Humic acid-induced formation of tobermorite upon hydrothermal treatment with municipal solid waste incineration bottom ash and its application for efficient removal of Cu(II) ions

In this study, conversion of municipal solid waste incineration bottom ash (IBA) into highly efficient sorbents for Cu(II) removal was reported. The formation of tobermorite induced by humic acid (HA) and IBA under hydrothermal condition was explored and its potential application for efficient remov...

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Main Authors: Luo, Hongwei, He, Dongqin, Zhu, Weiping, Wu, Yichao, Chen, Zhitao, Yang, En-Hua
Other Authors: School of Civil and Environmental Engineering
Format: Journal Article
Language:English
Published: 2019
Subjects:
Online Access:https://hdl.handle.net/10356/104247
http://hdl.handle.net/10220/50211
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author Luo, Hongwei
He, Dongqin
Zhu, Weiping
Wu, Yichao
Chen, Zhitao
Yang, En-Hua
author2 School of Civil and Environmental Engineering
author_facet School of Civil and Environmental Engineering
Luo, Hongwei
He, Dongqin
Zhu, Weiping
Wu, Yichao
Chen, Zhitao
Yang, En-Hua
author_sort Luo, Hongwei
collection NTU
description In this study, conversion of municipal solid waste incineration bottom ash (IBA) into highly efficient sorbents for Cu(II) removal was reported. The formation of tobermorite induced by humic acid (HA) and IBA under hydrothermal condition was explored and its potential application for efficient removal of Cu(II) ions was further investigated. After hydrothermal treatment, the morphology and microstructure of IBA remarkably changed from sheet-like to particle-like, thereby resulting in substantial increases of sorption capacity. The synthesized tobermorite exhibited a strongly enhanced sorption performance toward Cu(II), which was 270.3 mg g 1 and higher than other reported sorbents. The adsorption behaviors were subsequently examined by isotherm and kinetic studies. Langmuir model was found to describe the adsorption process well, suggesting that the adsorption was chemisorption in nature. Therefore, the hydrothermally synthesized tobermorite may be used as sorbents to remove Cu(II). Conversion of IBA into valuable minerals recovers waste into potential resources and alleviates the needs for ash disposal.
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spelling ntu-10356/1042472021-02-15T05:22:20Z Humic acid-induced formation of tobermorite upon hydrothermal treatment with municipal solid waste incineration bottom ash and its application for efficient removal of Cu(II) ions Luo, Hongwei He, Dongqin Zhu, Weiping Wu, Yichao Chen, Zhitao Yang, En-Hua School of Civil and Environmental Engineering Energy Research Institute @ NTU (ERI@N) Incineration Bottom Ash (IBA) Municipal Solid Waste (MSW) Engineering::Civil engineering In this study, conversion of municipal solid waste incineration bottom ash (IBA) into highly efficient sorbents for Cu(II) removal was reported. The formation of tobermorite induced by humic acid (HA) and IBA under hydrothermal condition was explored and its potential application for efficient removal of Cu(II) ions was further investigated. After hydrothermal treatment, the morphology and microstructure of IBA remarkably changed from sheet-like to particle-like, thereby resulting in substantial increases of sorption capacity. The synthesized tobermorite exhibited a strongly enhanced sorption performance toward Cu(II), which was 270.3 mg g 1 and higher than other reported sorbents. The adsorption behaviors were subsequently examined by isotherm and kinetic studies. Langmuir model was found to describe the adsorption process well, suggesting that the adsorption was chemisorption in nature. Therefore, the hydrothermally synthesized tobermorite may be used as sorbents to remove Cu(II). Conversion of IBA into valuable minerals recovers waste into potential resources and alleviates the needs for ash disposal. Accepted version 2019-10-22T02:19:36Z 2019-12-06T21:28:59Z 2019-10-22T02:19:36Z 2019-12-06T21:28:59Z 2019 Journal Article Luo, H., He, D., Zhu, W., Wu, Y., Chen, Z., & Yang, E.-H. (2019). Humic acid-induced formation of tobermorite upon hydrothermal treatment with municipal solid waste incineration bottom ash and its application for efficient removal of Cu(II) ions. Waste Management, 84, 83-90. doi:10.1016/j.wasman.2018.11.037 0956-053X https://hdl.handle.net/10356/104247 http://hdl.handle.net/10220/50211 10.1016/j.wasman.2018.11.037 84 83 90 en Waste Management © 2019 Elsevier. All rights reserved. This paper was published in Waste Management and is made available with permission of Elsevier. 32 p. application/pdf
spellingShingle Incineration Bottom Ash (IBA)
Municipal Solid Waste (MSW)
Engineering::Civil engineering
Luo, Hongwei
He, Dongqin
Zhu, Weiping
Wu, Yichao
Chen, Zhitao
Yang, En-Hua
Humic acid-induced formation of tobermorite upon hydrothermal treatment with municipal solid waste incineration bottom ash and its application for efficient removal of Cu(II) ions
title Humic acid-induced formation of tobermorite upon hydrothermal treatment with municipal solid waste incineration bottom ash and its application for efficient removal of Cu(II) ions
title_full Humic acid-induced formation of tobermorite upon hydrothermal treatment with municipal solid waste incineration bottom ash and its application for efficient removal of Cu(II) ions
title_fullStr Humic acid-induced formation of tobermorite upon hydrothermal treatment with municipal solid waste incineration bottom ash and its application for efficient removal of Cu(II) ions
title_full_unstemmed Humic acid-induced formation of tobermorite upon hydrothermal treatment with municipal solid waste incineration bottom ash and its application for efficient removal of Cu(II) ions
title_short Humic acid-induced formation of tobermorite upon hydrothermal treatment with municipal solid waste incineration bottom ash and its application for efficient removal of Cu(II) ions
title_sort humic acid induced formation of tobermorite upon hydrothermal treatment with municipal solid waste incineration bottom ash and its application for efficient removal of cu ii ions
topic Incineration Bottom Ash (IBA)
Municipal Solid Waste (MSW)
Engineering::Civil engineering
url https://hdl.handle.net/10356/104247
http://hdl.handle.net/10220/50211
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