Measurement of infrared optical constants with visible photons

We demonstrate a new scheme for infrared spectroscopy with visible light sources and detectors. The technique relies on the nonlinear interference of correlated photons, produced via spontaneous parametric down conversion in a nonlinear crystal. Visible and infrared photons are split into two paths...

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Main Authors: Paterova, Anna, Yang, Hongzhi, An, Chengwu, Kalashnikov, Dmitry, Krivitsky, Leonid
Other Authors: School of Electrical and Electronic Engineering
Format: Journal Article
Language:English
Published: 2018
Subjects:
Online Access:https://hdl.handle.net/10356/84296
http://hdl.handle.net/10220/45089
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author Paterova, Anna
Yang, Hongzhi
An, Chengwu
Kalashnikov, Dmitry
Krivitsky, Leonid
author2 School of Electrical and Electronic Engineering
author_facet School of Electrical and Electronic Engineering
Paterova, Anna
Yang, Hongzhi
An, Chengwu
Kalashnikov, Dmitry
Krivitsky, Leonid
author_sort Paterova, Anna
collection NTU
description We demonstrate a new scheme for infrared spectroscopy with visible light sources and detectors. The technique relies on the nonlinear interference of correlated photons, produced via spontaneous parametric down conversion in a nonlinear crystal. Visible and infrared photons are split into two paths and the infrared photons interact with the sample under study. The photons are reflected back to the crystal, resembling a conventional Michelson interferometer. Interference of the visible photons is observed and it is dependent on the phases of all three interacting photons: pump, visible and infrared. The transmission coefficient and the refractive index of the sample in the infrared range can be inferred from the interference pattern of visible photons. The method does not require the use of potentially expensive and inefficient infrared detectors and sources, it can be applied to a broad variety of samples, and it does not require a priori knowledge of sample properties in the visible range.
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spelling ntu-10356/842962020-03-07T13:57:25Z Measurement of infrared optical constants with visible photons Paterova, Anna Yang, Hongzhi An, Chengwu Kalashnikov, Dmitry Krivitsky, Leonid School of Electrical and Electronic Engineering IR Spectroscopy Interferometry We demonstrate a new scheme for infrared spectroscopy with visible light sources and detectors. The technique relies on the nonlinear interference of correlated photons, produced via spontaneous parametric down conversion in a nonlinear crystal. Visible and infrared photons are split into two paths and the infrared photons interact with the sample under study. The photons are reflected back to the crystal, resembling a conventional Michelson interferometer. Interference of the visible photons is observed and it is dependent on the phases of all three interacting photons: pump, visible and infrared. The transmission coefficient and the refractive index of the sample in the infrared range can be inferred from the interference pattern of visible photons. The method does not require the use of potentially expensive and inefficient infrared detectors and sources, it can be applied to a broad variety of samples, and it does not require a priori knowledge of sample properties in the visible range. ASTAR (Agency for Sci., Tech. and Research, S’pore) Published version 2018-07-17T02:14:35Z 2019-12-06T15:42:18Z 2018-07-17T02:14:35Z 2019-12-06T15:42:18Z 2018 Journal Article Paterova, A., Yang, H., An, C., Kalashnikov, D., & Krivitsky, L. (2018). Measurement of infrared optical constants with visible photons. New Journal of Physics, 20(4), 043015-. 1367-2630 https://hdl.handle.net/10356/84296 http://hdl.handle.net/10220/45089 10.1088/1367-2630/aab5ce en New Journal of Physics © 2018 The Author(s). Published by IOP Publishing Ltd on behalf of Deutsche Physikalische Gesellschaft 10 p. application/pdf
spellingShingle IR Spectroscopy
Interferometry
Paterova, Anna
Yang, Hongzhi
An, Chengwu
Kalashnikov, Dmitry
Krivitsky, Leonid
Measurement of infrared optical constants with visible photons
title Measurement of infrared optical constants with visible photons
title_full Measurement of infrared optical constants with visible photons
title_fullStr Measurement of infrared optical constants with visible photons
title_full_unstemmed Measurement of infrared optical constants with visible photons
title_short Measurement of infrared optical constants with visible photons
title_sort measurement of infrared optical constants with visible photons
topic IR Spectroscopy
Interferometry
url https://hdl.handle.net/10356/84296
http://hdl.handle.net/10220/45089
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