Width of phonon sidebands in the Brownian oscillator model

The line width dependence of zero-phonon lines and phonon sidebands on temperature, bath dissipation, and electron−phonon coupling is studied for an underdamped Brownian oscillator model with an Ohmic dissipative bath. Factors determining the line widths vary from the zero-phonon lines to the phonon...

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Main Authors: Ye, Jun, Zhao, Yang, Ng, Nathaniel, Cao, Jianshu
Other Authors: School of Materials Science & Engineering
Format: Journal Article
Language:English
Published: 2011
Subjects:
Online Access:https://hdl.handle.net/10356/101328
http://hdl.handle.net/10220/7401
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author Ye, Jun
Zhao, Yang
Ng, Nathaniel
Cao, Jianshu
author2 School of Materials Science & Engineering
author_facet School of Materials Science & Engineering
Ye, Jun
Zhao, Yang
Ng, Nathaniel
Cao, Jianshu
author_sort Ye, Jun
collection NTU
description The line width dependence of zero-phonon lines and phonon sidebands on temperature, bath dissipation, and electron−phonon coupling is studied for an underdamped Brownian oscillator model with an Ohmic dissipative bath. Factors determining the line widths vary from the zero-phonon lines to the phonon sidebands. The control-parameter space of line broadening has been mapped out, revealing that the line widths of the zero-phonon lines and phonon sidebands are linearly dependent on both the temperature and the Huang−Rhys factor. It is also found that the dependence of the line widths on the bath damping factor is linear for the zero-phonon lines and quadratic for the phonon sidebands.
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spelling ntu-10356/1013282020-06-01T10:26:49Z Width of phonon sidebands in the Brownian oscillator model Ye, Jun Zhao, Yang Ng, Nathaniel Cao, Jianshu School of Materials Science & Engineering DRNTU::Science::Chemistry::Physical chemistry::Solid state chemistry The line width dependence of zero-phonon lines and phonon sidebands on temperature, bath dissipation, and electron−phonon coupling is studied for an underdamped Brownian oscillator model with an Ohmic dissipative bath. Factors determining the line widths vary from the zero-phonon lines to the phonon sidebands. The control-parameter space of line broadening has been mapped out, revealing that the line widths of the zero-phonon lines and phonon sidebands are linearly dependent on both the temperature and the Huang−Rhys factor. It is also found that the dependence of the line widths on the bath damping factor is linear for the zero-phonon lines and quadratic for the phonon sidebands. 2011-12-15T06:18:19Z 2019-12-06T20:36:46Z 2011-12-15T06:18:19Z 2019-12-06T20:36:46Z 2009 2009 Journal Article Ye, J., Zhao, Y., Ng, N., & Cao, J. (2009). Width of Phonon Sidebands in the Brownian Oscillator Model. Journal of Physical Chemistry B, 113 (17), 5897–5904. https://hdl.handle.net/10356/101328 http://hdl.handle.net/10220/7401 10.1021/jp809425g en Journal of physical chemistry B © 2009 American Chemical Society
spellingShingle DRNTU::Science::Chemistry::Physical chemistry::Solid state chemistry
Ye, Jun
Zhao, Yang
Ng, Nathaniel
Cao, Jianshu
Width of phonon sidebands in the Brownian oscillator model
title Width of phonon sidebands in the Brownian oscillator model
title_full Width of phonon sidebands in the Brownian oscillator model
title_fullStr Width of phonon sidebands in the Brownian oscillator model
title_full_unstemmed Width of phonon sidebands in the Brownian oscillator model
title_short Width of phonon sidebands in the Brownian oscillator model
title_sort width of phonon sidebands in the brownian oscillator model
topic DRNTU::Science::Chemistry::Physical chemistry::Solid state chemistry
url https://hdl.handle.net/10356/101328
http://hdl.handle.net/10220/7401
work_keys_str_mv AT yejun widthofphononsidebandsinthebrownianoscillatormodel
AT zhaoyang widthofphononsidebandsinthebrownianoscillatormodel
AT ngnathaniel widthofphononsidebandsinthebrownianoscillatormodel
AT caojianshu widthofphononsidebandsinthebrownianoscillatormodel