Exploring Peltier effect in organic thermoelectric films

Organic materials are emerging thermoelectric candidates for flexible power generation and solid-cooling applications. Although the Peltier effect is a fundamental thermoelectric effect that enables site-specific and on-demand cooling applications, the Peltier effect in organic thermoelectric films...

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Main Authors: Jin, Wenlong, Liu, Liyao, Yang, Tao, Shen, Hongguang, Zhu, Jia, Xu, Wei, Li, Shuzhou, Li, Qing, Chi, Lifeng, Di, Chong-an, Zhu, Daoben
Other Authors: School of Materials Science & Engineering
Format: Journal Article
Language:English
Published: 2018
Subjects:
Online Access:https://hdl.handle.net/10356/89065
http://hdl.handle.net/10220/46072
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author Jin, Wenlong
Liu, Liyao
Yang, Tao
Shen, Hongguang
Zhu, Jia
Xu, Wei
Li, Shuzhou
Li, Qing
Chi, Lifeng
Di, Chong-an
Zhu, Daoben
author2 School of Materials Science & Engineering
author_facet School of Materials Science & Engineering
Jin, Wenlong
Liu, Liyao
Yang, Tao
Shen, Hongguang
Zhu, Jia
Xu, Wei
Li, Shuzhou
Li, Qing
Chi, Lifeng
Di, Chong-an
Zhu, Daoben
author_sort Jin, Wenlong
collection NTU
description Organic materials are emerging thermoelectric candidates for flexible power generation and solid-cooling applications. Although the Peltier effect is a fundamental thermoelectric effect that enables site-specific and on-demand cooling applications, the Peltier effect in organic thermoelectric films have not been investigated. Here we experimentally observed and quasi-quantitatively evaluated the Peltier effect in a poly(Ni-ett) film through the fabrication of thermally suspended devices combined with an infrared imaging technique. The experimental and simulation results confirm effective extraction of the Peltier effect and verify the Thomson relations in organic materials. More importantly, the working device based on poly(Ni-ett) film yields maximum temperature differences as large as 41 K at the two contacts and a cooling of 0.2 K even under heat-insulated condition. This exploration of the Peltier effect in organic thermoelectric films predicts that organic materials hold the ultimate potential to enable flexible solid-cooling applications.
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spelling ntu-10356/890652023-07-14T15:44:40Z Exploring Peltier effect in organic thermoelectric films Jin, Wenlong Liu, Liyao Yang, Tao Shen, Hongguang Zhu, Jia Xu, Wei Li, Shuzhou Li, Qing Chi, Lifeng Di, Chong-an Zhu, Daoben School of Materials Science & Engineering Centre for Programmable Materials DRNTU::Engineering::Materials Peltier Effect Thermoelectric Films Organic materials are emerging thermoelectric candidates for flexible power generation and solid-cooling applications. Although the Peltier effect is a fundamental thermoelectric effect that enables site-specific and on-demand cooling applications, the Peltier effect in organic thermoelectric films have not been investigated. Here we experimentally observed and quasi-quantitatively evaluated the Peltier effect in a poly(Ni-ett) film through the fabrication of thermally suspended devices combined with an infrared imaging technique. The experimental and simulation results confirm effective extraction of the Peltier effect and verify the Thomson relations in organic materials. More importantly, the working device based on poly(Ni-ett) film yields maximum temperature differences as large as 41 K at the two contacts and a cooling of 0.2 K even under heat-insulated condition. This exploration of the Peltier effect in organic thermoelectric films predicts that organic materials hold the ultimate potential to enable flexible solid-cooling applications. Published version 2018-09-24T05:33:14Z 2019-12-06T17:17:05Z 2018-09-24T05:33:14Z 2019-12-06T17:17:05Z 2018 Journal Article Jin, W., Liu, L., Yang, T., Shen, H., Zhu, J., Xu, W., . . . Zhu, D. (2018). Exploring Peltier effect in organic thermoelectric films. Nature Communications, 9(1), 3586-. doi:10.1038/s41467-018-05999-4 https://hdl.handle.net/10356/89065 http://hdl.handle.net/10220/46072 10.1038/s41467-018-05999-4 en Nature Communications © 2018 The Author(s). This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. 6 p. application/pdf
spellingShingle DRNTU::Engineering::Materials
Peltier Effect
Thermoelectric Films
Jin, Wenlong
Liu, Liyao
Yang, Tao
Shen, Hongguang
Zhu, Jia
Xu, Wei
Li, Shuzhou
Li, Qing
Chi, Lifeng
Di, Chong-an
Zhu, Daoben
Exploring Peltier effect in organic thermoelectric films
title Exploring Peltier effect in organic thermoelectric films
title_full Exploring Peltier effect in organic thermoelectric films
title_fullStr Exploring Peltier effect in organic thermoelectric films
title_full_unstemmed Exploring Peltier effect in organic thermoelectric films
title_short Exploring Peltier effect in organic thermoelectric films
title_sort exploring peltier effect in organic thermoelectric films
topic DRNTU::Engineering::Materials
Peltier Effect
Thermoelectric Films
url https://hdl.handle.net/10356/89065
http://hdl.handle.net/10220/46072
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