AGS-1238109) Joint Fire Science Program (13-1-01-4) 2015-04-02T17:49:05Z 2015-04-02T17:49:05Z 2015-03 2015-02 Article http://purl.org/eprint/type/JournalArticle 1680-7324 1680-7316 http://hdl.handle.net/1721.1/96343 Val Martin, M., C. L. Heald, J.-F. Lamarque, S. Tilmes, L. K. Emmons, and B. A. Schichtel. “How Emissions, Climate, and Land Use Change Will Impact Mid-Century Air Quality over the United States: a Focus on Effects at National Parks.” Atmospheric Chemistry and Physics 15, no. 5 (2015): 2805–2823. https://orcid.org/0000-0003-2894-5738 en_US http://dx.doi.org/10.5194/acp-15-2805-2015 Atmospheric Chemistry and Physics Creative Commons Attribution http://creativecommons.org/licenses/by/3.0/ application/pdf Copernicus GmbH Copernicus Publications
spellingShingle Val Martin, M.
Lamarque, Jean-Francois
Tilmes, S.
Emmons, L. K.
Schichtel, B. A.
Heald, Colette L.
How emissions, climate, and land use change will impact mid-century air quality over the United States: a focus on effects at national parks
title How emissions, climate, and land use change will impact mid-century air quality over the United States: a focus on effects at national parks
title_full How emissions, climate, and land use change will impact mid-century air quality over the United States: a focus on effects at national parks
title_fullStr How emissions, climate, and land use change will impact mid-century air quality over the United States: a focus on effects at national parks
title_full_unstemmed How emissions, climate, and land use change will impact mid-century air quality over the United States: a focus on effects at national parks
title_short How emissions, climate, and land use change will impact mid-century air quality over the United States: a focus on effects at national parks
title_sort how emissions climate and land use change will impact mid century air quality over the united states a focus on effects at national parks
url http://hdl.handle.net/1721.1/96343
https://orcid.org/0000-0003-2894-5738
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