Size and surface effects on transient photoconductivity in CdS nanobelts probed by time-resolved terahertz spectroscopy

Ultrafast optical-pump terahertz probe spectroscopy was performed over a graduated size distribution of CdS nanobelts to investigate the size and surface effects on the transient photoconductivity. It was found that the nanobelt size has a profound influence on the carrier localization and photocond...

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Main Authors: Li, Mingjie, Wu, Bo, Ekahana, Sandy Adhitia, Utama, Muhammad Iqbal Bakti, Xing, Guichuan, Xiong, Qihua, Sum, Tze Chien, Zhang, Xinhai
Other Authors: School of Electrical and Electronic Engineering
Format: Journal Article
Language:English
Published: 2013
Online Access:https://hdl.handle.net/10356/94940
http://hdl.handle.net/10220/9223
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author Li, Mingjie
Wu, Bo
Ekahana, Sandy Adhitia
Utama, Muhammad Iqbal Bakti
Xing, Guichuan
Xiong, Qihua
Sum, Tze Chien
Zhang, Xinhai
author2 School of Electrical and Electronic Engineering
author_facet School of Electrical and Electronic Engineering
Li, Mingjie
Wu, Bo
Ekahana, Sandy Adhitia
Utama, Muhammad Iqbal Bakti
Xing, Guichuan
Xiong, Qihua
Sum, Tze Chien
Zhang, Xinhai
author_sort Li, Mingjie
collection NTU
description Ultrafast optical-pump terahertz probe spectroscopy was performed over a graduated size distribution of CdS nanobelts to investigate the size and surface effects on the transient photoconductivity. It was found that the nanobelt size has a profound influence on the carrier localization and photoconductivity dynamics, brought about by the carrier trapping at surface defects. The strong carrier localization in the nanobelt is ascribed to the internal surface boundaries arising from the surface depletion layer. The increased thickness of surface depletion layer due to a continuous trapping of photocarriers at surface defects results in more pronounced carrier localization after photoexcitation.
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spelling ntu-10356/949402023-02-28T19:38:39Z Size and surface effects on transient photoconductivity in CdS nanobelts probed by time-resolved terahertz spectroscopy Li, Mingjie Wu, Bo Ekahana, Sandy Adhitia Utama, Muhammad Iqbal Bakti Xing, Guichuan Xiong, Qihua Sum, Tze Chien Zhang, Xinhai School of Electrical and Electronic Engineering Ultrafast optical-pump terahertz probe spectroscopy was performed over a graduated size distribution of CdS nanobelts to investigate the size and surface effects on the transient photoconductivity. It was found that the nanobelt size has a profound influence on the carrier localization and photoconductivity dynamics, brought about by the carrier trapping at surface defects. The strong carrier localization in the nanobelt is ascribed to the internal surface boundaries arising from the surface depletion layer. The increased thickness of surface depletion layer due to a continuous trapping of photocarriers at surface defects results in more pronounced carrier localization after photoexcitation. Published version 2013-02-21T08:04:09Z 2019-12-06T19:05:05Z 2013-02-21T08:04:09Z 2019-12-06T19:05:05Z 2012 2012 Journal Article Li, M., Wu, B., Ekahana, S. A., Utama, M. I. B., Xing, G., Xiong, Q., et al. (2012). Size and surface effects on transient photoconductivity in CdS nanobelts probed by time-resolved terahertz spectroscopy. Applied Physics Letters, 101(9). 0003-6951 https://hdl.handle.net/10356/94940 http://hdl.handle.net/10220/9223 10.1063/1.4748300 en Applied Physics Letters © 2012 American Institute of Physics. This paper was published in Applied Physics Letters and is made available as an electronic reprint (preprint) with permission of American Institute of Physics. The paper can be found at the following official DOI: [http://dx.doi.org/10.1063/1.4748300]. One print or electronic copy may be made for personal use only. Systematic or multiple reproduction, distribution to multiple locations via electronic or other means, duplication of any material in this paper for a fee or for commercial purposes, or modification of the content of the paper is prohibited and is subject to penalties under law. application/pdf
spellingShingle Li, Mingjie
Wu, Bo
Ekahana, Sandy Adhitia
Utama, Muhammad Iqbal Bakti
Xing, Guichuan
Xiong, Qihua
Sum, Tze Chien
Zhang, Xinhai
Size and surface effects on transient photoconductivity in CdS nanobelts probed by time-resolved terahertz spectroscopy
title Size and surface effects on transient photoconductivity in CdS nanobelts probed by time-resolved terahertz spectroscopy
title_full Size and surface effects on transient photoconductivity in CdS nanobelts probed by time-resolved terahertz spectroscopy
title_fullStr Size and surface effects on transient photoconductivity in CdS nanobelts probed by time-resolved terahertz spectroscopy
title_full_unstemmed Size and surface effects on transient photoconductivity in CdS nanobelts probed by time-resolved terahertz spectroscopy
title_short Size and surface effects on transient photoconductivity in CdS nanobelts probed by time-resolved terahertz spectroscopy
title_sort size and surface effects on transient photoconductivity in cds nanobelts probed by time resolved terahertz spectroscopy
url https://hdl.handle.net/10356/94940
http://hdl.handle.net/10220/9223
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