Restoration of the third law in spin ice thin films

A characteristic feature of spin ice is its apparent violation of the third law of thermodynamics. This leads to a number of interesting properties including the emergence of an effective vacuum for magnetic monopoles and their currents – magnetricity. Here we add a new dimension to the experimental...

Full description

Bibliographic Details
Main Authors: Bovo, L, Moya, X, Prabhakaran, D, Soh, Y, Boothroyd, A, Mathur, N, Aeppli, G, Bramwell, S
Format: Journal article
Language:English
Published: Springer Nature 2014
_version_ 1797050636206866432
author Bovo, L
Moya, X
Prabhakaran, D
Soh, Y
Boothroyd, A
Mathur, N
Aeppli, G
Bramwell, S
author_facet Bovo, L
Moya, X
Prabhakaran, D
Soh, Y
Boothroyd, A
Mathur, N
Aeppli, G
Bramwell, S
author_sort Bovo, L
collection OXFORD
description A characteristic feature of spin ice is its apparent violation of the third law of thermodynamics. This leads to a number of interesting properties including the emergence of an effective vacuum for magnetic monopoles and their currents – magnetricity. Here we add a new dimension to the experimental study of spin ice by fabricating thin epitaxial films of Dy2Ti2O7, varying between 5 and 60 monolayers on an inert substrate. The films show the distinctive characteristics of spin ice at temperatures >2 K, but at lower temperature we find evidence of a zero entropy state. This restoration of the third law in spin ice thin films is consistent with a predicted strain-induced ordering of a very unusual type, previously discussed for analogous electrical systems. Our results show how the physics of frustrated pyrochlore magnets such as spin ice may be significantly modified in thin-film samples.
first_indexed 2024-03-06T18:08:06Z
format Journal article
id oxford-uuid:021f3a0a-cfd6-4228-bcab-d59a85c36cf2
institution University of Oxford
language English
last_indexed 2024-03-06T18:08:06Z
publishDate 2014
publisher Springer Nature
record_format dspace
spelling oxford-uuid:021f3a0a-cfd6-4228-bcab-d59a85c36cf22022-03-26T08:38:48ZRestoration of the third law in spin ice thin filmsJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:021f3a0a-cfd6-4228-bcab-d59a85c36cf2EnglishSymplectic Elements at OxfordSpringer Nature2014Bovo, LMoya, XPrabhakaran, DSoh, YBoothroyd, AMathur, NAeppli, GBramwell, SA characteristic feature of spin ice is its apparent violation of the third law of thermodynamics. This leads to a number of interesting properties including the emergence of an effective vacuum for magnetic monopoles and their currents – magnetricity. Here we add a new dimension to the experimental study of spin ice by fabricating thin epitaxial films of Dy2Ti2O7, varying between 5 and 60 monolayers on an inert substrate. The films show the distinctive characteristics of spin ice at temperatures >2 K, but at lower temperature we find evidence of a zero entropy state. This restoration of the third law in spin ice thin films is consistent with a predicted strain-induced ordering of a very unusual type, previously discussed for analogous electrical systems. Our results show how the physics of frustrated pyrochlore magnets such as spin ice may be significantly modified in thin-film samples.
spellingShingle Bovo, L
Moya, X
Prabhakaran, D
Soh, Y
Boothroyd, A
Mathur, N
Aeppli, G
Bramwell, S
Restoration of the third law in spin ice thin films
title Restoration of the third law in spin ice thin films
title_full Restoration of the third law in spin ice thin films
title_fullStr Restoration of the third law in spin ice thin films
title_full_unstemmed Restoration of the third law in spin ice thin films
title_short Restoration of the third law in spin ice thin films
title_sort restoration of the third law in spin ice thin films
work_keys_str_mv AT bovol restorationofthethirdlawinspinicethinfilms
AT moyax restorationofthethirdlawinspinicethinfilms
AT prabhakarand restorationofthethirdlawinspinicethinfilms
AT sohy restorationofthethirdlawinspinicethinfilms
AT boothroyda restorationofthethirdlawinspinicethinfilms
AT mathurn restorationofthethirdlawinspinicethinfilms
AT aepplig restorationofthethirdlawinspinicethinfilms
AT bramwells restorationofthethirdlawinspinicethinfilms