Electrical and thermal effects on electromechanical performance of stretchable thin gold films on PDMS substrates for stretchable electronics

Stretchable electrodes comprising thin gold films with initial nanocracks on elastic substrates of poly(dimethylsiloxane) are developed in this work, which can be stretched reversibly while maintaining conductivity to an applied uniaxial strain as large as 120%. Reliable electromechanical performanc...

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Main Authors: Zhao, Yang, Yu, Mei, Liu, Zhiyuan, Yu, Zhe
Other Authors: School of Materials Science & Engineering
Format: Journal Article
Language:English
Published: 2019
Subjects:
Online Access:https://hdl.handle.net/10356/105009
http://hdl.handle.net/10220/48664
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author Zhao, Yang
Yu, Mei
Liu, Zhiyuan
Yu, Zhe
author2 School of Materials Science & Engineering
author_facet School of Materials Science & Engineering
Zhao, Yang
Yu, Mei
Liu, Zhiyuan
Yu, Zhe
author_sort Zhao, Yang
collection NTU
description Stretchable electrodes comprising thin gold films with initial nanocracks on elastic substrates of poly(dimethylsiloxane) are developed in this work, which can be stretched reversibly while maintaining conductivity to an applied uniaxial strain as large as 120%. Reliable electromechanical performance is essential for the application of stretchable electronics as bioelectronic interfaces under various working conditions; therefore, the electrical and thermal effects on the electromechanical performance of the stretchable gold film electrodes are investigated in this work. It is found that the stretchability deteriorates to some extent depending on the electrical and thermal treatments. Microstructures and stress analysis in the cracks are studied, along with crack quantification. It is believed that the decrease of the stretchability is ascribed to the combination of the crack widening by thermal mismatch stress and crack tip smoothening by the electromigration phenomenon. Therefore, the current density and temperature through the electrodes should be controlled within a certain range for wide applications in order to maintain a stable performance of the electrodes. This study also provides some guiding significance for the design of other stretchable electronic devices composed of two materials with large different physical properties.
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spelling ntu-10356/1050092023-07-14T15:55:59Z Electrical and thermal effects on electromechanical performance of stretchable thin gold films on PDMS substrates for stretchable electronics Zhao, Yang Yu, Mei Liu, Zhiyuan Yu, Zhe School of Materials Science & Engineering Electromigation DRNTU::Engineering::Materials Electrodes Stretchable electrodes comprising thin gold films with initial nanocracks on elastic substrates of poly(dimethylsiloxane) are developed in this work, which can be stretched reversibly while maintaining conductivity to an applied uniaxial strain as large as 120%. Reliable electromechanical performance is essential for the application of stretchable electronics as bioelectronic interfaces under various working conditions; therefore, the electrical and thermal effects on the electromechanical performance of the stretchable gold film electrodes are investigated in this work. It is found that the stretchability deteriorates to some extent depending on the electrical and thermal treatments. Microstructures and stress analysis in the cracks are studied, along with crack quantification. It is believed that the decrease of the stretchability is ascribed to the combination of the crack widening by thermal mismatch stress and crack tip smoothening by the electromigration phenomenon. Therefore, the current density and temperature through the electrodes should be controlled within a certain range for wide applications in order to maintain a stable performance of the electrodes. This study also provides some guiding significance for the design of other stretchable electronic devices composed of two materials with large different physical properties. Published version 2019-06-12T03:58:34Z 2019-12-06T21:44:27Z 2019-06-12T03:58:34Z 2019-12-06T21:44:27Z 2019 Journal Article Zhao, Y., Yu, M., Liu, Z., & Yu, Z. (2019). Electrical and thermal effects on electromechanical performance of stretchable thin gold films on PDMS substrates for stretchable electronics. Journal of Applied Physics, 125(16), 165305-. doi:10.1063/1.5079435 0021-8979 https://hdl.handle.net/10356/105009 http://hdl.handle.net/10220/48664 10.1063/1.5079435 en Journal of Applied Physics © 2019 The Author(s). All rights reserved. This paper was published by AIP in Journal of Applied Physics and is made available with permission of The Author(s). 7 p. application/pdf
spellingShingle Electromigation
DRNTU::Engineering::Materials
Electrodes
Zhao, Yang
Yu, Mei
Liu, Zhiyuan
Yu, Zhe
Electrical and thermal effects on electromechanical performance of stretchable thin gold films on PDMS substrates for stretchable electronics
title Electrical and thermal effects on electromechanical performance of stretchable thin gold films on PDMS substrates for stretchable electronics
title_full Electrical and thermal effects on electromechanical performance of stretchable thin gold films on PDMS substrates for stretchable electronics
title_fullStr Electrical and thermal effects on electromechanical performance of stretchable thin gold films on PDMS substrates for stretchable electronics
title_full_unstemmed Electrical and thermal effects on electromechanical performance of stretchable thin gold films on PDMS substrates for stretchable electronics
title_short Electrical and thermal effects on electromechanical performance of stretchable thin gold films on PDMS substrates for stretchable electronics
title_sort electrical and thermal effects on electromechanical performance of stretchable thin gold films on pdms substrates for stretchable electronics
topic Electromigation
DRNTU::Engineering::Materials
Electrodes
url https://hdl.handle.net/10356/105009
http://hdl.handle.net/10220/48664
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