Storing electricity as chemical energy : beyond traditional electrochemistry and double-layer compression

Extending the range of analysis of previous measurements on energy storage in ionic liquid (IL)-based supercapacitors with very well defined carbon materials indicates that there are two distinct processes at play: the one at lower voltages is (classically) related to the micropore inclusion of sing...

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Main Authors: Antonietti, Markus, Chen, Xiaodong, Yan, Runyu, Oschatz, Martin
Other Authors: School of Materials Science and Engineering
Format: Journal Article
Language:English
Published: 2020
Subjects:
Online Access:https://hdl.handle.net/10356/143839
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author Antonietti, Markus
Chen, Xiaodong
Yan, Runyu
Oschatz, Martin
author2 School of Materials Science and Engineering
author_facet School of Materials Science and Engineering
Antonietti, Markus
Chen, Xiaodong
Yan, Runyu
Oschatz, Martin
author_sort Antonietti, Markus
collection NTU
description Extending the range of analysis of previous measurements on energy storage in ionic liquid (IL)-based supercapacitors with very well defined carbon materials indicates that there are two distinct processes at play: the one at lower voltages is (classically) related to the micropore inclusion of single ions, while a previously unknown high voltage transition can be ascribed to a change in the structure and coordination number of the ionic liquid. This opinion article discusses a proof of circumstantial evidence for this so far weakly understood and often overlooked mode of energy storage, which in principle could take supercapacitors to a new level of energy storage.
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spelling ntu-10356/1438392023-07-14T15:46:18Z Storing electricity as chemical energy : beyond traditional electrochemistry and double-layer compression Antonietti, Markus Chen, Xiaodong Yan, Runyu Oschatz, Martin School of Materials Science and Engineering Engineering::Materials Ionic Liquids Supercapacitor Extending the range of analysis of previous measurements on energy storage in ionic liquid (IL)-based supercapacitors with very well defined carbon materials indicates that there are two distinct processes at play: the one at lower voltages is (classically) related to the micropore inclusion of single ions, while a previously unknown high voltage transition can be ascribed to a change in the structure and coordination number of the ionic liquid. This opinion article discusses a proof of circumstantial evidence for this so far weakly understood and often overlooked mode of energy storage, which in principle could take supercapacitors to a new level of energy storage. Published version 2020-09-25T05:41:17Z 2020-09-25T05:41:17Z 2018 Journal Article Antonietti, M., Chen, X., Yan, R., & Oschatz, M. (2018). Storing electricity as chemical energy : beyond traditional electrochemistry and double-layer compression. Energy & Environmental Science, 11(11), 3069-3074. doi:10.1039/C8EE01723A 1754-5692 https://hdl.handle.net/10356/143839 10.1039/C8EE01723A 11 11 3069 3074 en Energy & Environmental Science © 2018 The Author(s) (published by Royal Society of Chemistry). This is an open-access article distributed under the terms of the Creative Commons Attribution License. application/pdf
spellingShingle Engineering::Materials
Ionic Liquids
Supercapacitor
Antonietti, Markus
Chen, Xiaodong
Yan, Runyu
Oschatz, Martin
Storing electricity as chemical energy : beyond traditional electrochemistry and double-layer compression
title Storing electricity as chemical energy : beyond traditional electrochemistry and double-layer compression
title_full Storing electricity as chemical energy : beyond traditional electrochemistry and double-layer compression
title_fullStr Storing electricity as chemical energy : beyond traditional electrochemistry and double-layer compression
title_full_unstemmed Storing electricity as chemical energy : beyond traditional electrochemistry and double-layer compression
title_short Storing electricity as chemical energy : beyond traditional electrochemistry and double-layer compression
title_sort storing electricity as chemical energy beyond traditional electrochemistry and double layer compression
topic Engineering::Materials
Ionic Liquids
Supercapacitor
url https://hdl.handle.net/10356/143839
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AT chenxiaodong storingelectricityaschemicalenergybeyondtraditionalelectrochemistryanddoublelayercompression
AT yanrunyu storingelectricityaschemicalenergybeyondtraditionalelectrochemistryanddoublelayercompression
AT oschatzmartin storingelectricityaschemicalenergybeyondtraditionalelectrochemistryanddoublelayercompression