Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride

Photon-lattice (phonon) coupling is fundamental to light-matter interaction, particularly when it reaches the quantum limit of the phonon-coupled single-photon emission, which holds great potential for quantum manipulation and quantum information transduction. Here, we report single defect state-pho...

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Main Authors: Lai, Jia-Min, Tan, Qinghai, Song, Feilong, Chang, Haonan, Lv, Yanpei, Liu, Xue-Lu, Teng, Jinghua, Gao, Weibo, Tan, Ping-Heng, Zhang, Jun
Other Authors: School of Physical and Mathematical Sciences
Format: Journal Article
Language:English
Published: 2024
Subjects:
Online Access:https://hdl.handle.net/10356/180165
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author Lai, Jia-Min
Tan, Qinghai
Song, Feilong
Chang, Haonan
Lv, Yanpei
Liu, Xue-Lu
Teng, Jinghua
Gao, Weibo
Tan, Ping-Heng
Zhang, Jun
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Lai, Jia-Min
Tan, Qinghai
Song, Feilong
Chang, Haonan
Lv, Yanpei
Liu, Xue-Lu
Teng, Jinghua
Gao, Weibo
Tan, Ping-Heng
Zhang, Jun
author_sort Lai, Jia-Min
collection NTU
description Photon-lattice (phonon) coupling is fundamental to light-matter interaction, particularly when it reaches the quantum limit of the phonon-coupled single-photon emission, which holds great potential for quantum manipulation and quantum information transduction. Here, we report single defect state-phonon coupling in hexagonal boron nitride (hBN) at room temperature. An ultrabroad spectrum of single-photon emissions can be achieved by selecting the excitation energies. Using photoluminescence excitation spectroscopy, we observe single-phonon-assisted resonance-enhanced single-photon emission, along with multiple phonon replicas that herald the creation of phonon Fock state. We also develop a transition model to gain insight into the physical process behind the single defect state-phonon coupling. Our work sets the stage for manipulating electron-phonon coupling state with single quantum-level precision at room temperature.
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spelling ntu-10356/1801652024-09-23T00:56:55Z Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride Lai, Jia-Min Tan, Qinghai Song, Feilong Chang, Haonan Lv, Yanpei Liu, Xue-Lu Teng, Jinghua Gao, Weibo Tan, Ping-Heng Zhang, Jun School of Physical and Mathematical Sciences Institute of Materials Research and Engineering, A*STAR Physics Photon-phonon coupling Single-photon emission, h Photon-lattice (phonon) coupling is fundamental to light-matter interaction, particularly when it reaches the quantum limit of the phonon-coupled single-photon emission, which holds great potential for quantum manipulation and quantum information transduction. Here, we report single defect state-phonon coupling in hexagonal boron nitride (hBN) at room temperature. An ultrabroad spectrum of single-photon emissions can be achieved by selecting the excitation energies. Using photoluminescence excitation spectroscopy, we observe single-phonon-assisted resonance-enhanced single-photon emission, along with multiple phonon replicas that herald the creation of phonon Fock state. We also develop a transition model to gain insight into the physical process behind the single defect state-phonon coupling. Our work sets the stage for manipulating electron-phonon coupling state with single quantum-level precision at room temperature. Jun Zhang acknowledges the CAS Interdisciplinary Innovation Team, the National Natural Science Foundation of China (Grant No. 12074371), the Strategic Priority Research Program of Chinese Academy of Sciences (Grant No. XDB28000000), the Research Equipment Development Project of Chinese Academy of Sciences (Grant No. YJKYYQ20210001), the Chinese Academy of Sciences-the Scientific and Technological Research council of TÜRKİYE Joint Research Projects (Grant No. 172111KYSB20210004). 2024-09-23T00:56:54Z 2024-09-23T00:56:54Z 2024 Journal Article Lai, J., Tan, Q., Song, F., Chang, H., Lv, Y., Liu, X., Teng, J., Gao, W., Tan, P. & Zhang, J. (2024). Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride. Science China: Physics, Mechanics and Astronomy, 67(5). https://dx.doi.org/10.1007/s11433-023-2327-5 1674-7348 https://hdl.handle.net/10356/180165 10.1007/s11433-023-2327-5 2-s2.0-85187515130 5 67 en Science China: Physics, Mechanics and Astronomy © 2024 Science China Press. All rights reserved.
spellingShingle Physics
Photon-phonon coupling
Single-photon emission, h
Lai, Jia-Min
Tan, Qinghai
Song, Feilong
Chang, Haonan
Lv, Yanpei
Liu, Xue-Lu
Teng, Jinghua
Gao, Weibo
Tan, Ping-Heng
Zhang, Jun
Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride
title Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride
title_full Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride
title_fullStr Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride
title_full_unstemmed Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride
title_short Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride
title_sort room temperature phonon coupled single photon emission in hexagonal boron nitride
topic Physics
Photon-phonon coupling
Single-photon emission, h
url https://hdl.handle.net/10356/180165
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