Quantifying non-Markovianity for a chromophore-qubit pair in a super-Ohmic bath

An approach based on a non-Markovian time-convolutionless polaron master equation is used to probe the quantum dynamics of a chromophore-qubit in a super-Ohmic bath. Utilizing a measure of non-Markovianity based on dynamical fixed points, we study the effects of the environment temperature and the c...

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Bibliographic Details
Main Authors: Liu, Jing, Sun, Kewei, Wang, Xiaoguang, Zhao, Yang
Other Authors: School of Materials Science & Engineering
Format: Journal Article
Language:English
Published: 2015
Subjects:
Online Access:https://hdl.handle.net/10356/106709
http://hdl.handle.net/10220/25128
Description
Summary:An approach based on a non-Markovian time-convolutionless polaron master equation is used to probe the quantum dynamics of a chromophore-qubit in a super-Ohmic bath. Utilizing a measure of non-Markovianity based on dynamical fixed points, we study the effects of the environment temperature and the coupling strength on the non-Markovian behavior of the chromophore in a super-Ohmic bath. It is found that an increase in the temperature results in a reduction in the backflow information from the environment to the chromophore, and therefore, a suppression of non-Markovianity. In the weak coupling regime, increasing coupling strength will enhance the non-Markovianity, while the effect is reversed in the strong coupling regime.