Preventing and reversing vacuum-induced optical losses in high-finesse tantalum (V) oxide mirror coatings

High-finesse optical cavities placed under vacuum are foundational platforms in quantum information science with photons and atoms. We study the vacuum-induced degradation of high-finesse optical cavities with mirror coatings composed of SiO[subscript 2]-Ta[subscript 2]O[subscript 5] dielectric stac...

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Main Authors: Gangloff, Dorian, Shi, Molu, Wu, Tailin, Bylinskii, Alexei, Braverman, Boris, Nichols, Rosanna, Li, Junru, Aichholz, Kai, Cetina, Marko, Karpa, Leon, Gutierrez, Michael Steven, Jelenkovic, Branislav, Vuletic, Vladan, Chuang, Isaac L.
Other Authors: Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science
Format: Article
Language:en_US
Published: Optical Society of America 2015
Online Access:http://hdl.handle.net/1721.1/99933
https://orcid.org/0000-0001-7296-523X
https://orcid.org/0000-0002-7054-2310
https://orcid.org/0000-0001-8586-4999
https://orcid.org/0000-0001-5193-2711
https://orcid.org/0000-0002-9786-0538
https://orcid.org/0000-0001-6155-9463
https://orcid.org/0000-0001-8276-8256
https://orcid.org/0000-0002-8069-8327
https://orcid.org/0000-0002-7100-0847
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author Gangloff, Dorian
Shi, Molu
Wu, Tailin
Bylinskii, Alexei
Braverman, Boris
Nichols, Rosanna
Li, Junru
Aichholz, Kai
Cetina, Marko
Karpa, Leon
Gutierrez, Michael Steven
Jelenkovic, Branislav
Vuletic, Vladan
Chuang, Isaac L.
author2 Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science
author_facet Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science
Gangloff, Dorian
Shi, Molu
Wu, Tailin
Bylinskii, Alexei
Braverman, Boris
Nichols, Rosanna
Li, Junru
Aichholz, Kai
Cetina, Marko
Karpa, Leon
Gutierrez, Michael Steven
Jelenkovic, Branislav
Vuletic, Vladan
Chuang, Isaac L.
author_sort Gangloff, Dorian
collection MIT
description High-finesse optical cavities placed under vacuum are foundational platforms in quantum information science with photons and atoms. We study the vacuum-induced degradation of high-finesse optical cavities with mirror coatings composed of SiO[subscript 2]-Ta[subscript 2]O[subscript 5] dielectric stacks, and present methods to protect these coatings and to recover their initial low loss levels. For separate coatings with reflectivities centered at 370 nm and 422 nm, a vacuum-induced continuous increase in optical loss occurs if the surface-layer coating is made of Ta[subscript 2]O[subscript 5], while it does not occur if it is made of SiO[subscript 2]. The incurred optical loss can be reversed by filling the vacuum chamber with oxygen at atmospheric pressure, and the recovery rate can be strongly accelerated by continuous laser illumination at 422 nm. Both the degradation and the recovery processes depend strongly on temperature. We find that a 1 nm-thick layer of SiO[subscript 2] passivating the Ta[subscript 2]O[subscript 5] surface layer is sufficient to reduce the degradation rate by more than a factor of 10, strongly supporting surface oxygen depletion as the primary degradation mechanism.
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spelling mit-1721.1/999332022-09-30T08:30:43Z Preventing and reversing vacuum-induced optical losses in high-finesse tantalum (V) oxide mirror coatings Gangloff, Dorian Shi, Molu Wu, Tailin Bylinskii, Alexei Braverman, Boris Nichols, Rosanna Li, Junru Aichholz, Kai Cetina, Marko Karpa, Leon Gutierrez, Michael Steven Jelenkovic, Branislav Vuletic, Vladan Chuang, Isaac L. Massachusetts Institute of Technology. Department of Electrical Engineering and Computer Science Massachusetts Institute of Technology. Department of Physics Massachusetts Institute of Technology. Research Laboratory of Electronics MIT-Harvard Center for Ultracold Atoms Gangloff, Dorian Shi, Molu Wu, Tailin Bylinskii, Alexei Braverman, Boris Gutierrez, Michael Steven Nichols, Rosanna Li, Junru Aichholz, Kai Cetina, Marko Karpa, Leon Chuang, Isaac Vuletic, Vladan High-finesse optical cavities placed under vacuum are foundational platforms in quantum information science with photons and atoms. We study the vacuum-induced degradation of high-finesse optical cavities with mirror coatings composed of SiO[subscript 2]-Ta[subscript 2]O[subscript 5] dielectric stacks, and present methods to protect these coatings and to recover their initial low loss levels. For separate coatings with reflectivities centered at 370 nm and 422 nm, a vacuum-induced continuous increase in optical loss occurs if the surface-layer coating is made of Ta[subscript 2]O[subscript 5], while it does not occur if it is made of SiO[subscript 2]. The incurred optical loss can be reversed by filling the vacuum chamber with oxygen at atmospheric pressure, and the recovery rate can be strongly accelerated by continuous laser illumination at 422 nm. Both the degradation and the recovery processes depend strongly on temperature. We find that a 1 nm-thick layer of SiO[subscript 2] passivating the Ta[subscript 2]O[subscript 5] surface layer is sufficient to reduce the degradation rate by more than a factor of 10, strongly supporting surface oxygen depletion as the primary degradation mechanism. National Science Foundation (U.S.). Center for Ultracold Atoms United States. Intelligence Advanced Research Projects Activity. Multi-Qubit Coherent Operations Program 2015-11-16T13:08:46Z 2015-11-16T13:08:46Z 2015-07 2015-06 Article http://purl.org/eprint/type/JournalArticle 1094-4087 http://hdl.handle.net/1721.1/99933 Gangloff, Dorian, Molu Shi, Tailin Wu, Alexei Bylinskii, Boris Braverman, Michael Gutierrez, Rosanna Nichols, et al. “Preventing and Reversing Vacuum-Induced Optical Losses in High-Finesse Tantalum (V) Oxide Mirror Coatings.” Optics Express 23, no. 14 (2015): 18014. https://orcid.org/0000-0001-7296-523X https://orcid.org/0000-0002-7054-2310 https://orcid.org/0000-0001-8586-4999 https://orcid.org/0000-0001-5193-2711 https://orcid.org/0000-0002-9786-0538 https://orcid.org/0000-0001-6155-9463 https://orcid.org/0000-0001-8276-8256 https://orcid.org/0000-0002-8069-8327 https://orcid.org/0000-0002-7100-0847 en_US http://dx.doi.org/10.1364/oe.23.018014 Optics Express Creative Commons Attribution-Noncommercial-Share Alike http://creativecommons.org/licenses/by-nc-sa/4.0/ application/pdf Optical Society of America arXiv
spellingShingle Gangloff, Dorian
Shi, Molu
Wu, Tailin
Bylinskii, Alexei
Braverman, Boris
Nichols, Rosanna
Li, Junru
Aichholz, Kai
Cetina, Marko
Karpa, Leon
Gutierrez, Michael Steven
Jelenkovic, Branislav
Vuletic, Vladan
Chuang, Isaac L.
Preventing and reversing vacuum-induced optical losses in high-finesse tantalum (V) oxide mirror coatings
title Preventing and reversing vacuum-induced optical losses in high-finesse tantalum (V) oxide mirror coatings
title_full Preventing and reversing vacuum-induced optical losses in high-finesse tantalum (V) oxide mirror coatings
title_fullStr Preventing and reversing vacuum-induced optical losses in high-finesse tantalum (V) oxide mirror coatings
title_full_unstemmed Preventing and reversing vacuum-induced optical losses in high-finesse tantalum (V) oxide mirror coatings
title_short Preventing and reversing vacuum-induced optical losses in high-finesse tantalum (V) oxide mirror coatings
title_sort preventing and reversing vacuum induced optical losses in high finesse tantalum v oxide mirror coatings
url http://hdl.handle.net/1721.1/99933
https://orcid.org/0000-0001-7296-523X
https://orcid.org/0000-0002-7054-2310
https://orcid.org/0000-0001-8586-4999
https://orcid.org/0000-0001-5193-2711
https://orcid.org/0000-0002-9786-0538
https://orcid.org/0000-0001-6155-9463
https://orcid.org/0000-0001-8276-8256
https://orcid.org/0000-0002-8069-8327
https://orcid.org/0000-0002-7100-0847
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