Room temperature nanocavity laser with interlayer excitons in 2D heterostructures

Atomically thin layered two-dimensional (2D) materials have provided a rich library for both fundamental research and device applications. Bandgap engineering and controlled material response can be achieved from artificial heterostructures. Recently, excitonic lasers have been reported using transi...

Full description

Bibliographic Details
Main Authors: Liu, Yuanda, Fang, Hanlin, Abdullah Rasmita, Zhou, Yu, Li, Juntao, Yu, Ting, Xiong, Qihua, Zheludev, Nikolay, Liu, Jin, Gao, Weibo
Other Authors: School of Physical and Mathematical Sciences
Format: Journal Article
Language:English
Published: 2019
Subjects:
Online Access:https://hdl.handle.net/10356/106424
http://hdl.handle.net/10220/48937
_version_ 1826126132879032320
author Liu, Yuanda
Fang, Hanlin
Abdullah Rasmita
Zhou, Yu
Li, Juntao
Yu, Ting
Xiong, Qihua
Zheludev, Nikolay
Liu, Jin
Gao, Weibo
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Liu, Yuanda
Fang, Hanlin
Abdullah Rasmita
Zhou, Yu
Li, Juntao
Yu, Ting
Xiong, Qihua
Zheludev, Nikolay
Liu, Jin
Gao, Weibo
author_sort Liu, Yuanda
collection NTU
description Atomically thin layered two-dimensional (2D) materials have provided a rich library for both fundamental research and device applications. Bandgap engineering and controlled material response can be achieved from artificial heterostructures. Recently, excitonic lasers have been reported using transition metal dichalcogenides; however, the emission is still the intrinsic energy bandgap of the monolayers. Here, we report a room temperature interlayer exciton laser with MoS2/WSe2 heterostructures. The onset of lasing was identified by the distinct kink in the “L-L” curve and the noticeable spectral linewidth collapse. Different from visible emission of intralayer excitons in monolayer components, our laser works in the infrared range, which is fully compatible with the well-established technologies in silicon photonics. Long lifetime of interlayer excitons relaxes the requirement of the cavity quality factor by orders of magnitude. Room temperature interlayer exciton lasers might open new perspectives for developing coherent light sources with tailored optical properties on silicon photonics platforms.
first_indexed 2024-10-01T06:47:43Z
format Journal Article
id ntu-10356/106424
institution Nanyang Technological University
language English
last_indexed 2024-10-01T06:47:43Z
publishDate 2019
record_format dspace
spelling ntu-10356/1064242023-02-28T19:26:12Z Room temperature nanocavity laser with interlayer excitons in 2D heterostructures Liu, Yuanda Fang, Hanlin Abdullah Rasmita Zhou, Yu Li, Juntao Yu, Ting Xiong, Qihua Zheludev, Nikolay Liu, Jin Gao, Weibo School of Physical and Mathematical Sciences The Photonics Institute Centre for Disruptive Photonic Technologies (CDPT) DRNTU::Science::Physics Room Temperature Nanocavity Laser Atomically thin layered two-dimensional (2D) materials have provided a rich library for both fundamental research and device applications. Bandgap engineering and controlled material response can be achieved from artificial heterostructures. Recently, excitonic lasers have been reported using transition metal dichalcogenides; however, the emission is still the intrinsic energy bandgap of the monolayers. Here, we report a room temperature interlayer exciton laser with MoS2/WSe2 heterostructures. The onset of lasing was identified by the distinct kink in the “L-L” curve and the noticeable spectral linewidth collapse. Different from visible emission of intralayer excitons in monolayer components, our laser works in the infrared range, which is fully compatible with the well-established technologies in silicon photonics. Long lifetime of interlayer excitons relaxes the requirement of the cavity quality factor by orders of magnitude. Room temperature interlayer exciton lasers might open new perspectives for developing coherent light sources with tailored optical properties on silicon photonics platforms. NRF (Natl Research Foundation, S’pore) ASTAR (Agency for Sci., Tech. and Research, S’pore) MOE (Min. of Education, S’pore) Published version 2019-06-26T02:42:59Z 2019-12-06T22:11:26Z 2019-06-26T02:42:59Z 2019-12-06T22:11:26Z 2019 Journal Article Liu, Y., Fang, H., Abdullah Rasmita, Zhou, Y., Li, J., Yu, T., . . . Gao, W. (2019). Room temperature nanocavity laser with interlayer excitons in 2D heterostructures. Science Advances, 5(4), eaav4506-. doi:10.1126/sciadv.aav4506 https://hdl.handle.net/10356/106424 http://hdl.handle.net/10220/48937 10.1126/sciadv.aav4506 en Science Advances © 2019 The Author(s). Some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). 5 p. application/pdf
spellingShingle DRNTU::Science::Physics
Room Temperature
Nanocavity Laser
Liu, Yuanda
Fang, Hanlin
Abdullah Rasmita
Zhou, Yu
Li, Juntao
Yu, Ting
Xiong, Qihua
Zheludev, Nikolay
Liu, Jin
Gao, Weibo
Room temperature nanocavity laser with interlayer excitons in 2D heterostructures
title Room temperature nanocavity laser with interlayer excitons in 2D heterostructures
title_full Room temperature nanocavity laser with interlayer excitons in 2D heterostructures
title_fullStr Room temperature nanocavity laser with interlayer excitons in 2D heterostructures
title_full_unstemmed Room temperature nanocavity laser with interlayer excitons in 2D heterostructures
title_short Room temperature nanocavity laser with interlayer excitons in 2D heterostructures
title_sort room temperature nanocavity laser with interlayer excitons in 2d heterostructures
topic DRNTU::Science::Physics
Room Temperature
Nanocavity Laser
url https://hdl.handle.net/10356/106424
http://hdl.handle.net/10220/48937
work_keys_str_mv AT liuyuanda roomtemperaturenanocavitylaserwithinterlayerexcitonsin2dheterostructures
AT fanghanlin roomtemperaturenanocavitylaserwithinterlayerexcitonsin2dheterostructures
AT abdullahrasmita roomtemperaturenanocavitylaserwithinterlayerexcitonsin2dheterostructures
AT zhouyu roomtemperaturenanocavitylaserwithinterlayerexcitonsin2dheterostructures
AT lijuntao roomtemperaturenanocavitylaserwithinterlayerexcitonsin2dheterostructures
AT yuting roomtemperaturenanocavitylaserwithinterlayerexcitonsin2dheterostructures
AT xiongqihua roomtemperaturenanocavitylaserwithinterlayerexcitonsin2dheterostructures
AT zheludevnikolay roomtemperaturenanocavitylaserwithinterlayerexcitonsin2dheterostructures
AT liujin roomtemperaturenanocavitylaserwithinterlayerexcitonsin2dheterostructures
AT gaoweibo roomtemperaturenanocavitylaserwithinterlayerexcitonsin2dheterostructures