Effect of fluidized granular activated carbon (GAC) on critical flux in the microfiltration of particulate foulants

The fluidization of Granular Activated Carbon (GAC) particles has received much attention in recent years as a promising method for mitigating membrane fouling particularly in membrane bioreactors (MBRs). In particular, the fluidized GAC particles are acknowledged to be beneficial in terms of adsorp...

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Main Authors: Chew, Jia Wei, Wang, Jingwei, Wu, Bing, Liu, Yu, Fane, Anthony Gordon
Other Authors: School of Chemical and Biomedical Engineering
Format: Journal Article
Language:English
Published: 2017
Subjects:
Online Access:https://hdl.handle.net/10356/85579
http://hdl.handle.net/10220/43788
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author Chew, Jia Wei
Wang, Jingwei
Wu, Bing
Liu, Yu
Fane, Anthony Gordon
author2 School of Chemical and Biomedical Engineering
author_facet School of Chemical and Biomedical Engineering
Chew, Jia Wei
Wang, Jingwei
Wu, Bing
Liu, Yu
Fane, Anthony Gordon
author_sort Chew, Jia Wei
collection NTU
description The fluidization of Granular Activated Carbon (GAC) particles has received much attention in recent years as a promising method for mitigating membrane fouling particularly in membrane bioreactors (MBRs). In particular, the fluidized GAC particles are acknowledged to be beneficial in terms of adsorption of organic foulants, and mechanical scouring and surface shear of the membrane surface. Both lab-scale and pilot-scale studies have affirmed the efficacy of GAC fluidization in maintaining a depressed extent of membrane fouling in anaerobic fluidized bed - membrane bioreactors (AnFMBRs). More in-depth studies have also correlated the hydrodynamics of fluidized GAC particles with the effectiveness of membrane fouling mitigation. This study aimed at understanding the improvement of fine (micron-sized) particle critical flux in the presence of fluidized GAC via the Direct Observation Through the Membrane (DOTM) technique. The model foulant was a suspension of polystyrene particles (5 µm sized), and the parameters investigated included GAC particle diameter (dp), superficial liquid velocity (Ul) and thereby power requirement (Pr), and height along the vertically aligned membrane. Results indicate that: (i) fluidized GAC increased the critical flux by an order-of-magnitude relative to that with tangential liquid shear alone; (ii) the overall critical flux (Jcritical, overall) expectedly increased with power input (Pr), but the relationship between local critical flux (Jcritical) and power input (Pr) depended on the position along the membrane height; (iii) at the same Pr, although the larger GAC particles were more effective locally (i.e., higher Jcritical) due to greater particle inertia, the smaller GAC particles were more effective overall (i.e., higher Jcritical, overall) due to greater bed expansion enabling scouring of more membrane heights; and (iv) a higher power input (Pr) was required for sufficient bed expansion to enable more consistent critical flux (Jcritical) values over the whole membrane height.
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spelling ntu-10356/855792020-03-07T11:35:27Z Effect of fluidized granular activated carbon (GAC) on critical flux in the microfiltration of particulate foulants Chew, Jia Wei Wang, Jingwei Wu, Bing Liu, Yu Fane, Anthony Gordon School of Chemical and Biomedical Engineering School of Civil and Environmental Engineering Interdisciplinary Graduate School (IGS) Advanced Environmental Biotechnology Centre (AEBC) Nanyang Environment and Water Research Institute Singapore Membrane Technology Centre Membrane fouling mitigation Liquid-solid fluidization The fluidization of Granular Activated Carbon (GAC) particles has received much attention in recent years as a promising method for mitigating membrane fouling particularly in membrane bioreactors (MBRs). In particular, the fluidized GAC particles are acknowledged to be beneficial in terms of adsorption of organic foulants, and mechanical scouring and surface shear of the membrane surface. Both lab-scale and pilot-scale studies have affirmed the efficacy of GAC fluidization in maintaining a depressed extent of membrane fouling in anaerobic fluidized bed - membrane bioreactors (AnFMBRs). More in-depth studies have also correlated the hydrodynamics of fluidized GAC particles with the effectiveness of membrane fouling mitigation. This study aimed at understanding the improvement of fine (micron-sized) particle critical flux in the presence of fluidized GAC via the Direct Observation Through the Membrane (DOTM) technique. The model foulant was a suspension of polystyrene particles (5 µm sized), and the parameters investigated included GAC particle diameter (dp), superficial liquid velocity (Ul) and thereby power requirement (Pr), and height along the vertically aligned membrane. Results indicate that: (i) fluidized GAC increased the critical flux by an order-of-magnitude relative to that with tangential liquid shear alone; (ii) the overall critical flux (Jcritical, overall) expectedly increased with power input (Pr), but the relationship between local critical flux (Jcritical) and power input (Pr) depended on the position along the membrane height; (iii) at the same Pr, although the larger GAC particles were more effective locally (i.e., higher Jcritical) due to greater particle inertia, the smaller GAC particles were more effective overall (i.e., higher Jcritical, overall) due to greater bed expansion enabling scouring of more membrane heights; and (iv) a higher power input (Pr) was required for sufficient bed expansion to enable more consistent critical flux (Jcritical) values over the whole membrane height. NRF (Natl Research Foundation, S’pore) MOE (Min. of Education, S’pore) EDB (Economic Devt. Board, S’pore) 2017-09-22T05:23:18Z 2019-12-06T16:06:28Z 2017-09-22T05:23:18Z 2019-12-06T16:06:28Z 2016 Journal Article Wang, J., Wu, B., Liu, Y., Fane, A. G., & Chew, J. W. (2017). Effect of fluidized granular activated carbon (GAC) on critical flux in the microfiltration of particulate foulants. Journal of Membrane Science, 523, 409-417. 0376-7388 https://hdl.handle.net/10356/85579 http://hdl.handle.net/10220/43788 10.1016/j.memsci.2016.09.039 en Journal of Membrane Science © 2016 Elsevier
spellingShingle Membrane fouling mitigation
Liquid-solid fluidization
Chew, Jia Wei
Wang, Jingwei
Wu, Bing
Liu, Yu
Fane, Anthony Gordon
Effect of fluidized granular activated carbon (GAC) on critical flux in the microfiltration of particulate foulants
title Effect of fluidized granular activated carbon (GAC) on critical flux in the microfiltration of particulate foulants
title_full Effect of fluidized granular activated carbon (GAC) on critical flux in the microfiltration of particulate foulants
title_fullStr Effect of fluidized granular activated carbon (GAC) on critical flux in the microfiltration of particulate foulants
title_full_unstemmed Effect of fluidized granular activated carbon (GAC) on critical flux in the microfiltration of particulate foulants
title_short Effect of fluidized granular activated carbon (GAC) on critical flux in the microfiltration of particulate foulants
title_sort effect of fluidized granular activated carbon gac on critical flux in the microfiltration of particulate foulants
topic Membrane fouling mitigation
Liquid-solid fluidization
url https://hdl.handle.net/10356/85579
http://hdl.handle.net/10220/43788
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