Versatile MXenes for aqueous zinc batteries

Aqueous zinc-ion batteries (AZIBs) are gaining popularity for their cost-effectiveness, safety, and utilization of abundant resources. MXenes, which possess outstanding conductivity, controllable surface chemistry, and structural adaptability, are widely recognized as a highly versatile platform for...

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Main Authors: Liu, Huan, Xin, Zijun, Cao, Bin, Zhang, Bao, Fan, Hong Jin, Guo, Shaojun
Other Authors: School of Physical and Mathematical Sciences
Format: Journal Article
Language:English
Published: 2024
Subjects:
Online Access:https://hdl.handle.net/10356/173956
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author Liu, Huan
Xin, Zijun
Cao, Bin
Zhang, Bao
Fan, Hong Jin
Guo, Shaojun
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Liu, Huan
Xin, Zijun
Cao, Bin
Zhang, Bao
Fan, Hong Jin
Guo, Shaojun
author_sort Liu, Huan
collection NTU
description Aqueous zinc-ion batteries (AZIBs) are gaining popularity for their cost-effectiveness, safety, and utilization of abundant resources. MXenes, which possess outstanding conductivity, controllable surface chemistry, and structural adaptability, are widely recognized as a highly versatile platform for AZIBs. MXenes offer a unique set of functions for AZIBs, yet their significance has not been systematically recognized and summarized. This review article provides an up-to-date overview of MXenes-based electrode materials for AZIBs, with a focus on the unique functions of MXenes in these materials. The discussion starts with MXenes and their derivatives on the cathode side, where they serve as a 2D conductive substrate, 3D framework, flexible support, and coating layer. MXenes can act as both the active material and a precursor to the active material in the cathode. On the anode side, the functions of MXenes include active material host, zinc metal surface protection, electrolyte additive, and separator modification. The review also highlights technical challenges and key hurdles that MXenes currently face in AZIBs.
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spelling ntu-10356/1739562024-03-11T15:35:40Z Versatile MXenes for aqueous zinc batteries Liu, Huan Xin, Zijun Cao, Bin Zhang, Bao Fan, Hong Jin Guo, Shaojun School of Physical and Mathematical Sciences Physics Aqueous zinc-ion batteries Cathodes Aqueous zinc-ion batteries (AZIBs) are gaining popularity for their cost-effectiveness, safety, and utilization of abundant resources. MXenes, which possess outstanding conductivity, controllable surface chemistry, and structural adaptability, are widely recognized as a highly versatile platform for AZIBs. MXenes offer a unique set of functions for AZIBs, yet their significance has not been systematically recognized and summarized. This review article provides an up-to-date overview of MXenes-based electrode materials for AZIBs, with a focus on the unique functions of MXenes in these materials. The discussion starts with MXenes and their derivatives on the cathode side, where they serve as a 2D conductive substrate, 3D framework, flexible support, and coating layer. MXenes can act as both the active material and a precursor to the active material in the cathode. On the anode side, the functions of MXenes include active material host, zinc metal surface protection, electrolyte additive, and separator modification. The review also highlights technical challenges and key hurdles that MXenes currently face in AZIBs. Published version This work was supported by the National Natural Science Foundation ofChina (52273274) and Natural Science Basic Research Project of ShaanxiProvince (2022JQ-123). H. L. also acknowledges financial support from the China Scholarship Council (202008610034). 2024-03-08T00:34:26Z 2024-03-08T00:34:26Z 2024 Journal Article Liu, H., Xin, Z., Cao, B., Zhang, B., Fan, H. J. & Guo, S. (2024). Versatile MXenes for aqueous zinc batteries. Advanced Science, 11(8), 2305806-. https://dx.doi.org/10.1002/advs.202305806 2198-3844 https://hdl.handle.net/10356/173956 10.1002/advs.202305806 37985557 2-s2.0-85177056647 8 11 2305806 en Advanced Science © 2023 The Authors. Advanced Science published by Wiley-VCH GmbH. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited. application/pdf
spellingShingle Physics
Aqueous zinc-ion batteries
Cathodes
Liu, Huan
Xin, Zijun
Cao, Bin
Zhang, Bao
Fan, Hong Jin
Guo, Shaojun
Versatile MXenes for aqueous zinc batteries
title Versatile MXenes for aqueous zinc batteries
title_full Versatile MXenes for aqueous zinc batteries
title_fullStr Versatile MXenes for aqueous zinc batteries
title_full_unstemmed Versatile MXenes for aqueous zinc batteries
title_short Versatile MXenes for aqueous zinc batteries
title_sort versatile mxenes for aqueous zinc batteries
topic Physics
Aqueous zinc-ion batteries
Cathodes
url https://hdl.handle.net/10356/173956
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AT fanhongjin versatilemxenesforaqueouszincbatteries
AT guoshaojun versatilemxenesforaqueouszincbatteries