Ab initio cycloidal and chiral magnetoelectric responses in Cr2 O3

We present a thorough density functional theory study of the magneto-electric (ME) effect in Cr2O3. The spin-lattice ME tensor α was determined in the low-field and spin flop (SF) phases, using the method of dynamical magnetic charges, and found to be the sum of three distinct components. Two of the...

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Príomhchruthaitheoirí: Tillack, N, Yates, J, Radaelli, P
Formáid: Journal article
Foilsithe / Cruthaithe: American Physical Society 2016
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Achoimre:We present a thorough density functional theory study of the magneto-electric (ME) effect in Cr2O3. The spin-lattice ME tensor α was determined in the low-field and spin flop (SF) phases, using the method of dynamical magnetic charges, and found to be the sum of three distinct components. Two of them, a large relativistic "cycloidal" term and a small longitudinal term, are independent on the spin orientation. The third, only active in the SF phases is also of relativistic origin and arises from magnetic-field-induced chirality, leading to a non-toroidal ME response.