Interpenetrating PAA-PEDOT conductive hydrogels for flexible skin sensors

Conductive hydrogels are promising material candidates in artificial skin and muscles, flexible and implantable bioelectronics, and tissue engineering. However, it is still a challenge to formulate hydrogels with high electrical conductivity without compromising their physicochemical properties. Her...

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Main Authors: Fu, Fanfan, Wang, Jilei, Yu, Jing
Other Authors: School of Materials Science and Engineering
Format: Journal Article
Language:English
Published: 2022
Subjects:
Online Access:https://hdl.handle.net/10356/156081
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author Fu, Fanfan
Wang, Jilei
Yu, Jing
author2 School of Materials Science and Engineering
author_facet School of Materials Science and Engineering
Fu, Fanfan
Wang, Jilei
Yu, Jing
author_sort Fu, Fanfan
collection NTU
description Conductive hydrogels are promising material candidates in artificial skin and muscles, flexible and implantable bioelectronics, and tissue engineering. However, it is still a challenge to formulate hydrogels with high electrical conductivity without compromising their physicochemical properties. Herein, we report an interpenetrating poly(acrylic acid)-poly (3,4-ethylenedioxythiophene) (PAA-PEDOT) hydrogel with high electrical conductivity and good stretchability. A second PEDOT hydrogel network is electrochemically polymerized into an existing PAA hydrogel network. The interpenetrating hydrogel can be readily prepared and can be integrated into epidermal flexible electronic devices for the real-time, on-body detection of various ions in sweat. The interpenetrating PAA-PEDOT conductive hydrogel has the potential to be an important building material for various flexible electronic devices for personalized healthcare.
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spelling ntu-10356/1560812023-07-14T16:04:59Z Interpenetrating PAA-PEDOT conductive hydrogels for flexible skin sensors Fu, Fanfan Wang, Jilei Yu, Jing School of Materials Science and Engineering Engineering::Materials Electric Conductivity Hydrogels Conductive hydrogels are promising material candidates in artificial skin and muscles, flexible and implantable bioelectronics, and tissue engineering. However, it is still a challenge to formulate hydrogels with high electrical conductivity without compromising their physicochemical properties. Herein, we report an interpenetrating poly(acrylic acid)-poly (3,4-ethylenedioxythiophene) (PAA-PEDOT) hydrogel with high electrical conductivity and good stretchability. A second PEDOT hydrogel network is electrochemically polymerized into an existing PAA hydrogel network. The interpenetrating hydrogel can be readily prepared and can be integrated into epidermal flexible electronic devices for the real-time, on-body detection of various ions in sweat. The interpenetrating PAA-PEDOT conductive hydrogel has the potential to be an important building material for various flexible electronic devices for personalized healthcare. Ministry of Education (MOE) Submitted/Accepted version F. F. Fu, J. L. Wang and J. Yu acknowledge the AME Programmatic Funding Scheme of Cyber Physiochemical Interfaces (CPI) project (#A18A1b0045) and the Singapore Ministry of Education Academic Research Fund Tier 1 (RT 06/20). 2022-04-05T06:29:33Z 2022-04-05T06:29:33Z 2021 Journal Article Fu, F., Wang, J. & Yu, J. (2021). Interpenetrating PAA-PEDOT conductive hydrogels for flexible skin sensors. Journal of Materials Chemistry C, 9(35), 11794-11800. https://dx.doi.org/10.1039/D1TC01578H 2050-7526 https://hdl.handle.net/10356/156081 10.1039/D1TC01578H 35 9 11794 11800 en #A18A1b0045 RT 06/20 Journal of Materials Chemistry C © 2021 The Royal Society of Chemistry. All rights reserved. This paper was published in Journal of Materials Chemistry C and is made available with permission of The Royal Society of Chemistry. application/pdf
spellingShingle Engineering::Materials
Electric Conductivity
Hydrogels
Fu, Fanfan
Wang, Jilei
Yu, Jing
Interpenetrating PAA-PEDOT conductive hydrogels for flexible skin sensors
title Interpenetrating PAA-PEDOT conductive hydrogels for flexible skin sensors
title_full Interpenetrating PAA-PEDOT conductive hydrogels for flexible skin sensors
title_fullStr Interpenetrating PAA-PEDOT conductive hydrogels for flexible skin sensors
title_full_unstemmed Interpenetrating PAA-PEDOT conductive hydrogels for flexible skin sensors
title_short Interpenetrating PAA-PEDOT conductive hydrogels for flexible skin sensors
title_sort interpenetrating paa pedot conductive hydrogels for flexible skin sensors
topic Engineering::Materials
Electric Conductivity
Hydrogels
url https://hdl.handle.net/10356/156081
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AT wangjilei interpenetratingpaapedotconductivehydrogelsforflexibleskinsensors
AT yujing interpenetratingpaapedotconductivehydrogelsforflexibleskinsensors