Co-solvent induced self-roughness superhydrophobic coatings with self-healing property for versatile oil-water separation

Despite of the extensive effort made to construct a superhydrophobic surface in labs, achieving a short processing time and via a sustainable production route remains a challenge for practical applications. Here, with tetrahydrofuran and n-hexane as co-solvent, we demonstrate that roughness can be i...

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Main Authors: Gao, Shouwei, Dong, Xiuli, Huang, Jianying, Dong, Jianing, Cheng, Yan, Chen, Zhong, Lai, Yuekun
Other Authors: School of Materials Science & Engineering
Format: Journal Article
Language:English
Published: 2019
Subjects:
Online Access:https://hdl.handle.net/10356/80653
http://hdl.handle.net/10220/50057
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author Gao, Shouwei
Dong, Xiuli
Huang, Jianying
Dong, Jianing
Cheng, Yan
Chen, Zhong
Lai, Yuekun
author2 School of Materials Science & Engineering
author_facet School of Materials Science & Engineering
Gao, Shouwei
Dong, Xiuli
Huang, Jianying
Dong, Jianing
Cheng, Yan
Chen, Zhong
Lai, Yuekun
author_sort Gao, Shouwei
collection NTU
description Despite of the extensive effort made to construct a superhydrophobic surface in labs, achieving a short processing time and via a sustainable production route remains a challenge for practical applications. Here, with tetrahydrofuran and n-hexane as co-solvent, we demonstrate that roughness can be induced on polydimethylsiloxane (PDMS) coatings to achieve superhydrophobic coatings on different types of substrates including woven fabrics, non-woven fabrics, and melamine sponge. The sample constructed without adding particles exhibited excellent performance for versatile oil-water separation of mixtures of heavy oil and water, light oil and water, as well as oil-water emulsion. Due to the good solubility of the PDMS in the co-solvent, the dipping solution exhibited a long-time stability. Moreover, the abundant CH3 provided by the self-roughness PDMS coating helped the substrates recover its superhydrophobic property even after destroyed by plasma for 10 times. We believe that this extremely easy dipping-curing method would open up a new direction for fabricating a series of self-roughed superhydrophobic surface with self-healing property. Besides, the developed strategy is fast and easily scalable for industrial applications.
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spelling ntu-10356/806532023-07-14T15:57:04Z Co-solvent induced self-roughness superhydrophobic coatings with self-healing property for versatile oil-water separation Gao, Shouwei Dong, Xiuli Huang, Jianying Dong, Jianing Cheng, Yan Chen, Zhong Lai, Yuekun School of Materials Science & Engineering Engineering::Materials Superhydrophobicity Co-solvent Despite of the extensive effort made to construct a superhydrophobic surface in labs, achieving a short processing time and via a sustainable production route remains a challenge for practical applications. Here, with tetrahydrofuran and n-hexane as co-solvent, we demonstrate that roughness can be induced on polydimethylsiloxane (PDMS) coatings to achieve superhydrophobic coatings on different types of substrates including woven fabrics, non-woven fabrics, and melamine sponge. The sample constructed without adding particles exhibited excellent performance for versatile oil-water separation of mixtures of heavy oil and water, light oil and water, as well as oil-water emulsion. Due to the good solubility of the PDMS in the co-solvent, the dipping solution exhibited a long-time stability. Moreover, the abundant CH3 provided by the self-roughness PDMS coating helped the substrates recover its superhydrophobic property even after destroyed by plasma for 10 times. We believe that this extremely easy dipping-curing method would open up a new direction for fabricating a series of self-roughed superhydrophobic surface with self-healing property. Besides, the developed strategy is fast and easily scalable for industrial applications. Accepted version 2019-10-01T03:44:49Z 2019-12-06T13:54:01Z 2019-10-01T03:44:49Z 2019-12-06T13:54:01Z 2018 Journal Article Gao, S., Dong, X., Huang, J., Dong, J., Cheng, Y., Chen, Z., & Lai, Y. (2018). Co-solvent induced self-roughness superhydrophobic coatings with self-healing property for versatile oil-water separation. Applied Surface Science, 459, 512-519. doi:10.1016/j.apsusc.2018.08.041 0169-4332 https://hdl.handle.net/10356/80653 http://hdl.handle.net/10220/50057 10.1016/j.apsusc.2018.08.041 en Applied Surface Science © 2018 Elsevier B.V. All rights reserved. This paper was published in Applied Surface Science and is made available with permission of Elsevier B.V. 30 p. application/pdf
spellingShingle Engineering::Materials
Superhydrophobicity
Co-solvent
Gao, Shouwei
Dong, Xiuli
Huang, Jianying
Dong, Jianing
Cheng, Yan
Chen, Zhong
Lai, Yuekun
Co-solvent induced self-roughness superhydrophobic coatings with self-healing property for versatile oil-water separation
title Co-solvent induced self-roughness superhydrophobic coatings with self-healing property for versatile oil-water separation
title_full Co-solvent induced self-roughness superhydrophobic coatings with self-healing property for versatile oil-water separation
title_fullStr Co-solvent induced self-roughness superhydrophobic coatings with self-healing property for versatile oil-water separation
title_full_unstemmed Co-solvent induced self-roughness superhydrophobic coatings with self-healing property for versatile oil-water separation
title_short Co-solvent induced self-roughness superhydrophobic coatings with self-healing property for versatile oil-water separation
title_sort co solvent induced self roughness superhydrophobic coatings with self healing property for versatile oil water separation
topic Engineering::Materials
Superhydrophobicity
Co-solvent
url https://hdl.handle.net/10356/80653
http://hdl.handle.net/10220/50057
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