Light-scattering study of phonon-magnon coupling in antiferromagnetic FeCl2. 2H2O

Raman spectroscopy has been used to study the phonon-magnon coupling in the antiferromagnetic phase of ferrous chloride dihydrate. The interaction has been studied as a function of temperature, from 2 K to TN=23 K, and applied field, from 0 to 28 kG. The phonon is assigned as a Bg symmetry libration...

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Main Authors: Kinne, R, O'Sullivan, W, Ryan, J, Scott, J
Format: Journal article
Language:English
Published: 1975
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author Kinne, R
O'Sullivan, W
Ryan, J
Scott, J
author_facet Kinne, R
O'Sullivan, W
Ryan, J
Scott, J
author_sort Kinne, R
collection OXFORD
description Raman spectroscopy has been used to study the phonon-magnon coupling in the antiferromagnetic phase of ferrous chloride dihydrate. The interaction has been studied as a function of temperature, from 2 K to TN=23 K, and applied field, from 0 to 28 kG. The phonon is assigned as a Bg symmetry libration mode, in accord with the predictions of Torrance and Slonczewski; it is found to be "soft," decreasing in energy as T→0. The phonon-magnon coupling constant is nearly field independent but decreases to zero at TN. It is found that no zero-field splitting of the magnon occurs, within 0.2-cm-1 instrumental resolution, in contrast to the 0.8-cm-1 splitting inferred from the infrared spectrum. The magnon g value is determined to be 1.7 ± 0.1, in contrast to Torrance's value of 2.23 ± 0.02. © 1975 The American Physical Society.
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spelling oxford-uuid:0f686af5-55a1-4b4a-af6e-7643e7a6a1d82022-03-26T09:51:03ZLight-scattering study of phonon-magnon coupling in antiferromagnetic FeCl2. 2H2OJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:0f686af5-55a1-4b4a-af6e-7643e7a6a1d8EnglishSymplectic Elements at Oxford1975Kinne, RO'Sullivan, WRyan, JScott, JRaman spectroscopy has been used to study the phonon-magnon coupling in the antiferromagnetic phase of ferrous chloride dihydrate. The interaction has been studied as a function of temperature, from 2 K to TN=23 K, and applied field, from 0 to 28 kG. The phonon is assigned as a Bg symmetry libration mode, in accord with the predictions of Torrance and Slonczewski; it is found to be "soft," decreasing in energy as T→0. The phonon-magnon coupling constant is nearly field independent but decreases to zero at TN. It is found that no zero-field splitting of the magnon occurs, within 0.2-cm-1 instrumental resolution, in contrast to the 0.8-cm-1 splitting inferred from the infrared spectrum. The magnon g value is determined to be 1.7 ± 0.1, in contrast to Torrance's value of 2.23 ± 0.02. © 1975 The American Physical Society.
spellingShingle Kinne, R
O'Sullivan, W
Ryan, J
Scott, J
Light-scattering study of phonon-magnon coupling in antiferromagnetic FeCl2. 2H2O
title Light-scattering study of phonon-magnon coupling in antiferromagnetic FeCl2. 2H2O
title_full Light-scattering study of phonon-magnon coupling in antiferromagnetic FeCl2. 2H2O
title_fullStr Light-scattering study of phonon-magnon coupling in antiferromagnetic FeCl2. 2H2O
title_full_unstemmed Light-scattering study of phonon-magnon coupling in antiferromagnetic FeCl2. 2H2O
title_short Light-scattering study of phonon-magnon coupling in antiferromagnetic FeCl2. 2H2O
title_sort light scattering study of phonon magnon coupling in antiferromagnetic fecl2 2h2o
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AT scottj lightscatteringstudyofphononmagnoncouplinginantiferromagneticfecl22h2o