Radiation enhancement by graphene oxide on microelectromechanical system emitters for highly selective gas sensing

Infrared gas sensors have been proven promising for broad applications in Internet of Things and Industrial Internet of Things. However, the lack of miniaturized light sources with good compatibility and tunable spectral features hinders their widespread utilization. Herein, a strategy is proposed t...

Full description

Bibliographic Details
Main Authors: Li, Nanxi, Yuan, Hongye, Xu, Linfang, Tao, Jifang, Ng, Doris Keh Ting, Lee, Lennon Yao Ting, Cheam, Daw Don, Zeng, Yongquan, Qiang, Bo, Wang, Qijie, Cai, Hong, Singh, Navab, Zhao, Dan
Other Authors: School of Electrical and Electronic Engineering
Format: Journal Article
Language:English
Published: 2020
Subjects:
Online Access:https://hdl.handle.net/10356/138671
_version_ 1811679762941214720
author Li, Nanxi
Yuan, Hongye
Xu, Linfang
Tao, Jifang
Ng, Doris Keh Ting
Lee, Lennon Yao Ting
Cheam, Daw Don
Zeng, Yongquan
Qiang, Bo
Wang, Qijie
Cai, Hong
Singh, Navab
Zhao, Dan
author2 School of Electrical and Electronic Engineering
author_facet School of Electrical and Electronic Engineering
Li, Nanxi
Yuan, Hongye
Xu, Linfang
Tao, Jifang
Ng, Doris Keh Ting
Lee, Lennon Yao Ting
Cheam, Daw Don
Zeng, Yongquan
Qiang, Bo
Wang, Qijie
Cai, Hong
Singh, Navab
Zhao, Dan
author_sort Li, Nanxi
collection NTU
description Infrared gas sensors have been proven promising for broad applications in Internet of Things and Industrial Internet of Things. However, the lack of miniaturized light sources with good compatibility and tunable spectral features hinders their widespread utilization. Herein, a strategy is proposed to increase the radiated power from microelectromechanical-based thermal emitters by coating with graphene oxide (GO). The radiation can be substantially enhanced, which partially stems from the high emissivity of GO coating demonstrated by spectroscopic methods. Moreover, the sp2 structure within GO may induce plasmons and thus couple with photons to produce blackbody radiation and/or new thermal emission sources. As a proof-of-concept demonstration, the GO-coated emitter is integrated into a multifunctional monitoring platform and evaluated for gas detection. The platform exhibits sensitive and highly selective detection toward CO2 at room temperature with a detection limit of 50 ppm and short response/recovery time, outperforming the state-of-the-art gas sensors. This study demonstrates the emission tailorability of thermal emitters and the feasibility of improving the associated gas sensing property, offering perspectives for designing and fabricating high-end optical sensors with cost-effectiveness and superior performance.
first_indexed 2024-10-01T03:14:19Z
format Journal Article
id ntu-10356/138671
institution Nanyang Technological University
language English
last_indexed 2024-10-01T03:14:19Z
publishDate 2020
record_format dspace
spelling ntu-10356/1386712020-05-11T08:44:54Z Radiation enhancement by graphene oxide on microelectromechanical system emitters for highly selective gas sensing Li, Nanxi Yuan, Hongye Xu, Linfang Tao, Jifang Ng, Doris Keh Ting Lee, Lennon Yao Ting Cheam, Daw Don Zeng, Yongquan Qiang, Bo Wang, Qijie Cai, Hong Singh, Navab Zhao, Dan School of Electrical and Electronic Engineering Engineering::Electrical and electronic engineering MEMS Emitters Thermal Emission Infrared gas sensors have been proven promising for broad applications in Internet of Things and Industrial Internet of Things. However, the lack of miniaturized light sources with good compatibility and tunable spectral features hinders their widespread utilization. Herein, a strategy is proposed to increase the radiated power from microelectromechanical-based thermal emitters by coating with graphene oxide (GO). The radiation can be substantially enhanced, which partially stems from the high emissivity of GO coating demonstrated by spectroscopic methods. Moreover, the sp2 structure within GO may induce plasmons and thus couple with photons to produce blackbody radiation and/or new thermal emission sources. As a proof-of-concept demonstration, the GO-coated emitter is integrated into a multifunctional monitoring platform and evaluated for gas detection. The platform exhibits sensitive and highly selective detection toward CO2 at room temperature with a detection limit of 50 ppm and short response/recovery time, outperforming the state-of-the-art gas sensors. This study demonstrates the emission tailorability of thermal emitters and the feasibility of improving the associated gas sensing property, offering perspectives for designing and fabricating high-end optical sensors with cost-effectiveness and superior performance. NRF (Natl Research Foundation, S’pore) ASTAR (Agency for Sci., Tech. and Research, S’pore) Accepted version 2020-05-11T08:44:54Z 2020-05-11T08:44:54Z 2019 Journal Article Li, N., Yuan, H., Xu, L., Tao, J., Ng, D. K. T., Lee, L. Y. T., . . . Zhao, D. (2019). Radiation enhancement by graphene oxide on microelectromechanical system emitters for highly selective gas sensing. ACS Sensors, 4(10), 2746-2753. doi:10.1021/acssensors.9b01275 2379-3694 https://hdl.handle.net/10356/138671 10.1021/acssensors.9b01275 31524375 2-s2.0-85072972600 10 4 2746 2753 en ACS Sensors This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Sensors, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acssensors.9b01275 application/pdf
spellingShingle Engineering::Electrical and electronic engineering
MEMS Emitters
Thermal Emission
Li, Nanxi
Yuan, Hongye
Xu, Linfang
Tao, Jifang
Ng, Doris Keh Ting
Lee, Lennon Yao Ting
Cheam, Daw Don
Zeng, Yongquan
Qiang, Bo
Wang, Qijie
Cai, Hong
Singh, Navab
Zhao, Dan
Radiation enhancement by graphene oxide on microelectromechanical system emitters for highly selective gas sensing
title Radiation enhancement by graphene oxide on microelectromechanical system emitters for highly selective gas sensing
title_full Radiation enhancement by graphene oxide on microelectromechanical system emitters for highly selective gas sensing
title_fullStr Radiation enhancement by graphene oxide on microelectromechanical system emitters for highly selective gas sensing
title_full_unstemmed Radiation enhancement by graphene oxide on microelectromechanical system emitters for highly selective gas sensing
title_short Radiation enhancement by graphene oxide on microelectromechanical system emitters for highly selective gas sensing
title_sort radiation enhancement by graphene oxide on microelectromechanical system emitters for highly selective gas sensing
topic Engineering::Electrical and electronic engineering
MEMS Emitters
Thermal Emission
url https://hdl.handle.net/10356/138671
work_keys_str_mv AT linanxi radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT yuanhongye radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT xulinfang radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT taojifang radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT ngdoriskehting radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT leelennonyaoting radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT cheamdawdon radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT zengyongquan radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT qiangbo radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT wangqijie radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT caihong radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT singhnavab radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing
AT zhaodan radiationenhancementbygrapheneoxideonmicroelectromechanicalsystememittersforhighlyselectivegassensing