Real-time visualization of energy- and momentum-resolved carrier dynamics of spatially heterogeneous materials

Among a variety of methods for studying the ultrafast carrier dynamics in the solid-state materials, time-resolved photoemission electron microscopy (PEEM) has been regarded as a unique tool which can simultaneously achieve the femtosecond time resolution as well as non-diffraction-limited lateral s...

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Main Authors: Woo, Kyung Chul, Xu, Ce, Loh, Zhi-Heng
Other Authors: Asian Spectroscopy Conference 2020
Format: Conference Paper
Language:English
Published: 2020
Subjects:
Online Access:https://hdl.handle.net/10356/144317
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author Woo, Kyung Chul
Xu, Ce
Loh, Zhi-Heng
author2 Asian Spectroscopy Conference 2020
author_facet Asian Spectroscopy Conference 2020
Woo, Kyung Chul
Xu, Ce
Loh, Zhi-Heng
author_sort Woo, Kyung Chul
collection NTU
description Among a variety of methods for studying the ultrafast carrier dynamics in the solid-state materials, time-resolved photoemission electron microscopy (PEEM) has been regarded as a unique tool which can simultaneously achieve the femtosecond time resolution as well as non-diffraction-limited lateral spatial resolution, hence providing spatiotemporally resolved information on surfaces with structural heterogeneities [1]. When combined with an electron time-of-flight analyzer in the form of a delay-line detector [2], PEEM can be further extended to provide spectroscopic information. The consequent energy-resolved momentum-space images acquired at selected microscopic regions can be mapped, hence permitting the real-time visualization of the evolving photorelaxation dynamics of the band structure of solid-state materials. Here, preliminary spectromicroscopic results obtained from the time-resolved PEEM setup will be presented, and further on-going efforts to build a femtosecond megahertz-repetition-rate extreme ultraviolet radiation source will be introduced.
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spelling ntu-10356/1443172020-10-29T20:11:13Z Real-time visualization of energy- and momentum-resolved carrier dynamics of spatially heterogeneous materials Woo, Kyung Chul Xu, Ce Loh, Zhi-Heng Asian Spectroscopy Conference 2020 Institute of Advanced Studies Science::Chemistry Photoemission Electron Microscopy Ultrafast Carrier Dynamics Among a variety of methods for studying the ultrafast carrier dynamics in the solid-state materials, time-resolved photoemission electron microscopy (PEEM) has been regarded as a unique tool which can simultaneously achieve the femtosecond time resolution as well as non-diffraction-limited lateral spatial resolution, hence providing spatiotemporally resolved information on surfaces with structural heterogeneities [1]. When combined with an electron time-of-flight analyzer in the form of a delay-line detector [2], PEEM can be further extended to provide spectroscopic information. The consequent energy-resolved momentum-space images acquired at selected microscopic regions can be mapped, hence permitting the real-time visualization of the evolving photorelaxation dynamics of the band structure of solid-state materials. Here, preliminary spectromicroscopic results obtained from the time-resolved PEEM setup will be presented, and further on-going efforts to build a femtosecond megahertz-repetition-rate extreme ultraviolet radiation source will be introduced. Published version 2020-10-28T03:53:49Z 2020-10-28T03:53:49Z 2020 Conference Paper Woo, K. C., Xu, C., & Loh, Z.-H. (2020). Real-time visualization of energy- and momentum-resolved carrier dynamics of spatially heterogeneous materials. Proc. Of the 7th Asian Spectroscopy Conference (ASC 2020). doi:10.32655/ASC_8-10_Dec2020.55 https://hdl.handle.net/10356/144317 10.32655/ASC_8-10_Dec2020.55 en © 2020 Nanyang Technological University. application/pdf
spellingShingle Science::Chemistry
Photoemission Electron Microscopy
Ultrafast Carrier Dynamics
Woo, Kyung Chul
Xu, Ce
Loh, Zhi-Heng
Real-time visualization of energy- and momentum-resolved carrier dynamics of spatially heterogeneous materials
title Real-time visualization of energy- and momentum-resolved carrier dynamics of spatially heterogeneous materials
title_full Real-time visualization of energy- and momentum-resolved carrier dynamics of spatially heterogeneous materials
title_fullStr Real-time visualization of energy- and momentum-resolved carrier dynamics of spatially heterogeneous materials
title_full_unstemmed Real-time visualization of energy- and momentum-resolved carrier dynamics of spatially heterogeneous materials
title_short Real-time visualization of energy- and momentum-resolved carrier dynamics of spatially heterogeneous materials
title_sort real time visualization of energy and momentum resolved carrier dynamics of spatially heterogeneous materials
topic Science::Chemistry
Photoemission Electron Microscopy
Ultrafast Carrier Dynamics
url https://hdl.handle.net/10356/144317
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