Vibrationally coherent crossing and coupling of electronic states during internal conversion in β-carotene.
Coupling of nuclear and electronic degrees of freedom mediates energy flow in molecules after optical excitation. The associated coherent dynamics in polyatomic systems, however, remain experimentally unexplored. Here, we combined transient absorption spectroscopy with electronic population control...
| Main Authors: | , , |
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| Format: | Journal article |
| Language: | English |
| Published: |
American Physical Society
2014
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