Covalent organic frameworks for energy conversion in photocatalysis
Intensifying energy crises and severe environmental issues have led to the discovery of renewable energy sources, sustainable energy conversion, and storage technologies. Photocatalysis is a green technology that converts eco-friendly solar energy into high-energy chemicals. Covalent organic framewo...
| Main Authors: | , |
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| Other Authors: | |
| Format: | Journal Article |
| Language: | English |
| Published: |
2023
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| Subjects: | |
| Online Access: | https://hdl.handle.net/10356/170304 |
| _version_ | 1811690276417175552 |
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| author | He, Ting Zhao, Yanli |
| author2 | School of Chemistry, Chemical Engineering and Biotechnology |
| author_facet | School of Chemistry, Chemical Engineering and Biotechnology He, Ting Zhao, Yanli |
| author_sort | He, Ting |
| collection | NTU |
| description | Intensifying energy crises and severe environmental issues have led to the discovery of renewable energy sources, sustainable energy conversion, and storage technologies. Photocatalysis is a green technology that converts eco-friendly solar energy into high-energy chemicals. Covalent organic frameworks (COFs) are porous materials constructed by covalent bonds that show promising potential for converting solar energy into chemicals owing to their pre-designable structures, high crystallinity, and porosity. Herein, we highlight recent progress in the synthesis of COF-based photocatalysts and their applications in water splitting, CO2 reduction, and H2 O2 production. The challenges and future opportunities for the rational design of COFs for advanced photocatalysts are discussed. This Review is expected to promote further development of COFs toward photocatalysis. |
| first_indexed | 2024-10-01T06:01:25Z |
| format | Journal Article |
| id | ntu-10356/170304 |
| institution | Nanyang Technological University |
| language | English |
| last_indexed | 2024-10-01T06:01:25Z |
| publishDate | 2023 |
| record_format | dspace |
| spelling | ntu-10356/1703042023-09-06T03:56:04Z Covalent organic frameworks for energy conversion in photocatalysis He, Ting Zhao, Yanli School of Chemistry, Chemical Engineering and Biotechnology Engineering::Chemical engineering Photocatalysis CO2 Reduction Intensifying energy crises and severe environmental issues have led to the discovery of renewable energy sources, sustainable energy conversion, and storage technologies. Photocatalysis is a green technology that converts eco-friendly solar energy into high-energy chemicals. Covalent organic frameworks (COFs) are porous materials constructed by covalent bonds that show promising potential for converting solar energy into chemicals owing to their pre-designable structures, high crystallinity, and porosity. Herein, we highlight recent progress in the synthesis of COF-based photocatalysts and their applications in water splitting, CO2 reduction, and H2 O2 production. The challenges and future opportunities for the rational design of COFs for advanced photocatalysts are discussed. This Review is expected to promote further development of COFs toward photocatalysis. Agency for Science, Technology and Research (A*STAR) Ministry of Education (MOE) Y.Z. thanks the Ministry of Education, Singapore, under its Academic Research Funds (RG85/22, RG3/21 and MOET2EP10120‐0003) and the Singapore Agency for Science, Technology, and Research (A*STAR) under the Manufacturing, Trade, and Connectivity Individual Research Grant (M21K2c0105). 2023-09-06T03:56:04Z 2023-09-06T03:56:04Z 2023 Journal Article He, T. & Zhao, Y. (2023). Covalent organic frameworks for energy conversion in photocatalysis. Angewandte Chemie International Edition, 62(34), e202303086-. https://dx.doi.org/10.1002/anie.202303086 1433-7851 https://hdl.handle.net/10356/170304 10.1002/anie.202303086 37093128 2-s2.0-85159266871 34 62 e202303086 en M21K2c0105 MOE-T2EP10120-0003 RG85/22 RG3/21 Angewandte Chemie International Edition © 2023 Wiley-VCH GmbH. All rights reserved. |
| spellingShingle | Engineering::Chemical engineering Photocatalysis CO2 Reduction He, Ting Zhao, Yanli Covalent organic frameworks for energy conversion in photocatalysis |
| title | Covalent organic frameworks for energy conversion in photocatalysis |
| title_full | Covalent organic frameworks for energy conversion in photocatalysis |
| title_fullStr | Covalent organic frameworks for energy conversion in photocatalysis |
| title_full_unstemmed | Covalent organic frameworks for energy conversion in photocatalysis |
| title_short | Covalent organic frameworks for energy conversion in photocatalysis |
| title_sort | covalent organic frameworks for energy conversion in photocatalysis |
| topic | Engineering::Chemical engineering Photocatalysis CO2 Reduction |
| url | https://hdl.handle.net/10356/170304 |
| work_keys_str_mv | AT heting covalentorganicframeworksforenergyconversioninphotocatalysis AT zhaoyanli covalentorganicframeworksforenergyconversioninphotocatalysis |