Nonlinear optical response of Au nanorods for broadband pulse modulation in bulk visible lasers

Due to the lack of suitable optical modulators, directly generated Pr3+- and Dy3+-doped bulk visible lasers are limited in the continuous-wave operation; yet, pulsed visible lasers are only sparingly reported recently. It has been theoretically predicated that Au nanorods could modulate the visible...

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Main Authors: Wang, Shuxian, Zhang, Yuxia, Xing, Jun, Liu, Xinfeng, Yu, Haohai, Di Lieto, Alberto, Tonelli, Mauro, Sum, Tze Chien, Zhang, Huaijin, Xiong, Qihua
Other Authors: School of Electrical and Electronic Engineering
Format: Journal Article
Language:English
Published: 2015
Online Access:https://hdl.handle.net/10356/80977
http://hdl.handle.net/10220/38993
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author Wang, Shuxian
Zhang, Yuxia
Xing, Jun
Liu, Xinfeng
Yu, Haohai
Di Lieto, Alberto
Tonelli, Mauro
Sum, Tze Chien
Zhang, Huaijin
Xiong, Qihua
author2 School of Electrical and Electronic Engineering
author_facet School of Electrical and Electronic Engineering
Wang, Shuxian
Zhang, Yuxia
Xing, Jun
Liu, Xinfeng
Yu, Haohai
Di Lieto, Alberto
Tonelli, Mauro
Sum, Tze Chien
Zhang, Huaijin
Xiong, Qihua
author_sort Wang, Shuxian
collection NTU
description Due to the lack of suitable optical modulators, directly generated Pr3+- and Dy3+-doped bulk visible lasers are limited in the continuous-wave operation; yet, pulsed visible lasers are only sparingly reported recently. It has been theoretically predicated that Au nanorods could modulate the visible light operation, based on the nonlinear optical response of surface plasmon resonance. Here, we demonstrate the saturable absorption properties of Au nanorods in the visible region and experimentally realized the pulsed visible lasers over the spectral range of orange (605 nm), red (639 nm), and deep red (721 nm) with Au nanorods as the optical modulator. We show that Au nanorods have a broad nonlinear optical response and can serve as a type of broadband, low-cost, and eco-friendly candidate for optical switchers in the visible region. Our work also advocates the promise of plasmonic nanostructures for the development of pulsed lasers and other plasmonic devices.
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spelling ntu-10356/809772023-02-28T19:30:09Z Nonlinear optical response of Au nanorods for broadband pulse modulation in bulk visible lasers Wang, Shuxian Zhang, Yuxia Xing, Jun Liu, Xinfeng Yu, Haohai Di Lieto, Alberto Tonelli, Mauro Sum, Tze Chien Zhang, Huaijin Xiong, Qihua School of Electrical and Electronic Engineering School of Physical and Mathematical Sciences Due to the lack of suitable optical modulators, directly generated Pr3+- and Dy3+-doped bulk visible lasers are limited in the continuous-wave operation; yet, pulsed visible lasers are only sparingly reported recently. It has been theoretically predicated that Au nanorods could modulate the visible light operation, based on the nonlinear optical response of surface plasmon resonance. Here, we demonstrate the saturable absorption properties of Au nanorods in the visible region and experimentally realized the pulsed visible lasers over the spectral range of orange (605 nm), red (639 nm), and deep red (721 nm) with Au nanorods as the optical modulator. We show that Au nanorods have a broad nonlinear optical response and can serve as a type of broadband, low-cost, and eco-friendly candidate for optical switchers in the visible region. Our work also advocates the promise of plasmonic nanostructures for the development of pulsed lasers and other plasmonic devices. Published version 2015-12-08T02:39:57Z 2019-12-06T14:18:44Z 2015-12-08T02:39:57Z 2019-12-06T14:18:44Z 2015 Journal Article Wang, S., Zhang, Y., Xing, J., Liu, X., Yu, H., Di Lieto, A., et al. Nonlinear optical response of Au nanorods for broadband pulse modulation in bulk visible lasers. Applied Physics Letters, 107(16), 161103-. 0003-6951 https://hdl.handle.net/10356/80977 http://hdl.handle.net/10220/38993 10.1063/1.4934528 en Applied Physics Letters © 2015 AIP Publishing LLC. This paper was published in Applied Physics Letters and is made available as an electronic reprint (preprint) with permission of AIP Publishing LLC. The published version is available at: [http://dx.doi.org/10.1063/1.4934528]. One print or electronic copy may be made for personal use only. Systematic or multiple reproduction, distribution to multiple locations via electronic or other means, duplication of any material in this paper for a fee or for commercial purposes, or modification of the content of the paper is prohibited and is subject to penalties under law. 5 p. application/pdf
spellingShingle Wang, Shuxian
Zhang, Yuxia
Xing, Jun
Liu, Xinfeng
Yu, Haohai
Di Lieto, Alberto
Tonelli, Mauro
Sum, Tze Chien
Zhang, Huaijin
Xiong, Qihua
Nonlinear optical response of Au nanorods for broadband pulse modulation in bulk visible lasers
title Nonlinear optical response of Au nanorods for broadband pulse modulation in bulk visible lasers
title_full Nonlinear optical response of Au nanorods for broadband pulse modulation in bulk visible lasers
title_fullStr Nonlinear optical response of Au nanorods for broadband pulse modulation in bulk visible lasers
title_full_unstemmed Nonlinear optical response of Au nanorods for broadband pulse modulation in bulk visible lasers
title_short Nonlinear optical response of Au nanorods for broadband pulse modulation in bulk visible lasers
title_sort nonlinear optical response of au nanorods for broadband pulse modulation in bulk visible lasers
url https://hdl.handle.net/10356/80977
http://hdl.handle.net/10220/38993
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