Stability, dynamics, and tolerance to undersaturation of surface nanobubbles

The theoretical understanding of surface nanobubbles—nanoscale gaseous domains on immersed substrates—revolves around two contrasting perspectives. One perspective, which considers gas transport in the nanobubbles’ vicinity, explains numerous stability-related properties but systematically underesti...

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Main Authors: Tan, Beng Hau, An, Hongjie, Ohl, Claus-Dieter
Other Authors: School of Physical and Mathematical Sciences
Format: Journal Article
Language:English
Published: 2019
Subjects:
Online Access:https://hdl.handle.net/10356/105417
http://hdl.handle.net/10220/48672
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author Tan, Beng Hau
An, Hongjie
Ohl, Claus-Dieter
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Tan, Beng Hau
An, Hongjie
Ohl, Claus-Dieter
author_sort Tan, Beng Hau
collection NTU
description The theoretical understanding of surface nanobubbles—nanoscale gaseous domains on immersed substrates—revolves around two contrasting perspectives. One perspective, which considers gas transport in the nanobubbles’ vicinity, explains numerous stability-related properties but systematically underestimates the dynamical response timescale by orders of magnitude. The other perspective, which considers gas transport as the bulk liquid equilibrates with the external environment, recovers the experimentally observed dynamical timescale but incorrectly predicts that nanobubbles progressively shrink until dissolution. We propose a model that couples both perspectives, which is capable of explaining the stability, dynamics, and unexpected tolerance of surface nanobubbles to undersaturated environments.
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spelling ntu-10356/1054172023-02-28T19:39:55Z Stability, dynamics, and tolerance to undersaturation of surface nanobubbles Tan, Beng Hau An, Hongjie Ohl, Claus-Dieter School of Physical and Mathematical Sciences Singapore-MIT Alliance Programme Nanobubbles Polymers and Soft Matter DRNTU::Science::Physics The theoretical understanding of surface nanobubbles—nanoscale gaseous domains on immersed substrates—revolves around two contrasting perspectives. One perspective, which considers gas transport in the nanobubbles’ vicinity, explains numerous stability-related properties but systematically underestimates the dynamical response timescale by orders of magnitude. The other perspective, which considers gas transport as the bulk liquid equilibrates with the external environment, recovers the experimentally observed dynamical timescale but incorrectly predicts that nanobubbles progressively shrink until dissolution. We propose a model that couples both perspectives, which is capable of explaining the stability, dynamics, and unexpected tolerance of surface nanobubbles to undersaturated environments. Published version 2019-06-12T05:54:47Z 2019-12-06T21:50:49Z 2019-06-12T05:54:47Z 2019-12-06T21:50:49Z 2019 Journal Article Tan, B. H., An, H., & Ohl, C.-D. (2019). Stability, dynamics, and tolerance to undersaturation of surface nanobubbles. Physical Review Letters, 122(13), 134502-. doi:10.1103/PhysRevLett.122.134502 0031-9007 https://hdl.handle.net/10356/105417 http://hdl.handle.net/10220/48672 10.1103/PhysRevLett.122.134502 en Physical Review Letters © 2019 American Physical Society. All rights reserved. This paper was published in Physical Review Letters and is made available with permission of American Physical Society. 5 p. application/pdf
spellingShingle Nanobubbles
Polymers and Soft Matter
DRNTU::Science::Physics
Tan, Beng Hau
An, Hongjie
Ohl, Claus-Dieter
Stability, dynamics, and tolerance to undersaturation of surface nanobubbles
title Stability, dynamics, and tolerance to undersaturation of surface nanobubbles
title_full Stability, dynamics, and tolerance to undersaturation of surface nanobubbles
title_fullStr Stability, dynamics, and tolerance to undersaturation of surface nanobubbles
title_full_unstemmed Stability, dynamics, and tolerance to undersaturation of surface nanobubbles
title_short Stability, dynamics, and tolerance to undersaturation of surface nanobubbles
title_sort stability dynamics and tolerance to undersaturation of surface nanobubbles
topic Nanobubbles
Polymers and Soft Matter
DRNTU::Science::Physics
url https://hdl.handle.net/10356/105417
http://hdl.handle.net/10220/48672
work_keys_str_mv AT tanbenghau stabilitydynamicsandtolerancetoundersaturationofsurfacenanobubbles
AT anhongjie stabilitydynamicsandtolerancetoundersaturationofsurfacenanobubbles
AT ohlclausdieter stabilitydynamicsandtolerancetoundersaturationofsurfacenanobubbles