Recent advances of sustainable short-chain length polyhydroxyalkanoates (Scl-PHAs) – plant biomass composites

Plastic pollution has become a global threat to humanity. Fortunately, humanity has always found ways of overcoming such threats through multipronged approaches. To overcome this current threat brought about by anthropogenic linear pattern of take-make-use-dispose of fossil-based plastics, an intent...

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Main Authors: Muiruri, Joseph Kinyanjui, Yeo, Jayven Chee Chuan, Soo, Debbie Xiang Yun, Wang, Suxi, Liu, Hongfei, Kong, Junhua, Cao, Jing, Tan, Beng Hoon, Suwardi, Ady, Li, Zibiao, Xu, Jianwei, Loh, Xian Jun, Zhu, Qiang
其他作者: School of Chemistry, Chemical Engineering and Biotechnology
格式: Journal Article
语言:English
出版: 2023
主题:
在线阅读:https://hdl.handle.net/10356/170663
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author Muiruri, Joseph Kinyanjui
Yeo, Jayven Chee Chuan
Soo, Debbie Xiang Yun
Wang, Suxi
Liu, Hongfei
Kong, Junhua
Cao, Jing
Tan, Beng Hoon
Suwardi, Ady
Li, Zibiao
Xu, Jianwei
Loh, Xian Jun
Zhu, Qiang
author2 School of Chemistry, Chemical Engineering and Biotechnology
author_facet School of Chemistry, Chemical Engineering and Biotechnology
Muiruri, Joseph Kinyanjui
Yeo, Jayven Chee Chuan
Soo, Debbie Xiang Yun
Wang, Suxi
Liu, Hongfei
Kong, Junhua
Cao, Jing
Tan, Beng Hoon
Suwardi, Ady
Li, Zibiao
Xu, Jianwei
Loh, Xian Jun
Zhu, Qiang
author_sort Muiruri, Joseph Kinyanjui
collection NTU
description Plastic pollution has become a global threat to humanity. Fortunately, humanity has always found ways of overcoming such threats through multipronged approaches. To overcome this current threat brought about by anthropogenic linear pattern of take-make-use-dispose of fossil-based plastics, an intentional approach of adopting biobased plastics which are renewable has taken shape. In this approach, governments, industry, and academia are at the forefront of making determined commitments to slow down the spiralling carbon footprint and aim at net zero carbon emissions by 2050. In this regard, PHAs which have a rich resume of desired properties to replace non-renewable fossil-based plastics are increasingly becoming popular. However, PHA production cost is still high compared with the fossil-based plastics and there exists properties performance gap because they are typically brittle, especially the short chain length PHAs (Scl-PHAs). Considerable efforts are geared towards tuning the mechanical properties as well as reducing the cost to meet the market requirements. The most authentic way of tackling these twin-challenges of reducing the cost of PHA products and their properties enhancement is the incorporation of fillers sourced from renewable sources, especially the plant biomass. In this comprehensive review, Scl-PHAs biopolymers are discussed, their modifications with plant biomass (natural fibres and components, agro-residues, and industrial residues) are elucidated. Moreover, their wide scope of applications, sustainability performance (biodegradation studies) and other viable end-of-life options are amply discussed. Finally, we draw conclusions and highlight future opportunities in this exciting bioplastic area.
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spelling ntu-10356/1706632023-09-25T06:29:28Z Recent advances of sustainable short-chain length polyhydroxyalkanoates (Scl-PHAs) – plant biomass composites Muiruri, Joseph Kinyanjui Yeo, Jayven Chee Chuan Soo, Debbie Xiang Yun Wang, Suxi Liu, Hongfei Kong, Junhua Cao, Jing Tan, Beng Hoon Suwardi, Ady Li, Zibiao Xu, Jianwei Loh, Xian Jun Zhu, Qiang School of Chemistry, Chemical Engineering and Biotechnology Institute of Sustainability for Chemicals, Energy and Environment (ISCE2), A*STAR Institute of Materials Research and Engineering (IMRE), A*STAR Engineering::Chemical engineering Biomass Polyhydroxyalkanoate Plastic pollution has become a global threat to humanity. Fortunately, humanity has always found ways of overcoming such threats through multipronged approaches. To overcome this current threat brought about by anthropogenic linear pattern of take-make-use-dispose of fossil-based plastics, an intentional approach of adopting biobased plastics which are renewable has taken shape. In this approach, governments, industry, and academia are at the forefront of making determined commitments to slow down the spiralling carbon footprint and aim at net zero carbon emissions by 2050. In this regard, PHAs which have a rich resume of desired properties to replace non-renewable fossil-based plastics are increasingly becoming popular. However, PHA production cost is still high compared with the fossil-based plastics and there exists properties performance gap because they are typically brittle, especially the short chain length PHAs (Scl-PHAs). Considerable efforts are geared towards tuning the mechanical properties as well as reducing the cost to meet the market requirements. The most authentic way of tackling these twin-challenges of reducing the cost of PHA products and their properties enhancement is the incorporation of fillers sourced from renewable sources, especially the plant biomass. In this comprehensive review, Scl-PHAs biopolymers are discussed, their modifications with plant biomass (natural fibres and components, agro-residues, and industrial residues) are elucidated. Moreover, their wide scope of applications, sustainability performance (biodegradation studies) and other viable end-of-life options are amply discussed. Finally, we draw conclusions and highlight future opportunities in this exciting bioplastic area. Agency for Science, Technology and Research (A*STAR) The authors acknowledge financial support from A* STAR ’s Science and Engineering Research Council (Grant Reference No.: GAP/2019/00314). 2023-09-25T06:29:28Z 2023-09-25T06:29:28Z 2023 Journal Article Muiruri, J. K., Yeo, J. C. C., Soo, D. X. Y., Wang, S., Liu, H., Kong, J., Cao, J., Tan, B. H., Suwardi, A., Li, Z., Xu, J., Loh, X. J. & Zhu, Q. (2023). Recent advances of sustainable short-chain length polyhydroxyalkanoates (Scl-PHAs) – plant biomass composites. European Polymer Journal, 187, 111882-. https://dx.doi.org/10.1016/j.eurpolymj.2023.111882 0014-3057 https://hdl.handle.net/10356/170663 10.1016/j.eurpolymj.2023.111882 2-s2.0-85148014133 187 111882 en GAP/2019/00314 European Polymer Journal © 2023 Elsevier Ltd. All rights reserved.
spellingShingle Engineering::Chemical engineering
Biomass
Polyhydroxyalkanoate
Muiruri, Joseph Kinyanjui
Yeo, Jayven Chee Chuan
Soo, Debbie Xiang Yun
Wang, Suxi
Liu, Hongfei
Kong, Junhua
Cao, Jing
Tan, Beng Hoon
Suwardi, Ady
Li, Zibiao
Xu, Jianwei
Loh, Xian Jun
Zhu, Qiang
Recent advances of sustainable short-chain length polyhydroxyalkanoates (Scl-PHAs) – plant biomass composites
title Recent advances of sustainable short-chain length polyhydroxyalkanoates (Scl-PHAs) – plant biomass composites
title_full Recent advances of sustainable short-chain length polyhydroxyalkanoates (Scl-PHAs) – plant biomass composites
title_fullStr Recent advances of sustainable short-chain length polyhydroxyalkanoates (Scl-PHAs) – plant biomass composites
title_full_unstemmed Recent advances of sustainable short-chain length polyhydroxyalkanoates (Scl-PHAs) – plant biomass composites
title_short Recent advances of sustainable short-chain length polyhydroxyalkanoates (Scl-PHAs) – plant biomass composites
title_sort recent advances of sustainable short chain length polyhydroxyalkanoates scl phas plant biomass composites
topic Engineering::Chemical engineering
Biomass
Polyhydroxyalkanoate
url https://hdl.handle.net/10356/170663
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