Ultrafast, polarized, single-photon emission from m-plane InGaN Quantum Dots on GaN nanowires

We demonstrate single photon emission from self-assembled m-plane InGaN quantum dots (QDs) embedded on the side-walls of GaN nanowires. A combination of electron microscopy, cathodoluminescence, time-resolved µPL and photon autocorrelation experiments give a thorough evaluation of the QDs structural...

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Main Authors: Puchtler, T, Wang, T, Ren, C, Tang, F, Oliver, R, Taylor, R, Zhu, T
Format: Journal article
Published: American Chemical Society 2016
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author Puchtler, T
Wang, T
Ren, C
Tang, F
Oliver, R
Taylor, R
Zhu, T
author_facet Puchtler, T
Wang, T
Ren, C
Tang, F
Oliver, R
Taylor, R
Zhu, T
author_sort Puchtler, T
collection OXFORD
description We demonstrate single photon emission from self-assembled m-plane InGaN quantum dots (QDs) embedded on the side-walls of GaN nanowires. A combination of electron microscopy, cathodoluminescence, time-resolved µPL and photon autocorrelation experiments give a thorough evaluation of the QDs structural and optical properties. The QD exhibits anti-bunched emission up to 100 K, with a measured autocorrelation function of g^((2) ) (0) = 0.28 (0.03) at 5 K. Studies on a statistically significant number of QDs show that these m-plane QDs exhibit very fast radiative lifetimes (260 ± 55 ps) suggesting smaller internal fields than any of the previously reported c-plane and a-plane QDs. Moreover, the observed single photons are almost completely linearly polarized aligned perpendicular to the crystallographic c-axis with a degree of linear polarization of 0.84 ± 0.12. Such InGaN QDs incorporated in a nanowire system meet many of the requirements for implementation into quantum information systems and could potentially open the door to wholly new device concepts.
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spelling oxford-uuid:0ec2786f-c9a2-424b-aed4-191f3d8b0cc02022-03-26T09:47:40ZUltrafast, polarized, single-photon emission from m-plane InGaN Quantum Dots on GaN nanowiresJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:0ec2786f-c9a2-424b-aed4-191f3d8b0cc0Symplectic Elements at OxfordAmerican Chemical Society2016Puchtler, TWang, TRen, CTang, FOliver, RTaylor, RZhu, TWe demonstrate single photon emission from self-assembled m-plane InGaN quantum dots (QDs) embedded on the side-walls of GaN nanowires. A combination of electron microscopy, cathodoluminescence, time-resolved µPL and photon autocorrelation experiments give a thorough evaluation of the QDs structural and optical properties. The QD exhibits anti-bunched emission up to 100 K, with a measured autocorrelation function of g^((2) ) (0) = 0.28 (0.03) at 5 K. Studies on a statistically significant number of QDs show that these m-plane QDs exhibit very fast radiative lifetimes (260 ± 55 ps) suggesting smaller internal fields than any of the previously reported c-plane and a-plane QDs. Moreover, the observed single photons are almost completely linearly polarized aligned perpendicular to the crystallographic c-axis with a degree of linear polarization of 0.84 ± 0.12. Such InGaN QDs incorporated in a nanowire system meet many of the requirements for implementation into quantum information systems and could potentially open the door to wholly new device concepts.
spellingShingle Puchtler, T
Wang, T
Ren, C
Tang, F
Oliver, R
Taylor, R
Zhu, T
Ultrafast, polarized, single-photon emission from m-plane InGaN Quantum Dots on GaN nanowires
title Ultrafast, polarized, single-photon emission from m-plane InGaN Quantum Dots on GaN nanowires
title_full Ultrafast, polarized, single-photon emission from m-plane InGaN Quantum Dots on GaN nanowires
title_fullStr Ultrafast, polarized, single-photon emission from m-plane InGaN Quantum Dots on GaN nanowires
title_full_unstemmed Ultrafast, polarized, single-photon emission from m-plane InGaN Quantum Dots on GaN nanowires
title_short Ultrafast, polarized, single-photon emission from m-plane InGaN Quantum Dots on GaN nanowires
title_sort ultrafast polarized single photon emission from m plane ingan quantum dots on gan nanowires
work_keys_str_mv AT puchtlert ultrafastpolarizedsinglephotonemissionfrommplaneinganquantumdotsongannanowires
AT wangt ultrafastpolarizedsinglephotonemissionfrommplaneinganquantumdotsongannanowires
AT renc ultrafastpolarizedsinglephotonemissionfrommplaneinganquantumdotsongannanowires
AT tangf ultrafastpolarizedsinglephotonemissionfrommplaneinganquantumdotsongannanowires
AT oliverr ultrafastpolarizedsinglephotonemissionfrommplaneinganquantumdotsongannanowires
AT taylorr ultrafastpolarizedsinglephotonemissionfrommplaneinganquantumdotsongannanowires
AT zhut ultrafastpolarizedsinglephotonemissionfrommplaneinganquantumdotsongannanowires