Magnetic ordering in Cr-doped Bi₂Se₃ thin films

We report the structural and magnetic study of Cr-doped Bi2Se3 thin films using x-ray diffraction (XRD), magnetometry and polarized neutron reflectometry (PNR). Epitaxial layers were grown on c-plane sapphire by molecular beam epitaxy in a two-step process. Highresolution XRD shows the exceptionally...

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Main Authors: Collins-Mcintyre, LJ, Harrison, SE, Schoenherr, P, Steinke, N-J, Kinane, CJ, Charlton, TR, Alba-Veneroa, D, Phusp, A, Kellock, AJ, Parkin, SSP, Harris, JS, Langridge, S, van der Laan, G, Hesjedal, T
Format: Journal article
Jezik:English
Izdano: European Physical Society 2014
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author Collins-Mcintyre, LJ
Harrison, SE
Schoenherr, P
Steinke, N-J
Kinane, CJ
Charlton, TR
Alba-Veneroa, D
Phusp, A
Kellock, AJ
Parkin, SSP
Harris, JS
Langridge, S
van der Laan, G
Hesjedal, T
author_facet Collins-Mcintyre, LJ
Harrison, SE
Schoenherr, P
Steinke, N-J
Kinane, CJ
Charlton, TR
Alba-Veneroa, D
Phusp, A
Kellock, AJ
Parkin, SSP
Harris, JS
Langridge, S
van der Laan, G
Hesjedal, T
author_sort Collins-Mcintyre, LJ
collection OXFORD
description We report the structural and magnetic study of Cr-doped Bi2Se3 thin films using x-ray diffraction (XRD), magnetometry and polarized neutron reflectometry (PNR). Epitaxial layers were grown on c-plane sapphire by molecular beam epitaxy in a two-step process. Highresolution XRD shows the exceptionally high crystalline quality of the doped films with no parasitic phases up to a Cr concentration of 12% (in % of the Bi sites occupied by substitutional Cr). The magnetic moment, measured by SQUID magnetometry, was found to be ∼2.1 μB per Cr ion. The magnetic hysteresis curve shows an open loop with a coercive field of ∼10 mT. The ferromagnetic transition temperature was determined to be 8.5 K analyzing the magnetizationtemperature gradient. PNR shows the film to be homogeneously ferromagnetic with no enhanced magnetism near the surface or interface.
first_indexed 2024-03-06T21:39:21Z
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spelling oxford-uuid:475e372e-f5c9-4897-a0c0-b090e5d7f61b2022-03-26T15:19:44ZMagnetic ordering in Cr-doped Bi₂Se₃ thin filmsJournal articlehttp://purl.org/coar/resource_type/c_dcae04bcuuid:475e372e-f5c9-4897-a0c0-b090e5d7f61bEnglishSymplectic Elements at OxfordEuropean Physical Society2014Collins-Mcintyre, LJHarrison, SESchoenherr, PSteinke, N-JKinane, CJCharlton, TRAlba-Veneroa, DPhusp, AKellock, AJParkin, SSPHarris, JSLangridge, Svan der Laan, GHesjedal, TWe report the structural and magnetic study of Cr-doped Bi2Se3 thin films using x-ray diffraction (XRD), magnetometry and polarized neutron reflectometry (PNR). Epitaxial layers were grown on c-plane sapphire by molecular beam epitaxy in a two-step process. Highresolution XRD shows the exceptionally high crystalline quality of the doped films with no parasitic phases up to a Cr concentration of 12% (in % of the Bi sites occupied by substitutional Cr). The magnetic moment, measured by SQUID magnetometry, was found to be ∼2.1 μB per Cr ion. The magnetic hysteresis curve shows an open loop with a coercive field of ∼10 mT. The ferromagnetic transition temperature was determined to be 8.5 K analyzing the magnetizationtemperature gradient. PNR shows the film to be homogeneously ferromagnetic with no enhanced magnetism near the surface or interface.
spellingShingle Collins-Mcintyre, LJ
Harrison, SE
Schoenherr, P
Steinke, N-J
Kinane, CJ
Charlton, TR
Alba-Veneroa, D
Phusp, A
Kellock, AJ
Parkin, SSP
Harris, JS
Langridge, S
van der Laan, G
Hesjedal, T
Magnetic ordering in Cr-doped Bi₂Se₃ thin films
title Magnetic ordering in Cr-doped Bi₂Se₃ thin films
title_full Magnetic ordering in Cr-doped Bi₂Se₃ thin films
title_fullStr Magnetic ordering in Cr-doped Bi₂Se₃ thin films
title_full_unstemmed Magnetic ordering in Cr-doped Bi₂Se₃ thin films
title_short Magnetic ordering in Cr-doped Bi₂Se₃ thin films
title_sort magnetic ordering in cr doped bi₂se₃ thin films
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