Magnetism induced by excess electrons trapped at diamagnetic edge-quantum well in multi-layer graphene

In this paper, we clarified a robust mechanism of magnetism generated by excess electrons captured by edge-quantum well of diamagnetic armchair edges. Consistency between density functional theory calculations and electron cyclotron resonance experiments verified that: (1) Multi-layer armchair nanor...

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Main Authors: Zhang, Xi, Wang, Chao, Diao, Dongfeng, Sun, Chang Qing
Other Authors: School of Electrical and Electronic Engineering
Format: Journal Article
Language:English
Published: 2014
Subjects:
Online Access:https://hdl.handle.net/10356/104885
http://hdl.handle.net/10220/20367
http://dx.doi.org/10.1063/1.4891558
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author Zhang, Xi
Wang, Chao
Diao, Dongfeng
Sun, Chang Qing
author2 School of Electrical and Electronic Engineering
author_facet School of Electrical and Electronic Engineering
Zhang, Xi
Wang, Chao
Diao, Dongfeng
Sun, Chang Qing
author_sort Zhang, Xi
collection NTU
description In this paper, we clarified a robust mechanism of magnetism generated by excess electrons captured by edge-quantum well of diamagnetic armchair edges. Consistency between density functional theory calculations and electron cyclotron resonance experiments verified that: (1) Multi-layer armchair nanoribbons are stable with proper amounts of excess electrons which can provide net spin; (2) Since under-coordination induces lattice relaxation and potential well modulation, electrons tend to be trapped at edges; and (3) Neither large amount of excess electrons nor positive charges can induce magnetism. This work shed light on the development of graphene devices in its magnetic applications.
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spelling ntu-10356/1048852019-12-06T21:41:58Z Magnetism induced by excess electrons trapped at diamagnetic edge-quantum well in multi-layer graphene Zhang, Xi Wang, Chao Diao, Dongfeng Sun, Chang Qing School of Electrical and Electronic Engineering DRNTU::Engineering::Electrical and electronic engineering In this paper, we clarified a robust mechanism of magnetism generated by excess electrons captured by edge-quantum well of diamagnetic armchair edges. Consistency between density functional theory calculations and electron cyclotron resonance experiments verified that: (1) Multi-layer armchair nanoribbons are stable with proper amounts of excess electrons which can provide net spin; (2) Since under-coordination induces lattice relaxation and potential well modulation, electrons tend to be trapped at edges; and (3) Neither large amount of excess electrons nor positive charges can induce magnetism. This work shed light on the development of graphene devices in its magnetic applications. Published version 2014-08-21T06:21:42Z 2019-12-06T21:41:58Z 2014-08-21T06:21:42Z 2019-12-06T21:41:58Z 2014 2014 Journal Article Zhang, X., Wang, C., Sun, C. Q., & Diao, D. (2014). Magnetism induced by excess electrons trapped at diamagnetic edge-quantum well in multi-layer graphene. Applied Physics Letters, 105(4), 042402-. 0003-6951 https://hdl.handle.net/10356/104885 http://hdl.handle.net/10220/20367 http://dx.doi.org/10.1063/1.4891558 en Applied physics letters © 2014 AIP Publishing LLC. This paper was published in Applied Physics Letters and is made available as an electronic reprint (preprint) with permission of AIP Publishing LLC. The paper can be found at the following official DOI: [http://dx.doi.org/10.1063/1.4891558].  One print or electronic copy may be made for personal use only. Systematic or multiple reproduction, distribution to multiple locations via electronic or other means, duplication of any material in this paper for a fee or for commercial purposes, or modification of the content of the paper is prohibited and is subject to penalties under law. application/pdf
spellingShingle DRNTU::Engineering::Electrical and electronic engineering
Zhang, Xi
Wang, Chao
Diao, Dongfeng
Sun, Chang Qing
Magnetism induced by excess electrons trapped at diamagnetic edge-quantum well in multi-layer graphene
title Magnetism induced by excess electrons trapped at diamagnetic edge-quantum well in multi-layer graphene
title_full Magnetism induced by excess electrons trapped at diamagnetic edge-quantum well in multi-layer graphene
title_fullStr Magnetism induced by excess electrons trapped at diamagnetic edge-quantum well in multi-layer graphene
title_full_unstemmed Magnetism induced by excess electrons trapped at diamagnetic edge-quantum well in multi-layer graphene
title_short Magnetism induced by excess electrons trapped at diamagnetic edge-quantum well in multi-layer graphene
title_sort magnetism induced by excess electrons trapped at diamagnetic edge quantum well in multi layer graphene
topic DRNTU::Engineering::Electrical and electronic engineering
url https://hdl.handle.net/10356/104885
http://hdl.handle.net/10220/20367
http://dx.doi.org/10.1063/1.4891558
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AT diaodongfeng magnetisminducedbyexcesselectronstrappedatdiamagneticedgequantumwellinmultilayergraphene
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