Thermally induced continuous water flow in long nanotube channels
Despite its importance for nanofluidic systems, achieving continuous water flow in long nanochannels remains a major challenge. Here, we propose a general principle to overcome this challenge by introducing a method that involves the building of a series of cascadable driving units, each unit carryi...
Автори: | , , , , , , |
---|---|
Інші автори: | |
Формат: | Journal Article |
Мова: | English |
Опубліковано: |
2022
|
Предмети: | |
Онлайн доступ: | https://hdl.handle.net/10356/163623 |
_version_ | 1826120853588279296 |
---|---|
author | Leng, Jiantao Ying, Tianquan Guo, Zhengrong Zhang, Yingyan Chang, Tienchong Guo, Wanlin Gao, Huajian |
author2 | School of Mechanical and Aerospace Engineering |
author_facet | School of Mechanical and Aerospace Engineering Leng, Jiantao Ying, Tianquan Guo, Zhengrong Zhang, Yingyan Chang, Tienchong Guo, Wanlin Gao, Huajian |
author_sort | Leng, Jiantao |
collection | NTU |
description | Despite its importance for nanofluidic systems, achieving continuous water flow in long nanochannels remains a major challenge. Here, we propose a general principle to overcome this challenge by introducing a method that involves the building of a series of cascadable driving units, each unit carrying a net thermal gradient force, to maintain continuous water flow in an arbitrarily long nanochannel. Using molecular dynamics simulations and analytical modeling, we show that, within a single driving unit, the net thermal gradient force can be achieved through a multitude of strategies, including geometrical (e.g., a localized confinement), mechanical (e.g., a localized pinch), electrical (e.g., a point electric charge) and chemical (e.g., a point functionalization). The proposed method has fundamental significance for nanofluidic systems and potential applications in nanoscale mass transport and energy conversion devices. |
first_indexed | 2024-10-01T05:23:15Z |
format | Journal Article |
id | ntu-10356/163623 |
institution | Nanyang Technological University |
language | English |
last_indexed | 2024-10-01T05:23:15Z |
publishDate | 2022 |
record_format | dspace |
spelling | ntu-10356/1636232022-12-13T01:22:27Z Thermally induced continuous water flow in long nanotube channels Leng, Jiantao Ying, Tianquan Guo, Zhengrong Zhang, Yingyan Chang, Tienchong Guo, Wanlin Gao, Huajian School of Mechanical and Aerospace Engineering Institute of High-Performance Computing, A*STAR Engineering::Mechanical engineering Continuous Water Flow Carbon Nanotube Despite its importance for nanofluidic systems, achieving continuous water flow in long nanochannels remains a major challenge. Here, we propose a general principle to overcome this challenge by introducing a method that involves the building of a series of cascadable driving units, each unit carrying a net thermal gradient force, to maintain continuous water flow in an arbitrarily long nanochannel. Using molecular dynamics simulations and analytical modeling, we show that, within a single driving unit, the net thermal gradient force can be achieved through a multitude of strategies, including geometrical (e.g., a localized confinement), mechanical (e.g., a localized pinch), electrical (e.g., a point electric charge) and chemical (e.g., a point functionalization). The proposed method has fundamental significance for nanofluidic systems and potential applications in nanoscale mass transport and energy conversion devices. Agency for Science, Technology and Research (A*STAR) Nanyang Technological University T.C. acknowledges financial support from the NSF of China (Grant Nos. 12132008, 11872238), the Innovation Program of Shanghai Municipal Education Commission (No. 2017-01-07-00-09-E00019), the Program of Shanghai Academic Research Leader (19XD1401500), and the Key Research Project of Zhejiang Lab (2021PE0AC02). H.G. acknowledges a research start-up grant (002479-00001) from Nanyang Technological University and the Agency for Science, Technology and Research (A*STAR). 2022-12-13T01:22:27Z 2022-12-13T01:22:27Z 2022 Journal Article Leng, J., Ying, T., Guo, Z., Zhang, Y., Chang, T., Guo, W. & Gao, H. (2022). Thermally induced continuous water flow in long nanotube channels. Carbon, 191, 175-182. https://dx.doi.org/10.1016/j.carbon.2022.01.049 0008-6223 https://hdl.handle.net/10356/163623 10.1016/j.carbon.2022.01.049 2-s2.0-85123887666 191 175 182 en 002479-00001 Carbon © 2022 Elsevier Ltd. All rights reserved. |
spellingShingle | Engineering::Mechanical engineering Continuous Water Flow Carbon Nanotube Leng, Jiantao Ying, Tianquan Guo, Zhengrong Zhang, Yingyan Chang, Tienchong Guo, Wanlin Gao, Huajian Thermally induced continuous water flow in long nanotube channels |
title | Thermally induced continuous water flow in long nanotube channels |
title_full | Thermally induced continuous water flow in long nanotube channels |
title_fullStr | Thermally induced continuous water flow in long nanotube channels |
title_full_unstemmed | Thermally induced continuous water flow in long nanotube channels |
title_short | Thermally induced continuous water flow in long nanotube channels |
title_sort | thermally induced continuous water flow in long nanotube channels |
topic | Engineering::Mechanical engineering Continuous Water Flow Carbon Nanotube |
url | https://hdl.handle.net/10356/163623 |
work_keys_str_mv | AT lengjiantao thermallyinducedcontinuouswaterflowinlongnanotubechannels AT yingtianquan thermallyinducedcontinuouswaterflowinlongnanotubechannels AT guozhengrong thermallyinducedcontinuouswaterflowinlongnanotubechannels AT zhangyingyan thermallyinducedcontinuouswaterflowinlongnanotubechannels AT changtienchong thermallyinducedcontinuouswaterflowinlongnanotubechannels AT guowanlin thermallyinducedcontinuouswaterflowinlongnanotubechannels AT gaohuajian thermallyinducedcontinuouswaterflowinlongnanotubechannels |