Noble-metal-free NiS/C3N4 for efficient photocatalytic hydrogen evolution from water
A NiS/C3N4 photocatalyst containing earth-abundant elements only was constructed by means of a simple hydrothermal method. This photocatalyst shows efficient hydrogen evolution (48.2 μmol h−1) under visible light when using triethanolamine as a sacrificial reagent. The optimal loading of 1.1 wt % Ni...
| Main Authors: | , , , , |
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| Other Authors: | |
| Format: | Journal Article |
| Language: | English |
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2014
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| Online Access: | https://hdl.handle.net/10356/101707 http://hdl.handle.net/10220/19783 |
| _version_ | 1826120175244541952 |
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| author | Hong, Jindui Wang, Yongsheng Wang, Yabo Zhang, Wei Xu, Rong |
| author2 | School of Chemical and Biomedical Engineering |
| author_facet | School of Chemical and Biomedical Engineering Hong, Jindui Wang, Yongsheng Wang, Yabo Zhang, Wei Xu, Rong |
| author_sort | Hong, Jindui |
| collection | NTU |
| description | A NiS/C3N4 photocatalyst containing earth-abundant elements only was constructed by means of a simple hydrothermal method. This photocatalyst shows efficient hydrogen evolution (48.2 μmol h−1) under visible light when using triethanolamine as a sacrificial reagent. The optimal loading of 1.1 wt % NiS on C3N4 as a cocatalyst can enhance the H2 production by about 250 times compared with the native C3N4. The highest apparent quantum efficiency of 1.9 % was recorded at 440 nm. |
| first_indexed | 2024-10-01T05:12:13Z |
| format | Journal Article |
| id | ntu-10356/101707 |
| institution | Nanyang Technological University |
| language | English |
| last_indexed | 2024-10-01T05:12:13Z |
| publishDate | 2014 |
| record_format | dspace |
| spelling | ntu-10356/1017072020-03-07T11:40:20Z Noble-metal-free NiS/C3N4 for efficient photocatalytic hydrogen evolution from water Hong, Jindui Wang, Yongsheng Wang, Yabo Zhang, Wei Xu, Rong School of Chemical and Biomedical Engineering School of Mechanical and Aerospace Engineering DRNTU::Science::Chemistry::Physical chemistry::Catalysis A NiS/C3N4 photocatalyst containing earth-abundant elements only was constructed by means of a simple hydrothermal method. This photocatalyst shows efficient hydrogen evolution (48.2 μmol h−1) under visible light when using triethanolamine as a sacrificial reagent. The optimal loading of 1.1 wt % NiS on C3N4 as a cocatalyst can enhance the H2 production by about 250 times compared with the native C3N4. The highest apparent quantum efficiency of 1.9 % was recorded at 440 nm. NRF (Natl Research Foundation, S’pore) 2014-06-16T03:25:52Z 2019-12-06T20:43:06Z 2014-06-16T03:25:52Z 2019-12-06T20:43:06Z 2013 2013 Journal Article Hong, J., Wang, Y., Wang, Y., Zhang, W., & Xu, R. (2013). Noble-Metal-Free NiS/C3N4 for Efficient Photocatalytic Hydrogen Evolution from Water . ChemSusChem, 6(12), 2263-2268. 1864-5631 https://hdl.handle.net/10356/101707 http://hdl.handle.net/10220/19783 10.1002/cssc.201300647 en Chemsuschem © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. |
| spellingShingle | DRNTU::Science::Chemistry::Physical chemistry::Catalysis Hong, Jindui Wang, Yongsheng Wang, Yabo Zhang, Wei Xu, Rong Noble-metal-free NiS/C3N4 for efficient photocatalytic hydrogen evolution from water |
| title | Noble-metal-free NiS/C3N4 for efficient photocatalytic hydrogen evolution from water |
| title_full | Noble-metal-free NiS/C3N4 for efficient photocatalytic hydrogen evolution from water |
| title_fullStr | Noble-metal-free NiS/C3N4 for efficient photocatalytic hydrogen evolution from water |
| title_full_unstemmed | Noble-metal-free NiS/C3N4 for efficient photocatalytic hydrogen evolution from water |
| title_short | Noble-metal-free NiS/C3N4 for efficient photocatalytic hydrogen evolution from water |
| title_sort | noble metal free nis c3n4 for efficient photocatalytic hydrogen evolution from water |
| topic | DRNTU::Science::Chemistry::Physical chemistry::Catalysis |
| url | https://hdl.handle.net/10356/101707 http://hdl.handle.net/10220/19783 |
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