Spatially probed plasmonic photothermic nanoheater enhanced hybrid polymeric – metallic PVDF‐Ag nanogenerator

Surface plasmon-based photonics offers exciting opportunities to enable fine control of the site, span, and extent of mechanical harvesting. However, the interaction between plasmonic photothermic and piezoresponse still remains underexplored. Here, spatially localized and controllable piezoresponse...

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Main Authors: Liow, Chi Hao, Lu, Xin, Tan, Chuan Fu, Chan, Kwok Hoe, Zeng, Kaiyang, Li, Shuzhou, Ho, Ghim Wei
Other Authors: School of Materials Science & Engineering
Format: Journal Article
Language:English
Published: 2020
Subjects:
Online Access:https://hdl.handle.net/10356/139247
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author Liow, Chi Hao
Lu, Xin
Tan, Chuan Fu
Chan, Kwok Hoe
Zeng, Kaiyang
Li, Shuzhou
Ho, Ghim Wei
author2 School of Materials Science & Engineering
author_facet School of Materials Science & Engineering
Liow, Chi Hao
Lu, Xin
Tan, Chuan Fu
Chan, Kwok Hoe
Zeng, Kaiyang
Li, Shuzhou
Ho, Ghim Wei
author_sort Liow, Chi Hao
collection NTU
description Surface plasmon-based photonics offers exciting opportunities to enable fine control of the site, span, and extent of mechanical harvesting. However, the interaction between plasmonic photothermic and piezoresponse still remains underexplored. Here, spatially localized and controllable piezoresponse of a hybrid self-polarized polymeric-metallic system that correlates to plasmonic light-to-heat modulation of the local strain is demonstrated. The piezoresponse is associated to the localized plasmons that serve as efficient nanoheaters leading to self-regulated strain via thermal expansion of the electroactive polymer. Moreover, the finite-difference time-domain simulation and linear thermal model also deduce the local strain to the surface plasmon heat absorption. The distinct plasmonic photothermic-piezoelectric phenomenon mediates not only localized external stimulus light response but also enhances dynamic piezoelectric energy harvesting. The present work highlights a promising surface plasmon coordinated piezoelectric response which underpins energy localization and transfer for diversified design of unique photothermic-piezotronic technology.
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spelling ntu-10356/1392472020-06-01T10:26:30Z Spatially probed plasmonic photothermic nanoheater enhanced hybrid polymeric – metallic PVDF‐Ag nanogenerator Liow, Chi Hao Lu, Xin Tan, Chuan Fu Chan, Kwok Hoe Zeng, Kaiyang Li, Shuzhou Ho, Ghim Wei School of Materials Science & Engineering Engineering::Materials Photothermal Piezoelectric Surface plasmon-based photonics offers exciting opportunities to enable fine control of the site, span, and extent of mechanical harvesting. However, the interaction between plasmonic photothermic and piezoresponse still remains underexplored. Here, spatially localized and controllable piezoresponse of a hybrid self-polarized polymeric-metallic system that correlates to plasmonic light-to-heat modulation of the local strain is demonstrated. The piezoresponse is associated to the localized plasmons that serve as efficient nanoheaters leading to self-regulated strain via thermal expansion of the electroactive polymer. Moreover, the finite-difference time-domain simulation and linear thermal model also deduce the local strain to the surface plasmon heat absorption. The distinct plasmonic photothermic-piezoelectric phenomenon mediates not only localized external stimulus light response but also enhances dynamic piezoelectric energy harvesting. The present work highlights a promising surface plasmon coordinated piezoelectric response which underpins energy localization and transfer for diversified design of unique photothermic-piezotronic technology. NRF (Natl Research Foundation, S’pore) 2020-05-18T06:43:16Z 2020-05-18T06:43:16Z 2017 Journal Article Liow, C. H., Lu, X., Tan, C. F., Chan, K. H., Zeng, K., Li, S., & Ho, G. W. (2018). Spatially probed plasmonic photothermic nanoheater enhanced hybrid polymeric – metallic PVDF‐Ag nanogenerator. Small, 14(7), 1702268-. doi:10.1002/smll.201702268 1613-6810 https://hdl.handle.net/10356/139247 10.1002/smll.201702268 29239097 2-s2.0-85037995021 7 14 en Small © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim. All rights reserved.
spellingShingle Engineering::Materials
Photothermal
Piezoelectric
Liow, Chi Hao
Lu, Xin
Tan, Chuan Fu
Chan, Kwok Hoe
Zeng, Kaiyang
Li, Shuzhou
Ho, Ghim Wei
Spatially probed plasmonic photothermic nanoheater enhanced hybrid polymeric – metallic PVDF‐Ag nanogenerator
title Spatially probed plasmonic photothermic nanoheater enhanced hybrid polymeric – metallic PVDF‐Ag nanogenerator
title_full Spatially probed plasmonic photothermic nanoheater enhanced hybrid polymeric – metallic PVDF‐Ag nanogenerator
title_fullStr Spatially probed plasmonic photothermic nanoheater enhanced hybrid polymeric – metallic PVDF‐Ag nanogenerator
title_full_unstemmed Spatially probed plasmonic photothermic nanoheater enhanced hybrid polymeric – metallic PVDF‐Ag nanogenerator
title_short Spatially probed plasmonic photothermic nanoheater enhanced hybrid polymeric – metallic PVDF‐Ag nanogenerator
title_sort spatially probed plasmonic photothermic nanoheater enhanced hybrid polymeric metallic pvdf ag nanogenerator
topic Engineering::Materials
Photothermal
Piezoelectric
url https://hdl.handle.net/10356/139247
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