Thermally induced continuous water flow in long nanotube channels

Despite its importance for nanofluidic systems, achieving continuous water flow in long nanochannels remains a major challenge. Here, we propose a general principle to overcome this challenge by introducing a method that involves the building of a series of cascadable driving units, each unit carryi...

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Автори: Leng, Jiantao, Ying, Tianquan, Guo, Zhengrong, Zhang, Yingyan, Chang, Tienchong, Guo, Wanlin, Gao, Huajian
Інші автори: School of Mechanical and Aerospace Engineering
Формат: Journal Article
Мова:English
Опубліковано: 2022
Предмети:
Онлайн доступ:https://hdl.handle.net/10356/163623
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author Leng, Jiantao
Ying, Tianquan
Guo, Zhengrong
Zhang, Yingyan
Chang, Tienchong
Guo, Wanlin
Gao, Huajian
author2 School of Mechanical and Aerospace Engineering
author_facet School of Mechanical and Aerospace Engineering
Leng, Jiantao
Ying, Tianquan
Guo, Zhengrong
Zhang, Yingyan
Chang, Tienchong
Guo, Wanlin
Gao, Huajian
author_sort Leng, Jiantao
collection NTU
description Despite its importance for nanofluidic systems, achieving continuous water flow in long nanochannels remains a major challenge. Here, we propose a general principle to overcome this challenge by introducing a method that involves the building of a series of cascadable driving units, each unit carrying a net thermal gradient force, to maintain continuous water flow in an arbitrarily long nanochannel. Using molecular dynamics simulations and analytical modeling, we show that, within a single driving unit, the net thermal gradient force can be achieved through a multitude of strategies, including geometrical (e.g., a localized confinement), mechanical (e.g., a localized pinch), electrical (e.g., a point electric charge) and chemical (e.g., a point functionalization). The proposed method has fundamental significance for nanofluidic systems and potential applications in nanoscale mass transport and energy conversion devices.
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spelling ntu-10356/1636232022-12-13T01:22:27Z Thermally induced continuous water flow in long nanotube channels Leng, Jiantao Ying, Tianquan Guo, Zhengrong Zhang, Yingyan Chang, Tienchong Guo, Wanlin Gao, Huajian School of Mechanical and Aerospace Engineering Institute of High-Performance Computing, A*STAR Engineering::Mechanical engineering Continuous Water Flow Carbon Nanotube Despite its importance for nanofluidic systems, achieving continuous water flow in long nanochannels remains a major challenge. Here, we propose a general principle to overcome this challenge by introducing a method that involves the building of a series of cascadable driving units, each unit carrying a net thermal gradient force, to maintain continuous water flow in an arbitrarily long nanochannel. Using molecular dynamics simulations and analytical modeling, we show that, within a single driving unit, the net thermal gradient force can be achieved through a multitude of strategies, including geometrical (e.g., a localized confinement), mechanical (e.g., a localized pinch), electrical (e.g., a point electric charge) and chemical (e.g., a point functionalization). The proposed method has fundamental significance for nanofluidic systems and potential applications in nanoscale mass transport and energy conversion devices. Agency for Science, Technology and Research (A*STAR) Nanyang Technological University T.C. acknowledges financial support from the NSF of China (Grant Nos. 12132008, 11872238), the Innovation Program of Shanghai Municipal Education Commission (No. 2017-01-07-00-09-E00019), the Program of Shanghai Academic Research Leader (19XD1401500), and the Key Research Project of Zhejiang Lab (2021PE0AC02). H.G. acknowledges a research start-up grant (002479-00001) from Nanyang Technological University and the Agency for Science, Technology and Research (A*STAR). 2022-12-13T01:22:27Z 2022-12-13T01:22:27Z 2022 Journal Article Leng, J., Ying, T., Guo, Z., Zhang, Y., Chang, T., Guo, W. & Gao, H. (2022). Thermally induced continuous water flow in long nanotube channels. Carbon, 191, 175-182. https://dx.doi.org/10.1016/j.carbon.2022.01.049 0008-6223 https://hdl.handle.net/10356/163623 10.1016/j.carbon.2022.01.049 2-s2.0-85123887666 191 175 182 en 002479-00001 Carbon © 2022 Elsevier Ltd. All rights reserved.
spellingShingle Engineering::Mechanical engineering
Continuous Water Flow
Carbon Nanotube
Leng, Jiantao
Ying, Tianquan
Guo, Zhengrong
Zhang, Yingyan
Chang, Tienchong
Guo, Wanlin
Gao, Huajian
Thermally induced continuous water flow in long nanotube channels
title Thermally induced continuous water flow in long nanotube channels
title_full Thermally induced continuous water flow in long nanotube channels
title_fullStr Thermally induced continuous water flow in long nanotube channels
title_full_unstemmed Thermally induced continuous water flow in long nanotube channels
title_short Thermally induced continuous water flow in long nanotube channels
title_sort thermally induced continuous water flow in long nanotube channels
topic Engineering::Mechanical engineering
Continuous Water Flow
Carbon Nanotube
url https://hdl.handle.net/10356/163623
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AT yingtianquan thermallyinducedcontinuouswaterflowinlongnanotubechannels
AT guozhengrong thermallyinducedcontinuouswaterflowinlongnanotubechannels
AT zhangyingyan thermallyinducedcontinuouswaterflowinlongnanotubechannels
AT changtienchong thermallyinducedcontinuouswaterflowinlongnanotubechannels
AT guowanlin thermallyinducedcontinuouswaterflowinlongnanotubechannels
AT gaohuajian thermallyinducedcontinuouswaterflowinlongnanotubechannels