Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy
Experimental demonstrations and detailed theoretical explanations are provided for a thorough understanding of the various phase-cycling schemes in an optical pulse shaper assisted two-dimensional electronic spectroscopy (2DES) in a pump–probe beam geometry. We show that two and three-step phase-cyc...
| Main Authors: | , , , |
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| Other Authors: | |
| Format: | Journal Article |
| Language: | English |
| Published: |
2013
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| Online Access: | https://hdl.handle.net/10356/96120 http://hdl.handle.net/10220/10813 |
| _version_ | 1826112193112834048 |
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| author | Zhang, Zhengyang Wells, Kym Lewis Hyland, Edward William James Tan, Howe-Siang |
| author2 | School of Physical and Mathematical Sciences |
| author_facet | School of Physical and Mathematical Sciences Zhang, Zhengyang Wells, Kym Lewis Hyland, Edward William James Tan, Howe-Siang |
| author_sort | Zhang, Zhengyang |
| collection | NTU |
| description | Experimental demonstrations and detailed theoretical explanations are provided for a thorough understanding of the various phase-cycling schemes in an optical pulse shaper assisted two-dimensional electronic spectroscopy (2DES) in a pump–probe beam geometry. We show that two and three-step phase-cycling schemes can be employed to retrieve both rephasing and nonrephasing 2D spectra. The studies were performed on the Qy transition of chlorophyll a. |
| first_indexed | 2024-10-01T03:02:57Z |
| format | Journal Article |
| id | ntu-10356/96120 |
| institution | Nanyang Technological University |
| language | English |
| last_indexed | 2024-10-01T03:02:57Z |
| publishDate | 2013 |
| record_format | dspace |
| spelling | ntu-10356/961202020-03-07T12:37:05Z Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy Zhang, Zhengyang Wells, Kym Lewis Hyland, Edward William James Tan, Howe-Siang School of Physical and Mathematical Sciences Experimental demonstrations and detailed theoretical explanations are provided for a thorough understanding of the various phase-cycling schemes in an optical pulse shaper assisted two-dimensional electronic spectroscopy (2DES) in a pump–probe beam geometry. We show that two and three-step phase-cycling schemes can be employed to retrieve both rephasing and nonrephasing 2D spectra. The studies were performed on the Qy transition of chlorophyll a. 2013-06-27T06:42:45Z 2019-12-06T19:26:04Z 2013-06-27T06:42:45Z 2019-12-06T19:26:04Z 2012 2012 Journal Article Zhang, Z., Wells, K. L., Hyland, E. W. J., & Tan, H.-S. (2012). Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy. Chemical Physics Letters, 550, 156-161. 0009-2614 https://hdl.handle.net/10356/96120 http://hdl.handle.net/10220/10813 10.1016/j.cplett.2012.08.037 en Chemical physics letters © 2012 Elsevier B.V. |
| spellingShingle | Zhang, Zhengyang Wells, Kym Lewis Hyland, Edward William James Tan, Howe-Siang Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| title | Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| title_full | Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| title_fullStr | Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| title_full_unstemmed | Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| title_short | Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| title_sort | phase cycling schemes for pump probe beam geometry two dimensional electronic spectroscopy |
| url | https://hdl.handle.net/10356/96120 http://hdl.handle.net/10220/10813 |
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