Temperature dependent spectroscopic studies of all-inorganic lead halide perovskites : towards efficient and stable optoelectronic applications

Lead halide perovskites have attracted enormous interest for their excellent optoelectronic properties like the long carrier diffusion length, high quantum yield, bipolar charge carrier transport, high absorption coefficient, convenient spectral turnability, etc. They are promising candidates for ne...

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Main Author: Chen, Xiaoxuan
Other Authors: Sun Handong
Format: Thesis-Doctor of Philosophy
Language:English
Published: Nanyang Technological University 2021
Subjects:
Online Access:https://hdl.handle.net/10356/146946
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author Chen, Xiaoxuan
author2 Sun Handong
author_facet Sun Handong
Chen, Xiaoxuan
author_sort Chen, Xiaoxuan
collection NTU
description Lead halide perovskites have attracted enormous interest for their excellent optoelectronic properties like the long carrier diffusion length, high quantum yield, bipolar charge carrier transport, high absorption coefficient, convenient spectral turnability, etc. They are promising candidates for next-generation solar cells, optically pumped lasers, light-emitting diodes, and photodetectors. However, the most widely studied organic-inorganic hybrid lead halide perovskites suffer from instability during shelf storage as well as under operation conditions. All-inorganic perovskites are alternatives that present better stability and competitive performance. With the impetus to delve into this less-explored material system and accelerate the development of all-inorganic lead halide perovskites towards optoelectronics with high efficiency and stability, I have carried out systematic spectroscopic studies with temperature assessment.
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spelling ntu-10356/1469462023-02-28T23:38:20Z Temperature dependent spectroscopic studies of all-inorganic lead halide perovskites : towards efficient and stable optoelectronic applications Chen, Xiaoxuan Sun Handong School of Physical and Mathematical Sciences HDSun@ntu.edu.sg Science::Physics::Optics and light Lead halide perovskites have attracted enormous interest for their excellent optoelectronic properties like the long carrier diffusion length, high quantum yield, bipolar charge carrier transport, high absorption coefficient, convenient spectral turnability, etc. They are promising candidates for next-generation solar cells, optically pumped lasers, light-emitting diodes, and photodetectors. However, the most widely studied organic-inorganic hybrid lead halide perovskites suffer from instability during shelf storage as well as under operation conditions. All-inorganic perovskites are alternatives that present better stability and competitive performance. With the impetus to delve into this less-explored material system and accelerate the development of all-inorganic lead halide perovskites towards optoelectronics with high efficiency and stability, I have carried out systematic spectroscopic studies with temperature assessment. Doctor of Philosophy 2021-03-15T13:05:04Z 2021-03-15T13:05:04Z 2021 Thesis-Doctor of Philosophy Chen, X. (2021). Temperature dependent spectroscopic studies of all-inorganic lead halide perovskites : towards efficient and stable optoelectronic applications. Doctoral thesis, Nanyang Technological University, Singapore. https://hdl.handle.net/10356/146946 https://hdl.handle.net/10356/146946 10.32657/10356/146946 en This work is licensed under a Creative Commons Attribution-NonCommercial 4.0 International License (CC BY-NC 4.0). application/pdf Nanyang Technological University
spellingShingle Science::Physics::Optics and light
Chen, Xiaoxuan
Temperature dependent spectroscopic studies of all-inorganic lead halide perovskites : towards efficient and stable optoelectronic applications
title Temperature dependent spectroscopic studies of all-inorganic lead halide perovskites : towards efficient and stable optoelectronic applications
title_full Temperature dependent spectroscopic studies of all-inorganic lead halide perovskites : towards efficient and stable optoelectronic applications
title_fullStr Temperature dependent spectroscopic studies of all-inorganic lead halide perovskites : towards efficient and stable optoelectronic applications
title_full_unstemmed Temperature dependent spectroscopic studies of all-inorganic lead halide perovskites : towards efficient and stable optoelectronic applications
title_short Temperature dependent spectroscopic studies of all-inorganic lead halide perovskites : towards efficient and stable optoelectronic applications
title_sort temperature dependent spectroscopic studies of all inorganic lead halide perovskites towards efficient and stable optoelectronic applications
topic Science::Physics::Optics and light
url https://hdl.handle.net/10356/146946
work_keys_str_mv AT chenxiaoxuan temperaturedependentspectroscopicstudiesofallinorganicleadhalideperovskitestowardsefficientandstableoptoelectronicapplications