Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera
Laser-induced adiabatic alignment and mixed-field orientation of 2,6-difluoroiodobenzene (C6H3F2I) molecules are probed by Coulomb explosion imaging following either near-infrared strong-field ionization or extreme-ultraviolet multi-photon inner-shell ionization using free-electron laser pulses. The...
| Main Authors: | , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , , |
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| Format: | Journal article |
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AIP Publishing
2017
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| _version_ | 1826263810478964736 |
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| author | Amini, K Boll, R Lauer, A Burt, M Lee, J Christensen, L Brauβe, F Mullins, T Savelyev, E Ablikim, U Berrah, N Bomme, C Düsterer, S Erk, B Höppner, H Johnsson, P Kierspel, T Krecinic, F Küpper, J Müller, M Müller, E Redlin, H Rouzée, A Schirmel, N Thøgersen, J Techert, S Toleikis, S Treusch, R Trippel, S Ulmer, A Wiese, J Vallance, C Rudenko, A Stapelfeldt, H Brouard, M Rolles, D |
| author_facet | Amini, K Boll, R Lauer, A Burt, M Lee, J Christensen, L Brauβe, F Mullins, T Savelyev, E Ablikim, U Berrah, N Bomme, C Düsterer, S Erk, B Höppner, H Johnsson, P Kierspel, T Krecinic, F Küpper, J Müller, M Müller, E Redlin, H Rouzée, A Schirmel, N Thøgersen, J Techert, S Toleikis, S Treusch, R Trippel, S Ulmer, A Wiese, J Vallance, C Rudenko, A Stapelfeldt, H Brouard, M Rolles, D |
| author_sort | Amini, K |
| collection | OXFORD |
| description | Laser-induced adiabatic alignment and mixed-field orientation of 2,6-difluoroiodobenzene (C6H3F2I) molecules are probed by Coulomb explosion imaging following either near-infrared strong-field ionization or extreme-ultraviolet multi-photon inner-shell ionization using free-electron laser pulses. The resulting photoelectrons and fragment ions are captured by a double-sided velocity map imaging spectrometer and projected onto two position-sensitive detectors. The ion side of the spectrometer is equipped with a pixel imaging mass spectrometry camera, a time-stamping pixelated detector that can record the hit positions and arrival times of up to four ions per pixel per acquisition cycle. Thus, the time-of-flight trace and ion momentum distributions for all fragments can be recorded simultaneously. We show that we can obtain a high degree of one-and three-dimensional alignment and mixed-field orientation and compare the Coulomb explosion process induced at both wavelengths. |
| first_indexed | 2024-03-06T19:57:46Z |
| format | Journal article |
| id | oxford-uuid:263b1ebb-0e63-4cab-8602-c7fcbc69f620 |
| institution | University of Oxford |
| last_indexed | 2024-03-06T19:57:46Z |
| publishDate | 2017 |
| publisher | AIP Publishing |
| record_format | dspace |
| spelling | oxford-uuid:263b1ebb-0e63-4cab-8602-c7fcbc69f6202022-03-26T11:59:49ZAlignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) cameraJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:263b1ebb-0e63-4cab-8602-c7fcbc69f620Symplectic Elements at OxfordAIP Publishing2017Amini, KBoll, RLauer, ABurt, MLee, JChristensen, LBrauβe, FMullins, TSavelyev, EAblikim, UBerrah, NBomme, CDüsterer, SErk, BHöppner, HJohnsson, PKierspel, TKrecinic, FKüpper, JMüller, MMüller, ERedlin, HRouzée, ASchirmel, NThøgersen, JTechert, SToleikis, STreusch, RTrippel, SUlmer, AWiese, JVallance, CRudenko, AStapelfeldt, HBrouard, MRolles, DLaser-induced adiabatic alignment and mixed-field orientation of 2,6-difluoroiodobenzene (C6H3F2I) molecules are probed by Coulomb explosion imaging following either near-infrared strong-field ionization or extreme-ultraviolet multi-photon inner-shell ionization using free-electron laser pulses. The resulting photoelectrons and fragment ions are captured by a double-sided velocity map imaging spectrometer and projected onto two position-sensitive detectors. The ion side of the spectrometer is equipped with a pixel imaging mass spectrometry camera, a time-stamping pixelated detector that can record the hit positions and arrival times of up to four ions per pixel per acquisition cycle. Thus, the time-of-flight trace and ion momentum distributions for all fragments can be recorded simultaneously. We show that we can obtain a high degree of one-and three-dimensional alignment and mixed-field orientation and compare the Coulomb explosion process induced at both wavelengths. |
| spellingShingle | Amini, K Boll, R Lauer, A Burt, M Lee, J Christensen, L Brauβe, F Mullins, T Savelyev, E Ablikim, U Berrah, N Bomme, C Düsterer, S Erk, B Höppner, H Johnsson, P Kierspel, T Krecinic, F Küpper, J Müller, M Müller, E Redlin, H Rouzée, A Schirmel, N Thøgersen, J Techert, S Toleikis, S Treusch, R Trippel, S Ulmer, A Wiese, J Vallance, C Rudenko, A Stapelfeldt, H Brouard, M Rolles, D Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera |
| title | Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera |
| title_full | Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera |
| title_fullStr | Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera |
| title_full_unstemmed | Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera |
| title_short | Alignment, orientation, and Coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry (PImMS) camera |
| title_sort | alignment orientation and coulomb explosion of difluoroiodobenzene studied with the pixel imaging mass spectrometry pimms camera |
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