Multiscale heterogeneities-based piezoresistive interfaces with ultralow detection limitation and adaptively switchable pressure detectability

Mechanical compliance and electrical enhancement are crucial for pressure sensors to promote performances when perceiving external stimuli. Here we propose a bioinspired multiscale heterogeneity-based interface to adaptively regulate its structure layout and switch to desirable piezoresistive behavi...

Full description

Bibliographic Details
Main Authors: He, Xuecheng, Cui, Zequn, Zhang, Feilong, Li, Yanzhen, Tu, Jiaqi, Cao, Jinwei, Wang, Jianwu, Qiao, Yuchun, Xi, Pengxu, Xu, Tailin, Chen, Xiaodong, Zhang, Xueji
Other Authors: School of Materials Science and Engineering
Format: Journal Article
Language:English
Published: 2024
Subjects:
Online Access:https://hdl.handle.net/10356/174642
_version_ 1826129775259811840
author He, Xuecheng
Cui, Zequn
Zhang, Feilong
Li, Yanzhen
Tu, Jiaqi
Cao, Jinwei
Wang, Jianwu
Qiao, Yuchun
Xi, Pengxu
Xu, Tailin
Chen, Xiaodong
Zhang, Xueji
author2 School of Materials Science and Engineering
author_facet School of Materials Science and Engineering
He, Xuecheng
Cui, Zequn
Zhang, Feilong
Li, Yanzhen
Tu, Jiaqi
Cao, Jinwei
Wang, Jianwu
Qiao, Yuchun
Xi, Pengxu
Xu, Tailin
Chen, Xiaodong
Zhang, Xueji
author_sort He, Xuecheng
collection NTU
description Mechanical compliance and electrical enhancement are crucial for pressure sensors to promote performances when perceiving external stimuli. Here we propose a bioinspired multiscale heterogeneity-based interface to adaptively regulate its structure layout and switch to desirable piezoresistive behaviors with ultralow detection limitation. In such a multiscale heterogeneities system, the micro-/nanoscale spiny Ag-MnO2 heterostructure contributes to an ultralow detection limitation of 0.008 Pa and can perceive minor pressure increments under preloads with high resolution (0.0083%). The macroscale heterogeneous orientation of the cellular backbone enables anisotropic deformation, allowing the sensor to switch to rational sensitivity and working range (e.g., 580 kPa-1 for 0-20 kPa/54 kPa-1 for 60-140 kPa) as required. The sensor's stepwise activation progresses from the micro-/nanoscale heterostructure to the macroscale heterogeneous orientation, which can adaptively match diverse sensing tasks in complex applications scenarios. This multiscale heterogeneous and switchable design holds immense potential in the development of intelligent electromechanical devices, including wearable sensors, soft robotics, and smart actuators.
first_indexed 2024-10-01T07:46:04Z
format Journal Article
id ntu-10356/174642
institution Nanyang Technological University
language English
last_indexed 2024-10-01T07:46:04Z
publishDate 2024
record_format dspace
spelling ntu-10356/1746422024-04-05T15:47:41Z Multiscale heterogeneities-based piezoresistive interfaces with ultralow detection limitation and adaptively switchable pressure detectability He, Xuecheng Cui, Zequn Zhang, Feilong Li, Yanzhen Tu, Jiaqi Cao, Jinwei Wang, Jianwu Qiao, Yuchun Xi, Pengxu Xu, Tailin Chen, Xiaodong Zhang, Xueji School of Materials Science and Engineering Innovative Centre for Flexible Devices (iFLEX) Engineering Multiscale Heterogeneous Mechanical compliance and electrical enhancement are crucial for pressure sensors to promote performances when perceiving external stimuli. Here we propose a bioinspired multiscale heterogeneity-based interface to adaptively regulate its structure layout and switch to desirable piezoresistive behaviors with ultralow detection limitation. In such a multiscale heterogeneities system, the micro-/nanoscale spiny Ag-MnO2 heterostructure contributes to an ultralow detection limitation of 0.008 Pa and can perceive minor pressure increments under preloads with high resolution (0.0083%). The macroscale heterogeneous orientation of the cellular backbone enables anisotropic deformation, allowing the sensor to switch to rational sensitivity and working range (e.g., 580 kPa-1 for 0-20 kPa/54 kPa-1 for 60-140 kPa) as required. The sensor's stepwise activation progresses from the micro-/nanoscale heterostructure to the macroscale heterogeneous orientation, which can adaptively match diverse sensing tasks in complex applications scenarios. This multiscale heterogeneous and switchable design holds immense potential in the development of intelligent electromechanical devices, including wearable sensors, soft robotics, and smart actuators. Agency for Science, Technology and Research (A*STAR) Submitted/Accepted version The authors acknowledge funding from the Shenzhen University 2035 Program for Excellent Research (8690100000221),the Joint Fund of the Ministry of Education for Equipment Pre-research (8091B022142), A*STAR Advanced Manufacturing and Engineering (AME) Programmatic Grant (No. A18A1b0045), the Shenzhen Overseas Talent Program, the Shenzhen Key Laboratory for Nano-Biosensing Technology (ZDSYS20210112161400001), and the National Natural Science Foundation of China (22234006). X.H. also acknowledges the China Scholarship Council (CSC, No. 202006460067) for financial support. 2024-04-05T07:19:51Z 2024-04-05T07:19:51Z 2024 Journal Article He, X., Cui, Z., Zhang, F., Li, Y., Tu, J., Cao, J., Wang, J., Qiao, Y., Xi, P., Xu, T., Chen, X. & Zhang, X. (2024). Multiscale heterogeneities-based piezoresistive interfaces with ultralow detection limitation and adaptively switchable pressure detectability. ACS Nano, 18(11), 8296-8306. https://dx.doi.org/10.1021/acsnano.3c12513 1936-0851 https://hdl.handle.net/10356/174642 10.1021/acsnano.3c12513 38452476 2-s2.0-85187318309 11 18 8296 8306 en A18A1b0045 ACS Nano © 2024 American Chemical Society. All rights reserved. This article may be downloaded for personal use only. Any other use requires prior permission of the copyright holder. The Version of Record is available online at http://doi.org/10.1021/acsnano.3c12513. application/pdf
spellingShingle Engineering
Multiscale
Heterogeneous
He, Xuecheng
Cui, Zequn
Zhang, Feilong
Li, Yanzhen
Tu, Jiaqi
Cao, Jinwei
Wang, Jianwu
Qiao, Yuchun
Xi, Pengxu
Xu, Tailin
Chen, Xiaodong
Zhang, Xueji
Multiscale heterogeneities-based piezoresistive interfaces with ultralow detection limitation and adaptively switchable pressure detectability
title Multiscale heterogeneities-based piezoresistive interfaces with ultralow detection limitation and adaptively switchable pressure detectability
title_full Multiscale heterogeneities-based piezoresistive interfaces with ultralow detection limitation and adaptively switchable pressure detectability
title_fullStr Multiscale heterogeneities-based piezoresistive interfaces with ultralow detection limitation and adaptively switchable pressure detectability
title_full_unstemmed Multiscale heterogeneities-based piezoresistive interfaces with ultralow detection limitation and adaptively switchable pressure detectability
title_short Multiscale heterogeneities-based piezoresistive interfaces with ultralow detection limitation and adaptively switchable pressure detectability
title_sort multiscale heterogeneities based piezoresistive interfaces with ultralow detection limitation and adaptively switchable pressure detectability
topic Engineering
Multiscale
Heterogeneous
url https://hdl.handle.net/10356/174642
work_keys_str_mv AT hexuecheng multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability
AT cuizequn multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability
AT zhangfeilong multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability
AT liyanzhen multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability
AT tujiaqi multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability
AT caojinwei multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability
AT wangjianwu multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability
AT qiaoyuchun multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability
AT xipengxu multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability
AT xutailin multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability
AT chenxiaodong multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability
AT zhangxueji multiscaleheterogeneitiesbasedpiezoresistiveinterfaceswithultralowdetectionlimitationandadaptivelyswitchablepressuredetectability