Spatially reconfigurable antiferromagnetic states in topologically rich free-standing nanomembranes

Antiferromagnets hosting real-space topological textures are promising platforms to model fundamental ultrafast phenomena and explore spintronics. However, they have only been epitaxially fabricated on specific symmetry-matched substrates, thereby preserving their intrinsic magneto-crystalline order...

Full description

Bibliographic Details
Main Authors: Jani, H, Harrison, J, Hooda, S, Prakash, S, Nandi, P, Hu, J, Zeng, Z, Lin, J, Godfrey, C, Omar, GJ, Butcher, TA, Raabe, J, Finizio, S, Thean, AV, Ariando, A, Radaelli, PG
Format: Journal article
Language:English
Published: Nature Research 2024
_version_ 1826314898154455040
author Jani, H
Harrison, J
Hooda, S
Prakash, S
Nandi, P
Hu, J
Zeng, Z
Lin, J
Godfrey, C
Omar, GJ
Butcher, TA
Raabe, J
Finizio, S
Thean, AV
Ariando, A
Radaelli, PG
author_facet Jani, H
Harrison, J
Hooda, S
Prakash, S
Nandi, P
Hu, J
Zeng, Z
Lin, J
Godfrey, C
Omar, GJ
Butcher, TA
Raabe, J
Finizio, S
Thean, AV
Ariando, A
Radaelli, PG
author_sort Jani, H
collection OXFORD
description Antiferromagnets hosting real-space topological textures are promising platforms to model fundamental ultrafast phenomena and explore spintronics. However, they have only been epitaxially fabricated on specific symmetry-matched substrates, thereby preserving their intrinsic magneto-crystalline order. This curtails their integration with dissimilar supports, restricting the scope of fundamental and applied investigations. Here we circumvent this limitation by designing detachable crystalline antiferromagnetic nanomembranes of α-Fe2O3. First, we show—via transmission-based antiferromagnetic vector mapping—that flat nanomembranes host a spin-reorientation transition and rich topological phenomenology. Second, we exploit their extreme flexibility to demonstrate the reconfiguration of antiferromagnetic states across three-dimensional membrane folds resulting from flexure-induced strains. Finally, we combine these developments using a controlled manipulator to realize the strain-driven non-thermal generation of topological textures at room temperature. The integration of such free-standing antiferromagnetic layers with flat/curved nanostructures could enable spin texture designs via magnetoelastic/geometric effects in the quasi-static and dynamical regimes, opening new explorations into curvilinear antiferromagnetism and unconventional computing.
first_indexed 2024-09-25T04:15:09Z
format Journal article
id oxford-uuid:393fded3-3df7-4fd3-ba5e-046478e89831
institution University of Oxford
language English
last_indexed 2024-12-09T03:14:45Z
publishDate 2024
publisher Nature Research
record_format dspace
spelling oxford-uuid:393fded3-3df7-4fd3-ba5e-046478e898312024-10-16T09:44:18ZSpatially reconfigurable antiferromagnetic states in topologically rich free-standing nanomembranesJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:393fded3-3df7-4fd3-ba5e-046478e89831EnglishJisc Publications RouterNature Research2024Jani, HHarrison, JHooda, SPrakash, SNandi, PHu, JZeng, ZLin, JGodfrey, COmar, GJButcher, TARaabe, JFinizio, SThean, AVAriando, ARadaelli, PGAntiferromagnets hosting real-space topological textures are promising platforms to model fundamental ultrafast phenomena and explore spintronics. However, they have only been epitaxially fabricated on specific symmetry-matched substrates, thereby preserving their intrinsic magneto-crystalline order. This curtails their integration with dissimilar supports, restricting the scope of fundamental and applied investigations. Here we circumvent this limitation by designing detachable crystalline antiferromagnetic nanomembranes of α-Fe2O3. First, we show—via transmission-based antiferromagnetic vector mapping—that flat nanomembranes host a spin-reorientation transition and rich topological phenomenology. Second, we exploit their extreme flexibility to demonstrate the reconfiguration of antiferromagnetic states across three-dimensional membrane folds resulting from flexure-induced strains. Finally, we combine these developments using a controlled manipulator to realize the strain-driven non-thermal generation of topological textures at room temperature. The integration of such free-standing antiferromagnetic layers with flat/curved nanostructures could enable spin texture designs via magnetoelastic/geometric effects in the quasi-static and dynamical regimes, opening new explorations into curvilinear antiferromagnetism and unconventional computing.
spellingShingle Jani, H
Harrison, J
Hooda, S
Prakash, S
Nandi, P
Hu, J
Zeng, Z
Lin, J
Godfrey, C
Omar, GJ
Butcher, TA
Raabe, J
Finizio, S
Thean, AV
Ariando, A
Radaelli, PG
Spatially reconfigurable antiferromagnetic states in topologically rich free-standing nanomembranes
title Spatially reconfigurable antiferromagnetic states in topologically rich free-standing nanomembranes
title_full Spatially reconfigurable antiferromagnetic states in topologically rich free-standing nanomembranes
title_fullStr Spatially reconfigurable antiferromagnetic states in topologically rich free-standing nanomembranes
title_full_unstemmed Spatially reconfigurable antiferromagnetic states in topologically rich free-standing nanomembranes
title_short Spatially reconfigurable antiferromagnetic states in topologically rich free-standing nanomembranes
title_sort spatially reconfigurable antiferromagnetic states in topologically rich free standing nanomembranes
work_keys_str_mv AT janih spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT harrisonj spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT hoodas spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT prakashs spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT nandip spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT huj spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT zengz spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT linj spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT godfreyc spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT omargj spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT butcherta spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT raabej spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT finizios spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT theanav spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT ariandoa spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes
AT radaellipg spatiallyreconfigurableantiferromagneticstatesintopologicallyrichfreestandingnanomembranes