Engineering 2D architectures toward high-performance micro-supercapacitors

The rise of micro-supercapacitors is satisfying the demand for power storage in portable devices and wireless gadgets. But the miniaturization of the energy-storage components is significantly limited by their energy density. Electrode materials with adequate electrochemical active surfaces are ther...

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Main Authors: Da, Yumin, Liu, Jinxin, Zhou, Lu, Zhu, Xiaohui, Chen, Xiaodong, Fu, Lei
Other Authors: School of Materials Science & Engineering
Format: Journal Article
Language:English
Published: 2020
Subjects:
Online Access:https://hdl.handle.net/10356/138440
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author Da, Yumin
Liu, Jinxin
Zhou, Lu
Zhu, Xiaohui
Chen, Xiaodong
Fu, Lei
author2 School of Materials Science & Engineering
author_facet School of Materials Science & Engineering
Da, Yumin
Liu, Jinxin
Zhou, Lu
Zhu, Xiaohui
Chen, Xiaodong
Fu, Lei
author_sort Da, Yumin
collection NTU
description The rise of micro-supercapacitors is satisfying the demand for power storage in portable devices and wireless gadgets. But the miniaturization of the energy-storage components is significantly limited by their energy density. Electrode materials with adequate electrochemical active surfaces are therefore required for improving performance. 2D materials with ultralarge specific surface areas offer a broad portfolio of the development of high-performance micro-supercapacitors in spite of their several critical drawbacks. An architecture engineering strategy is therefore developed to break these natural limits and maximize the significant advantages of these materials. Based on the approaches of phase transformation, intercalation, surface modification, material hybridization, and hierarchical structuration, 2D architectures with improved conductivity, enlarged specific surface, enhanced redox activity, as well as the unique synergetic effect exhibit great promise in the application of miniaturized supercapacitors with highly enhanced performance. Herein, the architecture engineering of emerging 2D materials beyond graphene toward optimizing the performance of micro-supercapacitors is discussed, in order to promote the application of 2D architectures in miniaturized energy-storage devices.
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spelling ntu-10356/1384402020-06-01T10:01:58Z Engineering 2D architectures toward high-performance micro-supercapacitors Da, Yumin Liu, Jinxin Zhou, Lu Zhu, Xiaohui Chen, Xiaodong Fu, Lei School of Materials Science & Engineering Engineering::Materials 2D Materials Architecture Engineering The rise of micro-supercapacitors is satisfying the demand for power storage in portable devices and wireless gadgets. But the miniaturization of the energy-storage components is significantly limited by their energy density. Electrode materials with adequate electrochemical active surfaces are therefore required for improving performance. 2D materials with ultralarge specific surface areas offer a broad portfolio of the development of high-performance micro-supercapacitors in spite of their several critical drawbacks. An architecture engineering strategy is therefore developed to break these natural limits and maximize the significant advantages of these materials. Based on the approaches of phase transformation, intercalation, surface modification, material hybridization, and hierarchical structuration, 2D architectures with improved conductivity, enlarged specific surface, enhanced redox activity, as well as the unique synergetic effect exhibit great promise in the application of miniaturized supercapacitors with highly enhanced performance. Herein, the architecture engineering of emerging 2D materials beyond graphene toward optimizing the performance of micro-supercapacitors is discussed, in order to promote the application of 2D architectures in miniaturized energy-storage devices. 2020-05-06T03:45:16Z 2020-05-06T03:45:16Z 2018 Journal Article Da, Y., Liu, J., Zhou, L., Zhu, X., Chen, X., & Fu, L. (2018). Engineering 2D architectures toward high-performance micro-supercapacitors. Advanced Materials, 31, 1802793-. doi:10.1002/adma.201802793 0935-9648 https://hdl.handle.net/10356/138440 10.1002/adma.201802793 30133023 2-s2.0-85052372559 31 en Advanced Materials © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. All rights reserved. This paper was published in Advanced Materials and is made available with permission of WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
spellingShingle Engineering::Materials
2D Materials
Architecture Engineering
Da, Yumin
Liu, Jinxin
Zhou, Lu
Zhu, Xiaohui
Chen, Xiaodong
Fu, Lei
Engineering 2D architectures toward high-performance micro-supercapacitors
title Engineering 2D architectures toward high-performance micro-supercapacitors
title_full Engineering 2D architectures toward high-performance micro-supercapacitors
title_fullStr Engineering 2D architectures toward high-performance micro-supercapacitors
title_full_unstemmed Engineering 2D architectures toward high-performance micro-supercapacitors
title_short Engineering 2D architectures toward high-performance micro-supercapacitors
title_sort engineering 2d architectures toward high performance micro supercapacitors
topic Engineering::Materials
2D Materials
Architecture Engineering
url https://hdl.handle.net/10356/138440
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AT liujinxin engineering2darchitecturestowardhighperformancemicrosupercapacitors
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AT zhuxiaohui engineering2darchitecturestowardhighperformancemicrosupercapacitors
AT chenxiaodong engineering2darchitecturestowardhighperformancemicrosupercapacitors
AT fulei engineering2darchitecturestowardhighperformancemicrosupercapacitors