Tailoring the magnetic exchange interaction in MnBi2Te4 superlattices via the intercalation of ferromagnetic layers

<p>The intrinsic magnetic topological insulator MnBi<sub>2</sub>Te<sub>4</sub>&nbsp;(MBT) provides a platform for the creation of exotic quantum phenomena. Novel properties can be created by modification of the MnBi<sub>2</sub>Te<sub>4</sub>&...

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Bibliographic Details
Main Authors: Chen, P, Yao, Q, Xu, J, Sun, Q, Grutter, AJ, Quarterman, P, Balakrishnan, PP, Kinane, CJ, Caruana, AJ, Langridge, S, Li, A, Achinuq, B, Heppell, E, Ji, Y, Liu, S, Cui, B, Liu, J, Huang, P, Liu, Z, Yu, G, Xiu, F, Hesjedal, T, Zou, J, Han, X, Zhang, H, Yang, Y, Kou, X
Format: Journal article
Language:English
Published: Springer Nature 2022
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Summary:<p>The intrinsic magnetic topological insulator MnBi<sub>2</sub>Te<sub>4</sub>&nbsp;(MBT) provides a platform for the creation of exotic quantum phenomena. Novel properties can be created by modification of the MnBi<sub>2</sub>Te<sub>4</sub>&nbsp;framework, but the design of stable magnetic structures remains challenging. Here we report ferromagnet-intercalated MnBi<sub>2</sub>Te<sub>4</sub>&nbsp;superlattices with tunable magnetic exchange interactions. Using molecular beam epitaxy, we intercalate ferromagnetic MnTe layers into MnBi<sub>2</sub>Te<sub>4</sub>&nbsp;to create [(MBT)(MnTe)<sub><em>m</em></sub>]<sub><em>N</em></sub>&nbsp;superlattices and examine their magnetic interaction properties using polarized neutron reflectometry and magnetoresistance measurements. Incorporation of the ferromagnetic spacer tunes the antiferromagnetic interlayer coupling of the MnBi<sub>2</sub>Te<sub>4</sub>&nbsp;layers through the exchange-spring effect at MnBi<sub>2</sub>Te<sub>4</sub>/MnTe hetero-interfaces. The MnTe thickness can be used to modulate the relative strengths of the ferromagnetic and antiferromagnetic order, and the superlattice periodicity can tailor the spin configurations of the synthesized multilayers.</p>